Radulović, Katarina

Link to this page

Authority KeyName Variants
orcid::0000-0001-5898-6130
  • Radulović, Katarina (106)
Projects
Micro- Nanosystems and Sensors for Electric Power and Process Industry and Environmental Protection Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200026 (University of Belgrade, Institute of Chemistry, Technology and Metallurgy - IChTM)
Serbian Academy of Sciences and Arts, Project F-150 Reinforcement of Regional Microsystems and Nanosystems Centre
Atomic collision processes and photoacoustic spectroscopy of molecules and solids Rational design and synthesis of biologically active and coordination compounds and functional materials, relevant for (bio)nanotechnology
CNPq (National Council for Scientific and Technological Development), Research Productivity Grants Ministry of Sciences, Technologies and Development, Republic of Serbia Grant No. I.T.1.04.0062.B
Serbian Academy of Sciences and Arts (Project F-150) Digitalization and Technology Research Center of the Bundeswehr (project VITAL-SENSE)
Fundação para a Ciência e a Tecnologia IST-ID/156-2018 New permanent magnets for electric-vehicle drive applications
Electronic, transport and optical properties of nanostructured materials Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200007 (University of Belgrade, Institute for Biological Research 'Siniša Stanković')
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200168 (University of Belgrade, Faculty of Chemistry) An integral study to identify the regional genetic and environmental risk factors for the common noncommunicable diseases in the human population of Serbia - INGEMA_S
Advanced technologies for monitoring and environmental protection from chemical pollutants and radiation burden Fabrication and characterization of nano-photonic functional structrues in biomedicine and informatics
Measurements in a smart grid concept Predefined functional properties polymer composite materials processes and equipment development
Gramulsen - Graphene-Based Wearable Multiparameter Sensor Ministry for Science and Environmental Protection of the Republic of Serbia (project B 6150)
North Atlantic Treaty Organization: Science for Peace and Security Program: SP4LIFE Research Fund of the Serbian Academy of Sciences and Arts : F-190
Serbian Academy of Sciences and Arts (Project F/150) Serbian Academy of Sciences and Arts (Project F150)
Serbian Academy of Sciences and Arts, Project F-150 SP4LIFE
TR6151 - Micro and Nanosystem Technologies, Structures and Sensors

Author's Bibliography

Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates

Stanković, Jelena; Milošević, Đurađ; Paunović, Momir; Jovanović, Boris; Popović, Nataša; Tomović, Jelena; Atanacković, Ana; Radulović, Katarina; Lončarević, Davor; Raković, Maja

(MDPI, 2024)

