TY  - JOUR
AU  - Seidel, Carsten
AU  - Nikolić, Daliborka
AU  - Felischak, Matthias
AU  - Petkovska, Menka
AU  - Seidel-Morgenstern, Andreas
AU  - Kienle, Achim
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5623
AB  - Methanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.
PB  - Wiley
T2  - Chemical Engineering & Technology
T1  - Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor
VL  - 45
IS  - 12
SP  - 2261
EP  - 2272
DO  - 10.1002/ceat.202200286
ER  - 

@article{
author = "Seidel, Carsten and Nikolić, Daliborka and Felischak, Matthias and Petkovska, Menka and Seidel-Morgenstern, Andreas and Kienle, Achim",
year = "2022",
abstract = "Methanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.",
publisher = "Wiley",
journal = "Chemical Engineering & Technology",
title = "Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor",
volume = "45",
number = "12",
pages = "2261-2272",
doi = "10.1002/ceat.202200286"
}

Seidel, C., Nikolić, D., Felischak, M., Petkovska, M., Seidel-Morgenstern, A.,& Kienle, A.. (2022). Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor. in Chemical Engineering & Technology
Wiley., 45(12), 2261-2272.
https://doi.org/10.1002/ceat.202200286

Seidel C, Nikolić D, Felischak M, Petkovska M, Seidel-Morgenstern A, Kienle A. Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor. in Chemical Engineering & Technology. 2022;45(12):2261-2272.
doi:10.1002/ceat.202200286 .

Seidel, Carsten, Nikolić, Daliborka, Felischak, Matthias, Petkovska, Menka, Seidel-Morgenstern, Andreas, Kienle, Achim, "Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor" in Chemical Engineering & Technology, 45, no. 12 (2022):2261-2272,
https://doi.org/10.1002/ceat.202200286 . .