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Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor

Authorized Users Only
2016
Authors
Nikolić-Paunić, Daliborka
Felischak, Matthias
Seidel-Morgenstern, Andreas
Petkovska, Menka
Article (Published version)
Metadata
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Abstract
The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred-tank reactor (CSTR) when inlet concentration and/or flow rate are periodically modulated. The product yield was used for evaluating the performance improvements. Part I of this paper considered the general nonisothermal case. In this part, the results are applied to an adiabatic CSTR. A laboratory-scale adiabatic CSTR was analyzed by applying kinetic parameters for the hydrolysis of acetic anhydride. It is shown that improvement can be obtained for simultaneous modulation of the two inputs with appropriately chosen forcing parameters.
Keywords:
Adiabatic CSTR / Nonlinear frequency response / Periodic operation / Reactor modeling / Two-input modulation
Source:
Chemical Engineering & Technology, 2016, 39, 11, 2126-2134
Publisher:
  • Wiley-V C H Verlag Gmbh, Weinheim
Funding / projects:
  • The development of efficient chemical-engineering processes based on the transport phenomena research and process intensification principles (RS-172022)
  • Nanostructured Functional and Composite Materials in Catalytic and Sorption Processes (RS-45001)

DOI: 10.1002/ceat.201600187

ISSN: 0930-7516

WoS: 000387766900017

Scopus: 2-s2.0-84992061278
[ Google Scholar ]
12
11
URI
https://cer.ihtm.bg.ac.rs/handle/123456789/1890
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
IHTM
TY  - JOUR
AU  - Nikolić-Paunić, Daliborka
AU  - Felischak, Matthias
AU  - Seidel-Morgenstern, Andreas
AU  - Petkovska, Menka
PY  - 2016
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/1890
AB  - The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred-tank reactor (CSTR) when inlet concentration and/or flow rate are periodically modulated. The product yield was used for evaluating the performance improvements. Part I of this paper considered the general nonisothermal case. In this part, the results are applied to an adiabatic CSTR. A laboratory-scale adiabatic CSTR was analyzed by applying kinetic parameters for the hydrolysis of acetic anhydride. It is shown that improvement can be obtained for simultaneous modulation of the two inputs with appropriately chosen forcing parameters.
PB  - Wiley-V C H Verlag Gmbh, Weinheim
T2  - Chemical Engineering & Technology
T1  - Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor
VL  - 39
IS  - 11
SP  - 2126
EP  - 2134
DO  - 10.1002/ceat.201600187
ER  - 
@article{
author = "Nikolić-Paunić, Daliborka and Felischak, Matthias and Seidel-Morgenstern, Andreas and Petkovska, Menka",
year = "2016",
abstract = "The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred-tank reactor (CSTR) when inlet concentration and/or flow rate are periodically modulated. The product yield was used for evaluating the performance improvements. Part I of this paper considered the general nonisothermal case. In this part, the results are applied to an adiabatic CSTR. A laboratory-scale adiabatic CSTR was analyzed by applying kinetic parameters for the hydrolysis of acetic anhydride. It is shown that improvement can be obtained for simultaneous modulation of the two inputs with appropriately chosen forcing parameters.",
publisher = "Wiley-V C H Verlag Gmbh, Weinheim",
journal = "Chemical Engineering & Technology",
title = "Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor",
volume = "39",
number = "11",
pages = "2126-2134",
doi = "10.1002/ceat.201600187"
}
Nikolić-Paunić, D., Felischak, M., Seidel-Morgenstern, A.,& Petkovska, M.. (2016). Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor. in Chemical Engineering & Technology
Wiley-V C H Verlag Gmbh, Weinheim., 39(11), 2126-2134.
https://doi.org/10.1002/ceat.201600187
Nikolić-Paunić D, Felischak M, Seidel-Morgenstern A, Petkovska M. Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor. in Chemical Engineering & Technology. 2016;39(11):2126-2134.
doi:10.1002/ceat.201600187 .
Nikolić-Paunić, Daliborka, Felischak, Matthias, Seidel-Morgenstern, Andreas, Petkovska, Menka, "Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor" in Chemical Engineering & Technology, 39, no. 11 (2016):2126-2134,
https://doi.org/10.1002/ceat.201600187 . .

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