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Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts

Authorized Users Only
2015
Authors
Marković, Marijana
Dojčinović, Biljana
Obradović, Bratislav M.
Nesic, Jelena
Natić, Maja
Tosti, Tomislav
Kuraica, Milorad M.
Manojlović, Dragan
Article (Published version)
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Abstract
Experimental results of non-thermal plasma (NTP) utilization for degradation of 4-chlorphenol (4CP) with screening of toxicity were presented in this study. Degradation of 4CP was tested in the presence of homogeneous catalysts: hydrogen peroxide (H2O2) and iron (II) (Fe2+). The rate of degradation through eight consecutive passes of the 4CP solution in the NTP reactor was considered. Products of degradation as organic acids (acetic, formic or oxalic acid) and chloride were quantified using ion chromatography (IC). Anemia salina was used for the toxicity screening assay in order to estimate the potential and consequences of NTP reactor application in water treatment. The measured concentration of 4CP and degradation products confirmed very efficient removal of these substances from the water during the NTP treatment with the addition of a catalyst. Concerning bioassay, a significant difference in toxicity was determined between initial solution of 4CP in comparison with the solution ex...posed to catalytic NTP treatment.

Keywords:
Advanced oxidation processes (AOP) / 4-Chlorphenol / Dielectric barrier discharge (DBD) / Ecotoxicity / Non-thermal plasma (NTP)
Source:
Separation and Purification Technology, 2015, 154, 246-254
Publisher:
  • Elsevier
Funding / projects:
  • Application of advanced oxidation processes and nanostructured oxide materials for the removal of pollutants from the environment, development and optimisation of instrumental techniques for efficiency monitoring (RS-172030)
  • Simultaneous Bioremediation and Soilification of Degraded Areas to Preserve Natural Resources of Biologically Active Substances, and Development and Production of Biomaterials and Dietetic Products (RS-43004)

DOI: 10.1016/j.seppur.2015.09.030

ISSN: 1383-5866

WoS: 000364245500031

Scopus: 2-s2.0-84942890822
[ Google Scholar ]
28
23
URI
https://cer.ihtm.bg.ac.rs/handle/123456789/1821
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
IHTM
TY  - JOUR
AU  - Marković, Marijana
AU  - Dojčinović, Biljana
AU  - Obradović, Bratislav M.
AU  - Nesic, Jelena
AU  - Natić, Maja
AU  - Tosti, Tomislav
AU  - Kuraica, Milorad M.
AU  - Manojlović, Dragan
PY  - 2015
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/1821
AB  - Experimental results of non-thermal plasma (NTP) utilization for degradation of 4-chlorphenol (4CP) with screening of toxicity were presented in this study. Degradation of 4CP was tested in the presence of homogeneous catalysts: hydrogen peroxide (H2O2) and iron (II) (Fe2+). The rate of degradation through eight consecutive passes of the 4CP solution in the NTP reactor was considered. Products of degradation as organic acids (acetic, formic or oxalic acid) and chloride were quantified using ion chromatography (IC). Anemia salina was used for the toxicity screening assay in order to estimate the potential and consequences of NTP reactor application in water treatment. The measured concentration of 4CP and degradation products confirmed very efficient removal of these substances from the water during the NTP treatment with the addition of a catalyst. Concerning bioassay, a significant difference in toxicity was determined between initial solution of 4CP in comparison with the solution exposed to catalytic NTP treatment.
PB  - Elsevier
T2  - Separation and Purification Technology
T1  - Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts
VL  - 154
SP  - 246
EP  - 254
DO  - 10.1016/j.seppur.2015.09.030
ER  - 
@article{
author = "Marković, Marijana and Dojčinović, Biljana and Obradović, Bratislav M. and Nesic, Jelena and Natić, Maja and Tosti, Tomislav and Kuraica, Milorad M. and Manojlović, Dragan",
year = "2015",
abstract = "Experimental results of non-thermal plasma (NTP) utilization for degradation of 4-chlorphenol (4CP) with screening of toxicity were presented in this study. Degradation of 4CP was tested in the presence of homogeneous catalysts: hydrogen peroxide (H2O2) and iron (II) (Fe2+). The rate of degradation through eight consecutive passes of the 4CP solution in the NTP reactor was considered. Products of degradation as organic acids (acetic, formic or oxalic acid) and chloride were quantified using ion chromatography (IC). Anemia salina was used for the toxicity screening assay in order to estimate the potential and consequences of NTP reactor application in water treatment. The measured concentration of 4CP and degradation products confirmed very efficient removal of these substances from the water during the NTP treatment with the addition of a catalyst. Concerning bioassay, a significant difference in toxicity was determined between initial solution of 4CP in comparison with the solution exposed to catalytic NTP treatment.",
publisher = "Elsevier",
journal = "Separation and Purification Technology",
title = "Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts",
volume = "154",
pages = "246-254",
doi = "10.1016/j.seppur.2015.09.030"
}
Marković, M., Dojčinović, B., Obradović, B. M., Nesic, J., Natić, M., Tosti, T., Kuraica, M. M.,& Manojlović, D.. (2015). Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts. in Separation and Purification Technology
Elsevier., 154, 246-254.
https://doi.org/10.1016/j.seppur.2015.09.030
Marković M, Dojčinović B, Obradović BM, Nesic J, Natić M, Tosti T, Kuraica MM, Manojlović D. Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts. in Separation and Purification Technology. 2015;154:246-254.
doi:10.1016/j.seppur.2015.09.030 .
Marković, Marijana, Dojčinović, Biljana, Obradović, Bratislav M., Nesic, Jelena, Natić, Maja, Tosti, Tomislav, Kuraica, Milorad M., Manojlović, Dragan, "Degradation and detoxification of the 4-chlorophenol by non-thermal plasma-influence of homogeneous catalysts" in Separation and Purification Technology, 154 (2015):246-254,
https://doi.org/10.1016/j.seppur.2015.09.030 . .

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