TY  - JOUR
AU  - Stanković, Jelena
AU  - Milošević, Đurađ
AU  - Paunović, Momir
AU  - Jovanović, Boris
AU  - Popović, Nataša
AU  - Tomović, Jelena
AU  - Atanacković, Ana
AU  - Radulović, Katarina
AU  - Lončarević, Davor
AU  - Raković, Maja
PY  - 2024
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7554
AB  - This study was carried out at the Danube River and its tributaries during the Joint Danube
Survey 4 (JDS4) expedition. Three freshwater benthic species were used to estimate the quantity
of microplastics (MPs): Corbicula spp., Limnodrilus hoffmeisteri (Claparede, 1862), and Polypedilum nubeculosum (Meigen, 1804). Following the kick and sweep technique, individuals were sampled using a hand net or dredge. In order to estimate the number of MP articles/individual particles/g wet body mass, the body mass and total length of all specimens were measured. Alkaline (Corbicula spp.and L. hoffmaisteri) and enzymatic (P. nubeculosum) protocols were performed for tissue degradation. All samples were filtered through glass microfiber filters (mesh size 0.5 μm). The particles were photographed, measured, and counted. A total of 1904, 169, and 204 MPs were isolated from Corbicula spp., L. hoffmaisteri, and P. nubeculosum, respectively. To confirm the chemical composition of isolated MPs, a subsample of 46 particles of the fragmented particles from 14 sampling sites was analysed via μ-ATR-FTIR spectroscopy analysis. The particles were characterised as polycarbonate (PC), polyethylene terephthalate (PET), polypropylene–polyethylene copolymer (PP-PE), nylon (polyamide-PA) and cellophane, with the domination of PET.
PB  - MDPI
T2  - Water
T1  - Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates
VL  - 16
IS  - 7
SP  - 962
DO  - 10.3390/w16070962
ER  - 
@article{
author = "Stanković, Jelena and Milošević, Đurađ and Paunović, Momir and Jovanović, Boris and Popović, Nataša and Tomović, Jelena and Atanacković, Ana and Radulović, Katarina and Lončarević, Davor and Raković, Maja",
year = "2024",
abstract = "This study was carried out at the Danube River and its tributaries during the Joint Danube
Survey 4 (JDS4) expedition. Three freshwater benthic species were used to estimate the quantity
of microplastics (MPs): Corbicula spp., Limnodrilus hoffmeisteri (Claparede, 1862), and Polypedilum nubeculosum (Meigen, 1804). Following the kick and sweep technique, individuals were sampled using a hand net or dredge. In order to estimate the number of MP articles/individual particles/g wet body mass, the body mass and total length of all specimens were measured. Alkaline (Corbicula spp.and L. hoffmaisteri) and enzymatic (P. nubeculosum) protocols were performed for tissue degradation. All samples were filtered through glass microfiber filters (mesh size 0.5 μm). The particles were photographed, measured, and counted. A total of 1904, 169, and 204 MPs were isolated from Corbicula spp., L. hoffmaisteri, and P. nubeculosum, respectively. To confirm the chemical composition of isolated MPs, a subsample of 46 particles of the fragmented particles from 14 sampling sites was analysed via μ-ATR-FTIR spectroscopy analysis. The particles were characterised as polycarbonate (PC), polyethylene terephthalate (PET), polypropylene–polyethylene copolymer (PP-PE), nylon (polyamide-PA) and cellophane, with the domination of PET.",
publisher = "MDPI",
journal = "Water",
title = "Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates",
volume = "16",
number = "7",
pages = "962",
doi = "10.3390/w16070962"
}
Stanković, J., Milošević, Đ., Paunović, M., Jovanović, B., Popović, N., Tomović, J., Atanacković, A., Radulović, K., Lončarević, D.,& Raković, M.. (2024). Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates. in Water
MDPI., 16(7), 962.
https://doi.org/10.3390/w16070962
Stanković J, Milošević Đ, Paunović M, Jovanović B, Popović N, Tomović J, Atanacković A, Radulović K, Lončarević D, Raković M. Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates. in Water. 2024;16(7):962.
doi:10.3390/w16070962 .
Stanković, Jelena, Milošević, Đurađ, Paunović, Momir, Jovanović, Boris, Popović, Nataša, Tomović, Jelena, Atanacković, Ana, Radulović, Katarina, Lončarević, Davor, Raković, Maja, "Microplastics in the Danube River and Its Main Tributaries - Ingestion by Freshwater Macroinvertebrates" in Water, 16, no. 7 (2024):962,
https://doi.org/10.3390/w16070962 . .
3

Laser-induced graphene on PEO/PDMS composites

Pergal, Marija; Rašljić Rafajilović, Milena; Vićentić, Teodora; Pašti, Igor; Bajuk-Bogdanović, Danica; Radulović, Katarina; Spasenović, Marko

(Belgrade : Serbian Ceramic Society, 2023)

