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dc.creatorNikolić, Daliborka
dc.creatorSeidel, Carsten
dc.creatorKienle, Achim
dc.creatorSeidel-Morgenstern, Andreas
dc.creatorPetkovska, Menka
dc.date.accessioned2020-11-24T07:54:04Z
dc.date.available2020-11-24T07:54:04Z
dc.date.issued2019
dc.identifier.urihttps://kuleuvencongres.be/ipic2019/Home
dc.identifier.urihttps://cer.ihtm.bg.ac.rs/handle/123456789/3843
dc.description.abstractIn this work, the NFR method is implemented for evaluation of possible improvement for the reaction of methanol synthesis by hydrogenation of CO and CO2, using a standard Cu/ZnO/Al2O3 catalyst. For start, a forced periodically operated isothermal continuous-stirred tank reactor (CSTR) is considered. A simplified (lumped) kinetic model of methanol synthesis with 14 parameters which were estimated from the results of an extensive experimental investigation is used. The NFR method is performed for evaluation of possible increase of methanol production by modulating the mole fractions of CO and CO2 in the feed stream, as well as their simultaneous modulation. The necessary asymmetrical second order frequency response functions correlating the methanol production with the modulated inputs are derived and the forcing parameters leading to improvement of the reactor performance are determined. The results of the NFR analysis will further be used for rigorous optimisation of the forced periodic operations and planning the best experimental scenarios. The final step will be experimental investigation and confirmation on a laboratory scale reactor.en
dc.language.isoensr
dc.relationDFG Priority Programme 2080, SPP 2080 Catalyst and reactors under dynamic conditions for energy storage and conversionsr
dc.rightsopenAccesssr
dc.source2nd International Process Intensification Conference, Leuven, Belgiumsr
dc.subjectnonlinear frequency response analysissr
dc.subjectchemical reactorssr
dc.subjectmethanol synthesissr
dc.subjecthydrogenation of CO and CO2sr
dc.subjectcatalysissr
dc.titleIntensification of a chemical reactor for methanol synthesis through forced periodic operations- Evaluation based on Nonlinear Frequency Response Analysisen
dc.typeconferenceObjectsr
dc.rights.licenseBY-NC-NDsr
dcterms.abstractКиенле, Aцхим; Николић, Далиборка; Сеидел, Царстен; Сеидел-Моргенстерн, Aндреас; Петковска, Менка;
dc.description.otherIPIC 2, 27-29 May 2019, Leuven, Belgiumsr
dc.identifier.fulltexthttp://cer.ihtm.bg.ac.rs/bitstream/id/17888/Template_abstract_IPIC2_V2_Daliborka_2_menka.pdf
dc.type.versionpublishedVersionsr


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