TY  - JOUR
AU  - Šuljagić, Marija
AU  - Petronijević, Ivan
AU  - Mirković, Miljana
AU  - Kremenović, Aleksandar
AU  - Džunuzović, Adis
AU  - Pavlović, Vladimir B.
AU  - Kalezić-Glišović, Aleksandra
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5865
AB  - To investigate the influence of spinel structure and sintering temperature on the functional properties of BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface from acetylacetonate precursors. As-prepared powders were additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the detailed examination of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were investigated. The optimal phase composition in the BaTiO3/NiFe2O4 composite, sintered at 1150 °C, resulted in a wide frequency range stability. Additionally, particular phase composition indicates favorable properties such as low conductivity and ideal-like hysteresis loop behavior. The favorable properties of BaTiO3/NiFe2O4 make this particular composite an ideal material choice for further studies on applications of multi-ferroic devices.
PB  - MDPI
T2  - Inorganics
T1  - BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties
VL  - 11
IS  - 2
SP  - 51
DO  - 10.3390/inorganics11020051
ER  - 

@article{
author = "Šuljagić, Marija and Petronijević, Ivan and Mirković, Miljana and Kremenović, Aleksandar and Džunuzović, Adis and Pavlović, Vladimir B. and Kalezić-Glišović, Aleksandra and Anđelković, Ljubica",
year = "2023",
abstract = "To investigate the influence of spinel structure and sintering temperature on the functional properties of BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface from acetylacetonate precursors. As-prepared powders were additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the detailed examination of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were investigated. The optimal phase composition in the BaTiO3/NiFe2O4 composite, sintered at 1150 °C, resulted in a wide frequency range stability. Additionally, particular phase composition indicates favorable properties such as low conductivity and ideal-like hysteresis loop behavior. The favorable properties of BaTiO3/NiFe2O4 make this particular composite an ideal material choice for further studies on applications of multi-ferroic devices.",
publisher = "MDPI",
journal = "Inorganics",
title = "BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties",
volume = "11",
number = "2",
pages = "51",
doi = "10.3390/inorganics11020051"
}

Šuljagić, M., Petronijević, I., Mirković, M., Kremenović, A., Džunuzović, A., Pavlović, V. B., Kalezić-Glišović, A.,& Anđelković, L.. (2023). BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties. in Inorganics
MDPI., 11(2), 51.
https://doi.org/10.3390/inorganics11020051

Šuljagić M, Petronijević I, Mirković M, Kremenović A, Džunuzović A, Pavlović VB, Kalezić-Glišović A, Anđelković L. BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties. in Inorganics. 2023;11(2):51.
doi:10.3390/inorganics11020051 .

Šuljagić, Marija, Petronijević, Ivan, Mirković, Miljana, Kremenović, Aleksandar, Džunuzović, Adis, Pavlović, Vladimir B., Kalezić-Glišović, Aleksandra, Anđelković, Ljubica, "BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties" in Inorganics, 11, no. 2 (2023):51,
https://doi.org/10.3390/inorganics11020051 . .

TY  - CONF
AU  - Šuljagić, Marija
AU  - Petronijević, Ivan
AU  - Mirković, Miljana
AU  - Kremenović, Aleksandar
AU  - Džunuzović, Adis
AU  - Pavlović, Vladimir
AU  - Kalezić-Glišović, Aleksandra
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6328
AB  - In order to examine the influence of phase composition and sintering temperature on the functional properties of perovskite/spinel composites, BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The obtained powders were compressed to pellets and sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive investigation of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C, which resulted in a wide frequency range stability. Furthermore, particular phase composition led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior [1]. These functional properties of BaTiO3/NiFe2O4 make this composite a “material of choice“ for further studies on applications of multiferroic devices.
AB  - U cilju ispitivanja uticaja faznog sastava i temperature sinterovanja na funkcionalna svojstva perovskit/spinel kompozita BaTiO3/NixZn1−xFe2O4 (x = 0, 0,5, 1), NiFe2O4, ZnFe2O4, i Ni0,5Zn0,5Fe2O4 pripremljeni su in situ metodom termalne dekompozicije. U sintezi su korišćeni acetilacetonatni kompleksi kao prekursori. Dobijeni prahovi su komprimovani u tablete i sinterovani na 1150 °C i 1300 °C. Za detaljno ispitivanje faznog sastava i morfologije sintetisanih kompozita korišćene su metode rendgenske difrakcije praha (XRPD) i skenirajuće elektronske mikroskopije (SEM) spregnute sa energetsko disperzivnom spektroskopijom (EDS). Ispitivana su i magnetna, dielektrična i feroelektrična svojstva sinterovanih kompozita. Ustanovljeno je da optimalni fazni sastav pronađen kod kompozita BaTiO3/NiFe2O4 sinterovanog na 1150 °C dovodi do stabilnosti u širokom opsegu frekvencija. Optimalni fazni sastav pomenutog kompozita povoljno je uticao na funkcionalna svojstva kao što su niska provodnost i feroelektrično ponašenje koje se ogleda u zadovoljavajućem izgledu histerezisa [1]. Ova svojstva nedvosmisleno ukazuju da je kompozit BaTiO3/NiFe2O4 odgovarajući izbor za dalja istraživanja posvećena primeni multiferoičnih materijala.
PB  - Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo
C3  - 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija
T1  - BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties
T1  - Uticaj faznog sastava i temperature sinterovanja na fizička svojstva BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) kompozita sintetisanih metodom termalne dekompozicije
SP  - 36
EP  - 37
UR  - https://hdl.handle.net/21.15107/rcub_cer_6328
ER  - 