TY  - CONF
AU  - Pergal, Marija
AU  - Rašljić Rafajilović, Milena
AU  - Vićentić, Teodora
AU  - Pašti, Igor
AU  - Bajuk-Bogdanović, Danica
AU  - Radulović, Katarina
AU  - Spasenović, Marko
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7114
AB  - Laser-induced graphene (LIG) has emerged as one of the most promising materials for
flexible functional devices. One-step fabrication of LIG offers advantages such as low cost,
patterning of desired geometries, and high sensitivity. However, previous attempts to obtain
LIG on elastomeric substrates have been unsuccessful, limiting its potential for use in
stretchable electronics. In this study, we propose using a substrate composed of
polydimethylsiloxane (PDMS) and poly(ethylene oxide) (PEO) with a low molecular weight
as a platform for manufacturing LIG. A series of PDMS/PEO materials with varying
concentrations of PEO (1, 5, 10, 20, 30, 40 and 50 wt.%) were prepared using a cast-based
approach, starting from divinyl-terminated-PDMS and poly(methyl-hydrogensiloxane). The
prepared PDMS/PEO/graphene composites were characterized using Raman spectroscopy,
Fourier transform infrared spectroscopy (FTIR), and scanning electron microscopy (SEM)
analysis. FTIR analysis confirmed the structure of the prepared PDMS/PEO and
PDMS/PEO/graphene materials. The results demonstrated that the prepared PDMS/PEO
composites exhibited a higher degree of graphenization compared to pure PDMS networks.
SEM analysis revealed the formation of a porous graphene structure. Based on these findings,
the PDMS/PEO/graphene composites show promise for further investigation as electronic
device applications.
PB  - Belgrade : Serbian Ceramic Society
C3  - Program and book of abstracts - Serbian Ceramics Society Conference - Advanced Ceramics and Application XI, New Frontiers in Multifunctional Material Science and Processing,18-20 th September 2023. Belgrade, Serbia
T1  - Laser-induced graphene on PEO/PDMS composites
SP  - 59
EP  - 59
UR  - https://hdl.handle.net/21.15107/rcub_cer_7114
ER  - 
@conference{
author = "Pergal, Marija and Rašljić Rafajilović, Milena and Vićentić, Teodora and Pašti, Igor and Bajuk-Bogdanović, Danica and Radulović, Katarina and Spasenović, Marko",
year = "2023",
abstract = "Laser-induced graphene (LIG) has emerged as one of the most promising materials for
flexible functional devices. One-step fabrication of LIG offers advantages such as low cost,
patterning of desired geometries, and high sensitivity. However, previous attempts to obtain
LIG on elastomeric substrates have been unsuccessful, limiting its potential for use in
stretchable electronics. In this study, we propose using a substrate composed of
polydimethylsiloxane (PDMS) and poly(ethylene oxide) (PEO) with a low molecular weight
as a platform for manufacturing LIG. A series of PDMS/PEO materials with varying
concentrations of PEO (1, 5, 10, 20, 30, 40 and 50 wt.%) were prepared using a cast-based
approach, starting from divinyl-terminated-PDMS and poly(methyl-hydrogensiloxane). The
prepared PDMS/PEO/graphene composites were characterized using Raman spectroscopy,
Fourier transform infrared spectroscopy (FTIR), and scanning electron microscopy (SEM)
analysis. FTIR analysis confirmed the structure of the prepared PDMS/PEO and
PDMS/PEO/graphene materials. The results demonstrated that the prepared PDMS/PEO
composites exhibited a higher degree of graphenization compared to pure PDMS networks.
SEM analysis revealed the formation of a porous graphene structure. Based on these findings,
the PDMS/PEO/graphene composites show promise for further investigation as electronic
device applications.",
publisher = "Belgrade : Serbian Ceramic Society",
journal = "Program and book of abstracts - Serbian Ceramics Society Conference - Advanced Ceramics and Application XI, New Frontiers in Multifunctional Material Science and Processing,18-20 th September 2023. Belgrade, Serbia",
title = "Laser-induced graphene on PEO/PDMS composites",
pages = "59-59",
url = "https://hdl.handle.net/21.15107/rcub_cer_7114"
}
Pergal, M., Rašljić Rafajilović, M., Vićentić, T., Pašti, I., Bajuk-Bogdanović, D., Radulović, K.,& Spasenović, M.. (2023). Laser-induced graphene on PEO/PDMS composites. in Program and book of abstracts - Serbian Ceramics Society Conference - Advanced Ceramics and Application XI, New Frontiers in Multifunctional Material Science and Processing,18-20 th September 2023. Belgrade, Serbia
Belgrade : Serbian Ceramic Society., 59-59.
https://hdl.handle.net/21.15107/rcub_cer_7114
Pergal M, Rašljić Rafajilović M, Vićentić T, Pašti I, Bajuk-Bogdanović D, Radulović K, Spasenović M. Laser-induced graphene on PEO/PDMS composites. in Program and book of abstracts - Serbian Ceramics Society Conference - Advanced Ceramics and Application XI, New Frontiers in Multifunctional Material Science and Processing,18-20 th September 2023. Belgrade, Serbia. 2023;:59-59.
https://hdl.handle.net/21.15107/rcub_cer_7114 .
Pergal, Marija, Rašljić Rafajilović, Milena, Vićentić, Teodora, Pašti, Igor, Bajuk-Bogdanović, Danica, Radulović, Katarina, Spasenović, Marko, "Laser-induced graphene on PEO/PDMS composites" in Program and book of abstracts - Serbian Ceramics Society Conference - Advanced Ceramics and Application XI, New Frontiers in Multifunctional Material Science and Processing,18-20 th September 2023. Belgrade, Serbia (2023):59-59,
https://hdl.handle.net/21.15107/rcub_cer_7114 .

Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials

Rašljić Rafajilović, Milena; Vićentić, Teodora; Spasenović, Marko; Bajuk-Bogdanović, Danica; Pašti, Igor; Radulović, Katarina; Pergal, Marija

(Академија наука и умјетности Републике Српске / Academy of Sciences and Arts of the Republic of Srpska, 2023)

TY  - CONF
AU  - Rašljić Rafajilović, Milena
AU  - Vićentić, Teodora
AU  - Spasenović, Marko
AU  - Bajuk-Bogdanović, Danica
AU  - Pašti, Igor
AU  - Radulović, Katarina
AU  - Pergal, Marija
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7115
AB  - The objective of this study was to develop optimal laser parameters (resolution, power, and velocity) for the formation of graphene on poly(dimethylsiloxane) (PDMS)-based materials using laser-induced graphene (LIG). A series of novel PDMS/poly(ethylene glycol) (PEG) materials with varying concentrations of PEG (30, 40, and 50 wt.%) was prepared through a blending approach. For comparison, pure PDMS was prepared using a casting method. To the best of our knowledge, the synthesis of PDMS/PEG materials and the direct laser graphenization (LIG) of PDMS/PEG materials have not been reported in the literature. Once the optimal laser parameters were established, the prepared PDMS/PEG/graphene composites were characterized using Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, and scanning electron microscopy (SEM). The results demonstrated that the addition of PEG led to an enhanced degree of graphenization compared to the pure PDMS sample, which did not induce graphene formation. Among the materials tested, the PDMS/PEG/graphene composite with 30 wt.% PEG in the PDMS matrix exhibited the optimal degree of graphenization. SEM analysis of the LIG on PDMS/PEG material revealed a porous network structure. With their improved properties, the developed PDMS/PEG/graphene composites hold promise as materials suitable for the production of flexible electronic devices.
PB  - Академија наука и умјетности Републике Српске / Academy of Sciences and Arts of the Republic of Srpska
C3  - XVI Mеђународни научни скуп Савремени материјали 2023, Програм рада и Књига апстраката, 7 - 8. септембар 2023. године, Бања Лука /XVI International Scientific Conference Contemporary Materials 2023, Programme and the Book Of Abstracts, September 7 - 8, 2023, Banja Luka
T1  - Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials
SP  - 40
EP  - 40
UR  - https://hdl.handle.net/21.15107/rcub_cer_7115
ER  - 
@conference{
author = "Rašljić Rafajilović, Milena and Vićentić, Teodora and Spasenović, Marko and Bajuk-Bogdanović, Danica and Pašti, Igor and Radulović, Katarina and Pergal, Marija",
year = "2023",
