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The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer

Authorized Users Only
2021
Authors
Marinković, Aleksandar D.
Vuksanović, Marija M.
Karić, Nataša
Đokić, Veljko
Popović, Mina
Jančić Heinemann, Radmila
Tomić, Nataša Z.
Article (Published version)
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Abstract
As a renewable resource, starch is considered to be fully biodegradable and nonpolluting to the environment but the hygroscopicity of starch is the main disadvantage for wider applicability in the production of a polymer-based material. Hydrophobically modified starch prepared using natural-based plasticizers/modifiers in a first step ([−]-diisopropyl D-tartrate [DiPT], ricinoleic acid [RA] and epoxidized soybean oil [ESO]), and maleated polypropylene (MAPP) in a second step contributed to better compatibility, and thus reinforcing of composites. Tailored processing conditions, structural/morphological properties, hydrophobicity, and water-resistance of the modified starch were established. In addition, the Charpy impact and tensile strength of composites, based on poly(ethylene-co-acrylic acid) (EAA) and modified starches, were determined. Increased tensile strength and Young modulus of the composite using starch-modified with DiPT-MAPP, that is, 3 and 83%, respectively, indicated the... possible applicability of obtained materials.

Keywords:
composites / hydrophobic starch / mechanical properties / modification / structure-property relations
Source:
Polimer Composites, 2021, 42, 3, 1325-1337
Publisher:
  • Wiley
Funding / projects:
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200135 (University of Belgrade, Faculty of Technology and Metallurgy) (RS-200135)
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200287 (Innovation Center of the Faculty of Technology and Metallurgy) (RS-200287)

DOI: 10.1002/pc.25903

ISSN: 0272-8397; 1548-0569

WoS: 000596432200001

Scopus: 2-s2.0-85097298341
[ Google Scholar ]
4
2
URI
https://cer.ihtm.bg.ac.rs/handle/123456789/4828
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
IHTM
TY  - JOUR
AU  - Marinković, Aleksandar D.
AU  - Vuksanović, Marija M.
AU  - Karić, Nataša
AU  - Đokić, Veljko
AU  - Popović, Mina
AU  - Jančić  Heinemann, Radmila
AU  - Tomić, Nataša Z.
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4828
AB  - As a renewable resource, starch is considered to be fully biodegradable and nonpolluting to the environment but the hygroscopicity of starch is the main disadvantage for wider applicability in the production of a polymer-based material. Hydrophobically modified starch prepared using natural-based plasticizers/modifiers in a first step ([−]-diisopropyl D-tartrate [DiPT], ricinoleic acid [RA] and epoxidized soybean oil [ESO]), and maleated polypropylene (MAPP) in a second step contributed to better compatibility, and thus reinforcing of composites. Tailored processing conditions, structural/morphological properties, hydrophobicity, and water-resistance of the modified starch were established. In addition, the Charpy impact and tensile strength of composites, based on poly(ethylene-co-acrylic acid) (EAA) and modified starches, were determined. Increased tensile strength and Young modulus of the composite using starch-modified with DiPT-MAPP, that is, 3 and 83%, respectively, indicated the possible applicability of obtained materials.
PB  - Wiley
T2  - Polimer Composites
T1  - The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer
VL  - 42
IS  - 3
SP  - 1325
EP  - 1337
DO  - 10.1002/pc.25903
ER  - 
@article{
author = "Marinković, Aleksandar D. and Vuksanović, Marija M. and Karić, Nataša and Đokić, Veljko and Popović, Mina and Jančić  Heinemann, Radmila and Tomić, Nataša Z.",
year = "2021",
abstract = "As a renewable resource, starch is considered to be fully biodegradable and nonpolluting to the environment but the hygroscopicity of starch is the main disadvantage for wider applicability in the production of a polymer-based material. Hydrophobically modified starch prepared using natural-based plasticizers/modifiers in a first step ([−]-diisopropyl D-tartrate [DiPT], ricinoleic acid [RA] and epoxidized soybean oil [ESO]), and maleated polypropylene (MAPP) in a second step contributed to better compatibility, and thus reinforcing of composites. Tailored processing conditions, structural/morphological properties, hydrophobicity, and water-resistance of the modified starch were established. In addition, the Charpy impact and tensile strength of composites, based on poly(ethylene-co-acrylic acid) (EAA) and modified starches, were determined. Increased tensile strength and Young modulus of the composite using starch-modified with DiPT-MAPP, that is, 3 and 83%, respectively, indicated the possible applicability of obtained materials.",
publisher = "Wiley",
journal = "Polimer Composites",
title = "The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer",
volume = "42",
number = "3",
pages = "1325-1337",
doi = "10.1002/pc.25903"
}
Marinković, A. D., Vuksanović, M. M., Karić, N., Đokić, V., Popović, M., Jančić  Heinemann, R.,& Tomić, N. Z.. (2021). The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer. in Polimer Composites
Wiley., 42(3), 1325-1337.
https://doi.org/10.1002/pc.25903
Marinković AD, Vuksanović MM, Karić N, Đokić V, Popović M, Jančić  Heinemann R, Tomić NZ. The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer. in Polimer Composites. 2021;42(3):1325-1337.
doi:10.1002/pc.25903 .
Marinković, Aleksandar D., Vuksanović, Marija M., Karić, Nataša, Đokić, Veljko, Popović, Mina, Jančić  Heinemann, Radmila, Tomić, Nataša Z., "The effect of natural modifiers for starch hydrophobization on performance of composite based on ethylene acrylic acid copolymer" in Polimer Composites, 42, no. 3 (2021):1325-1337,
https://doi.org/10.1002/pc.25903 . .

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