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Visible light promoted photoredox C(sp3)-H bond functionalization of tetrahydroisoquinolines in flow

dc.creatorFilipović, Ana
dc.creatorDžambaski, Zdravko
dc.creatorVasiljević-Radović, Dana
dc.creatorBondžić, Bojan
dc.date.accessioned2021-04-23T13:12:32Z
dc.date.available2021-04-23T13:12:32Z
dc.date.issued2021
dc.identifier.issn1477-0520
dc.identifier.urihttps://cer.ihtm.bg.ac.rs/handle/123456789/4494
dc.description.abstractA merger of organocatalysis and visible light photoredox catalysis performed in flow allowed access to a wide range of functionalizedN-aryl-substituted tetrahydroisoquinolines (THIQs) in a formal C-H oxidation/Mannich reaction. Strecker type functionalization and copper-catalyzed alkynylation of severalN-aryl-substituted THIQs were also successfully performed in flow, giving valuable products with high efficiencies. The use of custom-made porous polymeric type microreactors proved to be crucial regarding the C-H oxidation step and overall reaction performance.sr
dc.language.isoensr
dc.publisherRoyal Society of Chemistrysr
dc.relationinfo:eu-repo/grantAgreement/MESTD/inst-2020/200026/RS//sr
dc.relationThe Proof of Concept project of Innovation Fund of Republic of Serbia no. 5183.sr
dc.relation.isreferencedbyhttps://cer.ihtm.bg.ac.rs/handle/123456789/4495
dc.rightsrestrictedAccesssr
dc.sourceOrganic and Biomolecular Chemistrysr
dc.subjectLightsr
dc.subjectCatalysissr
dc.subjectAlkynylationssr
dc.subjectCopper catalyzedsr
dc.subjectFunctionalizationssr
dc.subjectMicro reactorsr
dc.subjectOrganocatalysissr
dc.subjectOverall reactionssr
dc.subjectPhotoredox catalysissr
dc.subjectTetrahydroisoquinolinessr
dc.titleVisible light promoted photoredox C(sp3)-H bond functionalization of tetrahydroisoquinolines in flowsr
dc.typearticlesr
dc.rights.licenseARRsr
dcterms.abstractДжамбаски, Здравко; Филиповић, Aна; Васиљевић-Радовић, Дана; Бонджић, Бојан;
dc.citation.volume19
dc.citation.issue12
dc.citation.spage2668
dc.citation.epage2675
dc.citation.rankM21~
dc.description.otherSupplementary material: [https://cer.ihtm.bg.ac.rs/handle/123456789/4495]
dc.identifier.pmid33666639
dc.identifier.doi10.1039/d0ob02582h
dc.identifier.scopus2-s2.0-85103475295
dc.identifier.wos000635741400006
dc.type.versionpublishedVersionsr


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