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dc.creatorNikolić, Daliborka
dc.creatorSeidel, Carsten
dc.creatorFelischak, Matthias
dc.creatorMiličić, Tamara
dc.creatorKienle, Achim
dc.creatorSeidel-Morgenstern, Andreas
dc.creatorPetkovska, Menka
dc.date.accessioned2021-10-27T13:35:52Z
dc.date.available2023-09-21
dc.date.issued2022
dc.identifier.issn0009-2509
dc.identifier.urihttps://cer.ihtm.bg.ac.rs/handle/123456789/4819
dc.description.abstractIn this two-part paper a comprehensive study of the potential to improve performance criteria of a methanol synthesis reactor through forced periodical operations is presented. The study uses the Nonlinear Frequency Response method, a powerful analytical and approximate tool which gives an answer whether and under which conditions certain periodic operation would lead to improvement of process performance. To demonstrate the method, isothermal and isobaric methanol synthesis in a lab-scale CSTR is considered. In Part I, the analysis is performed for single input modulations. Partial pressures of each reactant in the feed stream and the total inlet volumetric flow-rate are considered as possible modulated inputs. The results show that modulations of single inputs essentially do not provide potential for significant improvements. In Part II, the study will be extended to analysis of periodic operations with simultaneous modulations of two inputs and conditions offering significant performance enhancements will be identified.sr
dc.language.isoensr
dc.publisherElseviersr
dc.relationinfo:eu-repo/grantAgreement/MESTD/inst-2020/200135/RS//sr
dc.relationThe German Research Foundation, grant PE 2915/1-1sr
dc.relationThe German Research Foundation, Kl 417/6-1sr
dc.relationThe German Research Foundation, SE 586/24-1sr
dc.relation.isversionofhttps://doi.org/10.1016/j.ces.2021.117134
dc.relation.isversionofhttps://cer.ihtm.bg.ac.rs/handle/123456789/4813
dc.rightsembargoedAccesssr
dc.rights.urihttps://creativecommons.org/licenses/by-nc-nd/4.0/
dc.sourceChemical Engineering Sciencesr
dc.subjectForced periodic operationssr
dc.subjectMethanol synthesissr
dc.subjectNonlinear frequency responsesr
dc.subjectProcess improvementsr
dc.subjectSingle input modulationssr
dc.titleForced periodic operations of a chemical reactor for methanol synthesis – The search for the best scenario based on Nonlinear Frequency Response Method. Part I Single input modulationssr
dc.typearticlesr
dc.rights.licenseBY-NC-NDsr
dcterms.abstractФелисцхак, Маттхиас; Миличић, Тамара; Киенле, Aцхим; Сеидел-Моргенстерн, Aндреас; Петковска, Менка; Николић, Далиборка; Сеидел, Царстен;
dc.citation.volume248
dc.citation.spage117134
dc.citation.rankM21~
dc.description.otherThis is the peer-reviewed version of the article: Daliborka Nikolić, Carsten Seidel, Matthias Felischak, Tamara Miličić, Achim Kienle, Andreas Seidel-Morgenstern, Menka Petkovska, Forced periodic operations of a chemical reactor for methanol synthesis – the search for the best scenario based on Nonlinear Frequency Response Method. Part I Single input modulations, Chemical Engineering Science, 2022, 248, 117134, doi: [https://doi.org/10.1016/j.ces.2021.117134]
dc.description.otherThe published version: [https://cer.ihtm.bg.ac.rs/handle/123456789/4813]
dc.identifier.doi10.1016/j.ces.2021.117134
dc.identifier.fulltexthttp://cer.ihtm.bg.ac.rs/bitstream/id/20990/acc_1-s2.0-S0009250921006990-main.pdf
dc.identifier.scopus2-s2.0-85116624953
dc.identifier.wos000709895200001
dc.type.versionacceptedVersionsr


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