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Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties

Authorized Users Only
2019
Authors
Marković, Maja D.
Spasojević, Pavle
Šešlija, Sanja
Popović, Ivanka G.
Veljović, Đorđe
Pjanović, Rada
Panić, Vesna
Article (Published version)
,
Elsevier BV
Metadata
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Abstract
The design of complex polymeric materials with predefined task-specific properties meets challenging issues: to establish synthesis-structure-properties relationship, as well as to understand the arrangement and interactions of the involved components. Hybrid networks of protein (casein) and polyelectrolyte (poly(methacrylic acid)) were synthesized and their swelling, dynamic-mechanical and morphological properties were investigated as functions of the neutralization degree of methacrylic acid and the concentrations of caseinate and crosslinker. The domination of different interactions between components led to diverse forms of casein macromolecules- from micelles to unfold chains. That resulted in very different structures and thereby properties of derived hybrid networks: from porous unswellable to highly swellable and reinforced ones. A great opportunity to easily modulate the final characteristics of the reported hybrid system to fit the need of specific application just through th...e change of one synthesis parameter was thereby demonstrated.

Keywords:
Casein / Hybrid polymer network / Poly(methacrylic acid) / Synthesis-structure-properties relationship
Source:
European Polymer Journal, 2019, 113, 276-288
Publisher:
  • Elsevier
Funding / projects:
  • Synthesis and characterization of novel functional polymers and polymeric nanocomposites (RS-172062)
  • Novel encapsulation and enzyme technologies for designing of new biocatalysts and biologically active compounds targeting enhancement of food quality, safety and competitiveness (RS-46010)

DOI: 10.1016/j.eurpolymj.2019.01.065

ISSN: 00143057

WoS: 000463979200032

Scopus: 2-s2.0-85060975410
[ Google Scholar ]
8
6
URI
https://cer.ihtm.bg.ac.rs/handle/123456789/2990
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
IHTM
TY  - JOUR
AU  - Marković, Maja D.
AU  - Spasojević, Pavle
AU  - Šešlija, Sanja
AU  - Popović, Ivanka G.
AU  - Veljović, Đorđe
AU  - Pjanović, Rada
AU  - Panić, Vesna
PY  - 2019
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/2990
AB  - The design of complex polymeric materials with predefined task-specific properties meets challenging issues: to establish synthesis-structure-properties relationship, as well as to understand the arrangement and interactions of the involved components. Hybrid networks of protein (casein) and polyelectrolyte (poly(methacrylic acid)) were synthesized and their swelling, dynamic-mechanical and morphological properties were investigated as functions of the neutralization degree of methacrylic acid and the concentrations of caseinate and crosslinker. The domination of different interactions between components led to diverse forms of casein macromolecules- from micelles to unfold chains. That resulted in very different structures and thereby properties of derived hybrid networks: from porous unswellable to highly swellable and reinforced ones. A great opportunity to easily modulate the final characteristics of the reported hybrid system to fit the need of specific application just through the change of one synthesis parameter was thereby demonstrated.
PB  - Elsevier
T2  - European Polymer Journal
T1  - Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties
VL  - 113
SP  - 276
EP  - 288
DO  - 10.1016/j.eurpolymj.2019.01.065
ER  - 
@article{
author = "Marković, Maja D. and Spasojević, Pavle and Šešlija, Sanja and Popović, Ivanka G. and Veljović, Đorđe and Pjanović, Rada and Panić, Vesna",
year = "2019",
abstract = "The design of complex polymeric materials with predefined task-specific properties meets challenging issues: to establish synthesis-structure-properties relationship, as well as to understand the arrangement and interactions of the involved components. Hybrid networks of protein (casein) and polyelectrolyte (poly(methacrylic acid)) were synthesized and their swelling, dynamic-mechanical and morphological properties were investigated as functions of the neutralization degree of methacrylic acid and the concentrations of caseinate and crosslinker. The domination of different interactions between components led to diverse forms of casein macromolecules- from micelles to unfold chains. That resulted in very different structures and thereby properties of derived hybrid networks: from porous unswellable to highly swellable and reinforced ones. A great opportunity to easily modulate the final characteristics of the reported hybrid system to fit the need of specific application just through the change of one synthesis parameter was thereby demonstrated.",
publisher = "Elsevier",
journal = "European Polymer Journal",
title = "Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties",
volume = "113",
pages = "276-288",
doi = "10.1016/j.eurpolymj.2019.01.065"
}
Marković, M. D., Spasojević, P., Šešlija, S., Popović, I. G., Veljović, Đ., Pjanović, R.,& Panić, V.. (2019). Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties. in European Polymer Journal
Elsevier., 113, 276-288.
https://doi.org/10.1016/j.eurpolymj.2019.01.065
Marković MD, Spasojević P, Šešlija S, Popović IG, Veljović Đ, Pjanović R, Panić V. Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties. in European Polymer Journal. 2019;113:276-288.
doi:10.1016/j.eurpolymj.2019.01.065 .
Marković, Maja D., Spasojević, Pavle, Šešlija, Sanja, Popović, Ivanka G., Veljović, Đorđe, Pjanović, Rada, Panić, Vesna, "Casein-poly(methacrylic acid) hybrid soft networks with easy tunable properties" in European Polymer Journal, 113 (2019):276-288,
https://doi.org/10.1016/j.eurpolymj.2019.01.065 . .

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