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The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films

Authorized Users Only
2020
Authors
Kalifa, Mustafa
Tomić, Nataša Z.
Vuksanović, Marija M.
Stevanović, Sanja
Đokić, Veljko
Volkov-Husović, Tatjana
Pavlović, Vladimir B.
Jančić-Heinemann, Radmila
Marinković, Aleksandar D.
Article (Published version)
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Abstract
Cavitation erosion of hybrid acrylate composite films with polyhedral oligosilsesquioxanes (POSS) was investigated in this study. The hybrid films are made with 1, 3 and 5 wt% of POSS reagents containing: (a) hydroxyl (POSS-M), (b) both hydroxyl and allyl (POSS-M-A) and (c) methacryloyl groups (POSS-MCl). Addition of 5 wt% POSS-M-A caused the highest microhardness increase for 49.8%, in comparison to the pure matrix material. Cavitation resistance of hybrid films, estimated as the time-dependent mass loss, was improved by POSS addition. POSS-M-A addition (5 wt%) contributed to 94% lower mass loss comparing to pure Bis-GMA/TEGDMA film. Scanning electron (SEM) and atomic force microscopy (AFM) showed the lowest surface roughness obtained for composite with POSS-M-A. The improved hardness and wear resistance of the composite films indicated that POSS-M-A filler enhanced interfacial adhesion and reinforcing of the Bis-GMA/TEGDMA matrix.
Keywords:
cavitation erosion / coatings / crosslinking / microscopy / surfaces
Source:
Polymer Composites, 2020, 41, 8, 3403-3410
Publisher:
  • John Wiley and Sons Inc
Funding / projects:
  • Predefined functional properties polymer composite materials processes and equipment development (RS-34011)
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200135 (University of Belgrade, Faculty of Technology and Metallurgy) (RS-200135)

DOI: 10.1002/pc.25629

ISSN: 0272-8397; 1548-0569

WoS: 000532986100001

Scopus: 2-s2.0-85085014224
[ Google Scholar ]
1
URI
https://cer.ihtm.bg.ac.rs/handle/123456789/3589
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
IHTM
TY  - JOUR
AU  - Kalifa, Mustafa
AU  - Tomić, Nataša Z.
AU  - Vuksanović, Marija M.
AU  - Stevanović, Sanja
AU  - Đokić, Veljko
AU  - Volkov-Husović, Tatjana
AU  - Pavlović, Vladimir B.
AU  - Jančić-Heinemann, Radmila
AU  - Marinković, Aleksandar D.
PY  - 2020
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3589
AB  - Cavitation erosion of hybrid acrylate composite films with polyhedral
oligosilsesquioxanes (POSS) was investigated in this study. The hybrid films are
made with 1, 3 and 5 wt% of POSS reagents containing: (a) hydroxyl (POSS-M),
(b) both hydroxyl and allyl (POSS-M-A) and (c) methacryloyl groups (POSS-MCl).
Addition of 5 wt% POSS-M-A caused the highest microhardness increase for
49.8%, in comparison to the pure matrix material. Cavitation resistance of hybrid
films, estimated as the time-dependent mass loss, was improved by POSS addition.
POSS-M-A addition (5 wt%) contributed to 94% lower mass loss comparing
to pure Bis-GMA/TEGDMA film. Scanning electron (SEM) and atomic force
microscopy (AFM) showed the lowest surface roughness obtained for composite
with POSS-M-A. The improved hardness and wear resistance of the composite
films indicated that POSS-M-A filler enhanced interfacial adhesion and reinforcing
of the Bis-GMA/TEGDMA matrix.
PB  - John Wiley and Sons Inc
T2  - Polymer Composites
T1  - The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films
VL  - 41
IS  - 8
SP  - 3403
EP  - 3410
DO  - 10.1002/pc.25629
ER  - 
@article{
author = "Kalifa, Mustafa and Tomić, Nataša Z. and Vuksanović, Marija M. and Stevanović, Sanja and Đokić, Veljko and Volkov-Husović, Tatjana and Pavlović, Vladimir B. and Jančić-Heinemann, Radmila and Marinković, Aleksandar D.",
year = "2020",
abstract = "Cavitation erosion of hybrid acrylate composite films with polyhedral
oligosilsesquioxanes (POSS) was investigated in this study. The hybrid films are
made with 1, 3 and 5 wt% of POSS reagents containing: (a) hydroxyl (POSS-M),
(b) both hydroxyl and allyl (POSS-M-A) and (c) methacryloyl groups (POSS-MCl).
Addition of 5 wt% POSS-M-A caused the highest microhardness increase for
49.8%, in comparison to the pure matrix material. Cavitation resistance of hybrid
films, estimated as the time-dependent mass loss, was improved by POSS addition.
POSS-M-A addition (5 wt%) contributed to 94% lower mass loss comparing
to pure Bis-GMA/TEGDMA film. Scanning electron (SEM) and atomic force
microscopy (AFM) showed the lowest surface roughness obtained for composite
with POSS-M-A. The improved hardness and wear resistance of the composite
films indicated that POSS-M-A filler enhanced interfacial adhesion and reinforcing
of the Bis-GMA/TEGDMA matrix.",
publisher = "John Wiley and Sons Inc",
journal = "Polymer Composites",
title = "The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films",
volume = "41",
number = "8",
pages = "3403-3410",
doi = "10.1002/pc.25629"
}
Kalifa, M., Tomić, N. Z., Vuksanović, M. M., Stevanović, S., Đokić, V., Volkov-Husović, T., Pavlović, V. B., Jančić-Heinemann, R.,& Marinković, A. D.. (2020). The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films. in Polymer Composites
John Wiley and Sons Inc., 41(8), 3403-3410.
https://doi.org/10.1002/pc.25629
Kalifa M, Tomić NZ, Vuksanović MM, Stevanović S, Đokić V, Volkov-Husović T, Pavlović VB, Jančić-Heinemann R, Marinković AD. The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films. in Polymer Composites. 2020;41(8):3403-3410.
doi:10.1002/pc.25629 .
Kalifa, Mustafa, Tomić, Nataša Z., Vuksanović, Marija M., Stevanović, Sanja, Đokić, Veljko, Volkov-Husović, Tatjana, Pavlović, Vladimir B., Jančić-Heinemann, Radmila, Marinković, Aleksandar D., "The effect of polyhedral oligosilsesquioxanes (POSS) on cavitation resistance of hybrid acrylate films" in Polymer Composites, 41, no. 8 (2020):3403-3410,
https://doi.org/10.1002/pc.25629 . .

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