@conference{
author = "Šuljagić, Marija and Petronijević, Ivan and Mirković, Miljana and Kremenović, Aleksandar and Džunuzović, Adis and Pavlović, Vladimir and Kalezić-Glišović, Aleksandra and Anđelković, Ljubica",
year = "2023",
abstract = "In order to examine the influence of phase composition and sintering temperature on the functional properties of perovskite/spinel composites, BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The obtained powders were compressed to pellets and sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive investigation of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C, which resulted in a wide frequency range stability. Furthermore, particular phase composition led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior [1]. These functional properties of BaTiO3/NiFe2O4 make this composite a “material of choice“ for further studies on applications of multiferroic devices., U cilju ispitivanja uticaja faznog sastava i temperature sinterovanja na funkcionalna svojstva perovskit/spinel kompozita BaTiO3/NixZn1−xFe2O4 (x = 0, 0,5, 1), NiFe2O4, ZnFe2O4, i Ni0,5Zn0,5Fe2O4 pripremljeni su in situ metodom termalne dekompozicije. U sintezi su korišćeni acetilacetonatni kompleksi kao prekursori. Dobijeni prahovi su komprimovani u tablete i sinterovani na 1150 °C i 1300 °C. Za detaljno ispitivanje faznog sastava i morfologije sintetisanih kompozita korišćene su metode rendgenske difrakcije praha (XRPD) i skenirajuće elektronske mikroskopije (SEM) spregnute sa energetsko disperzivnom spektroskopijom (EDS). Ispitivana su i magnetna, dielektrična i feroelektrična svojstva sinterovanih kompozita. Ustanovljeno je da optimalni fazni sastav pronađen kod kompozita BaTiO3/NiFe2O4 sinterovanog na 1150 °C dovodi do stabilnosti u širokom opsegu frekvencija. Optimalni fazni sastav pomenutog kompozita povoljno je uticao na funkcionalna svojstva kao što su niska provodnost i feroelektrično ponašenje koje se ogleda u zadovoljavajućem izgledu histerezisa [1]. Ova svojstva nedvosmisleno ukazuju da je kompozit BaTiO3/NiFe2O4 odgovarajući izbor za dalja istraživanja posvećena primeni multiferoičnih materijala.",
publisher = "Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo",
journal = "28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija",
title = "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties, Uticaj faznog sastava i temperature sinterovanja na fizička svojstva BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) kompozita sintetisanih metodom termalne dekompozicije",
pages = "36-37",
url = "https://hdl.handle.net/21.15107/rcub_cer_6328"
}

Šuljagić, M., Petronijević, I., Mirković, M., Kremenović, A., Džunuzović, A., Pavlović, V., Kalezić-Glišović, A.,& Anđelković, L.. (2023). BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties. in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija
Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo., 36-37.
https://hdl.handle.net/21.15107/rcub_cer_6328

Šuljagić M, Petronijević I, Mirković M, Kremenović A, Džunuzović A, Pavlović V, Kalezić-Glišović A, Anđelković L. BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties. in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija. 2023;:36-37.
https://hdl.handle.net/21.15107/rcub_cer_6328 .

Šuljagić, Marija, Petronijević, Ivan, Mirković, Miljana, Kremenović, Aleksandar, Džunuzović, Adis, Pavlović, Vladimir, Kalezić-Glišović, Aleksandra, Anđelković, Ljubica, "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties" in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija (2023):36-37,
https://hdl.handle.net/21.15107/rcub_cer_6328 .

