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Visible light promoted photoredox C(sp3)-H bond functionalization of tetrahydroisoquinolines in flow
dc.creator | Filipović, Ana | |
dc.creator | Džambaski, Zdravko | |
dc.creator | Vasiljević-Radović, Dana | |
dc.creator | Bondžić, Bojan | |
dc.date.accessioned | 2021-04-23T13:12:32Z | |
dc.date.available | 2021-04-23T13:12:32Z | |
dc.date.issued | 2021 | |
dc.identifier.issn | 1477-0520 | |
dc.identifier.uri | https://cer.ihtm.bg.ac.rs/handle/123456789/4494 | |
dc.description.abstract | A merger of organocatalysis and visible light photoredox catalysis performed in flow allowed access to a wide range of functionalizedN-aryl-substituted tetrahydroisoquinolines (THIQs) in a formal C-H oxidation/Mannich reaction. Strecker type functionalization and copper-catalyzed alkynylation of severalN-aryl-substituted THIQs were also successfully performed in flow, giving valuable products with high efficiencies. The use of custom-made porous polymeric type microreactors proved to be crucial regarding the C-H oxidation step and overall reaction performance. | sr |
dc.language.iso | en | sr |
dc.publisher | Royal Society of Chemistry | sr |
dc.relation | info:eu-repo/grantAgreement/MESTD/inst-2020/200026/RS// | sr |
dc.relation | The Proof of Concept project of Innovation Fund of Republic of Serbia no. 5183. | sr |
dc.relation.isreferencedby | https://cer.ihtm.bg.ac.rs/handle/123456789/4495 | |
dc.rights | restrictedAccess | sr |
dc.source | Organic and Biomolecular Chemistry | sr |
dc.subject | Light | sr |
dc.subject | Catalysis | sr |
dc.subject | Alkynylations | sr |
dc.subject | Copper catalyzed | sr |
dc.subject | Functionalizations | sr |
dc.subject | Micro reactor | sr |
dc.subject | Organocatalysis | sr |
dc.subject | Overall reactions | sr |
dc.subject | Photoredox catalysis | sr |
dc.subject | Tetrahydroisoquinolines | sr |
dc.title | Visible light promoted photoredox C(sp3)-H bond functionalization of tetrahydroisoquinolines in flow | sr |
dc.type | article | sr |
dc.rights.license | ARR | sr |
dcterms.abstract | Джамбаски, Здравко; Филиповић, Aна; Васиљевић-Радовић, Дана; Бонджић, Бојан; | |
dc.citation.volume | 19 | |
dc.citation.issue | 12 | |
dc.citation.spage | 2668 | |
dc.citation.epage | 2675 | |
dc.citation.rank | M21~ | |
dc.description.other | Supplementary material: [https://cer.ihtm.bg.ac.rs/handle/123456789/4495] | |
dc.identifier.pmid | 33666639 | |
dc.identifier.doi | 10.1039/d0ob02582h | |
dc.identifier.scopus | 2-s2.0-85103475295 | |
dc.identifier.wos | 000635741400006 | |
dc.type.version | publishedVersion | sr |