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Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part II: Adiabatic Continuous Stirred-Tank Reactor

Authorized Users Only
2016
Authors
Nikolić-Paunić, Daliborka
Felischak, Matthias
Seidel-Morgenstern, Andreas
Petkovska, Menka
Article (Published version)
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Abstract
The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred-tank reactor (CSTR) when inlet concentration and/or flow rate are periodically modulated. The product yield was used for evaluating the performance improvements. Part I of this paper considered the general nonisothermal case. In this part, the results are applied to an adiabatic CSTR. A laboratory-scale adiabatic CSTR was analyzed by applying kinetic parameters for the hydrolysis of acetic anhydride. It is shown that improvement can be obtained for simultaneous modulation of the two inputs with appropriately chosen forcing parameters.
Keywords:
Adiabatic CSTR / Nonlinear frequency response / Periodic operation / Reactor modeling / Two-input modulation
Source:
Chemical Engineering & Technology, 2016, 39, 11, 2126-2134
Publisher:
  • Wiley-V C H Verlag Gmbh, Weinheim
Projects:
  • The development of efficient chemical-engineering processes based on the transport phenomena research and process intensification principles (RS-172022)
  • Nanostructured Functional and Composite Materials in Catalytic and Sorption Processes (RS-45001)

DOI: 10.1002/ceat.201600187

ISSN: 0930-7516

WoS: 000387766900017

Scopus: 2-s2.0-84992061278
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URI
http://cer.ihtm.bg.ac.rs/handle/123456789/1890
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