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Kremenović, Aleksandar
AU  - Petronijević, Ivan
AU  - Džunuzović, Adis
AU  - Mirković, Miljana
AU  - Pavlović, Vladimir
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6643
AB  - To investigate the effect of synthesis procedure and sintering temperature on the functional properties of perovskite/spinel ceramics, BaTiO3/CoFe2O4 composites were prepared by thermal decomposition, coprecipitation, and microemulsion method, and sintered at 1150°C and 1300°C. The phase composition and morphology of as-prepared powders as well as sintered ceramics were thoroughly examined by X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS). The dielectric and ferroelectric measurements were performed in detail. Generally, the samples sintered at 1300°C had better performances than those sintered at 1150°C. The composite synthesized by thermal decomposition and sintered at 1300 °C stands out among other prepared BaTiO3/CoFe2O4 ceramics, owing to high stability in the wide frequency range and low leakage currents. The obtained results indicate that such composite might be successfully applied as a functional multiferroic.
AB  - У циљу испитивања утицаја методе синтезе као и температуре синтеровања на функционална својства керамике перовскитно/спинелне структуре, синтетисани су BaTiO3/CoFe2O4 композити методама термалне декомпозиције, копреципитације и микроемулзије, а затим синтеровани на 1150 °C и 1300 °C. Фазни састав и морфологија синтетисаних узорака детаљно су испитани пре и после синтеровања помоћу рендгенске дифракције на праху (XRPD) и скенирајуће електронске микроскпије (SEM) спрегнуте са елекрон дисперзивном спектроскопијом (EDS). Изведена су опсежна испитивања како диелектричних, тако и фероелектричних својстава датих композита. У већини случајева узорци синтеровани на 1300 °C показали су боља својства од узорака синтерованих на 1150 °C. Композит синтетисан методом термалне декомпозиције и синтерован на 1300 °C издваја се од осталих синтетисаних BaTiO3/CoFe2O4 узорака захваљујући великој стабилносту у широком фреквентном опсегу и малим струјама цурења. Добијени резултати недвосмислено указују да истакнути композит може бити успешно примењен као функционални мултифероик.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites
VL  - 55
SP  - 367
EP  - 381
DO  - 10.2298/SOS220512013S
ER  - 

@article{
author = "Šuljagić, Marija and Kremenović, Aleksandar and Petronijević, Ivan and Džunuzović, Adis and Mirković, Miljana and Pavlović, Vladimir and Anđelković, Ljubica",
year = "2023",
abstract = "To investigate the effect of synthesis procedure and sintering temperature on the functional properties of perovskite/spinel ceramics, BaTiO3/CoFe2O4 composites were prepared by thermal decomposition, coprecipitation, and microemulsion method, and sintered at 1150°C and 1300°C. The phase composition and morphology of as-prepared powders as well as sintered ceramics were thoroughly examined by X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS). The dielectric and ferroelectric measurements were performed in detail. Generally, the samples sintered at 1300°C had better performances than those sintered at 1150°C. The composite synthesized by thermal decomposition and sintered at 1300 °C stands out among other prepared BaTiO3/CoFe2O4 ceramics, owing to high stability in the wide frequency range and low leakage currents. The obtained results indicate that such composite might be successfully applied as a functional multiferroic., У циљу испитивања утицаја методе синтезе као и температуре синтеровања на функционална својства керамике перовскитно/спинелне структуре, синтетисани су BaTiO3/CoFe2O4 композити методама термалне декомпозиције, копреципитације и микроемулзије, а затим синтеровани на 1150 °C и 1300 °C. Фазни састав и морфологија синтетисаних узорака детаљно су испитани пре и после синтеровања помоћу рендгенске дифракције на праху (XRPD) и скенирајуће електронске микроскпије (SEM) спрегнуте са елекрон дисперзивном спектроскопијом (EDS). Изведена су опсежна испитивања како диелектричних, тако и фероелектричних својстава датих композита. У већини случајева узорци синтеровани на 1300 °C показали су боља својства од узорака синтерованих на 1150 °C. Композит синтетисан методом термалне декомпозиције и синтерован на 1300 °C издваја се од осталих синтетисаних BaTiO3/CoFe2O4 узорака захваљујући великој стабилносту у широком фреквентном опсегу и малим струјама цурења. Добијени резултати недвосмислено указују да истакнути композит може бити успешно примењен као функционални мултифероик.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites",
volume = "55",
pages = "367-381",
doi = "10.2298/SOS220512013S"
}

Šuljagić, M., Kremenović, A., Petronijević, I., Džunuzović, A., Mirković, M., Pavlović, V.,& Anđelković, L.. (2023). Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites. in Science of Sintering
Association for ETRAN Society., 55, 367-381.
https://doi.org/10.2298/SOS220512013S

Šuljagić M, Kremenović A, Petronijević I, Džunuzović A, Mirković M, Pavlović V, Anđelković L. Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites. in Science of Sintering. 2023;55:367-381.
doi:10.2298/SOS220512013S .

Šuljagić, Marija, Kremenović, Aleksandar, Petronijević, Ivan, Džunuzović, Adis, Mirković, Miljana, Pavlović, Vladimir, Anđelković, Ljubica, "Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites" in Science of Sintering, 55 (2023):367-381,
https://doi.org/10.2298/SOS220512013S . .