abstract = "The objective of this study was to develop optimal laser parameters (resolution, power, and velocity) for the formation of graphene on poly(dimethylsiloxane) (PDMS)-based materials using laser-induced graphene (LIG). A series of novel PDMS/poly(ethylene glycol) (PEG) materials with varying concentrations of PEG (30, 40, and 50 wt.%) was prepared through a blending approach. For comparison, pure PDMS was prepared using a casting method. To the best of our knowledge, the synthesis of PDMS/PEG materials and the direct laser graphenization (LIG) of PDMS/PEG materials have not been reported in the literature. Once the optimal laser parameters were established, the prepared PDMS/PEG/graphene composites were characterized using Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, and scanning electron microscopy (SEM). The results demonstrated that the addition of PEG led to an enhanced degree of graphenization compared to the pure PDMS sample, which did not induce graphene formation. Among the materials tested, the PDMS/PEG/graphene composite with 30 wt.% PEG in the PDMS matrix exhibited the optimal degree of graphenization. SEM analysis of the LIG on PDMS/PEG material revealed a porous network structure. With their improved properties, the developed PDMS/PEG/graphene composites hold promise as materials suitable for the production of flexible electronic devices.",
publisher = "Академија наука и умјетности Републике Српске / Academy of Sciences and Arts of the Republic of Srpska",
journal = "XVI Mеђународни научни скуп Савремени материјали 2023, Програм рада и Књига апстраката, 7 - 8. септембар 2023. године, Бања Лука /XVI International Scientific Conference Contemporary Materials 2023, Programme and the Book Of Abstracts, September 7 - 8, 2023, Banja Luka",
title = "Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials",
pages = "40-40",
url = "https://hdl.handle.net/21.15107/rcub_cer_7115"
}
Rašljić Rafajilović, M., Vićentić, T., Spasenović, M., Bajuk-Bogdanović, D., Pašti, I., Radulović, K.,& Pergal, M.. (2023). Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials. in XVI Mеђународни научни скуп Савремени материјали 2023, Програм рада и Књига апстраката, 7 - 8. септембар 2023. године, Бања Лука /XVI International Scientific Conference Contemporary Materials 2023, Programme and the Book Of Abstracts, September 7 - 8, 2023, Banja Luka
Академија наука и умјетности Републике Српске / Academy of Sciences and Arts of the Republic of Srpska., 40-40.
https://hdl.handle.net/21.15107/rcub_cer_7115
Rašljić Rafajilović M, Vićentić T, Spasenović M, Bajuk-Bogdanović D, Pašti I, Radulović K, Pergal M. Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials. in XVI Mеђународни научни скуп Савремени материјали 2023, Програм рада и Књига апстраката, 7 - 8. септембар 2023. године, Бања Лука /XVI International Scientific Conference Contemporary Materials 2023, Programme and the Book Of Abstracts, September 7 - 8, 2023, Banja Luka. 2023;:40-40.
https://hdl.handle.net/21.15107/rcub_cer_7115 .
Rašljić Rafajilović, Milena, Vićentić, Teodora, Spasenović, Marko, Bajuk-Bogdanović, Danica, Pašti, Igor, Radulović, Katarina, Pergal, Marija, "Optimal laser parameters for laser induction of graphene on poly(dimethylsiloxane)-based materials" in XVI Mеђународни научни скуп Савремени материјали 2023, Програм рада и Књига апстраката, 7 - 8. септембар 2023. године, Бања Лука /XVI International Scientific Conference Contemporary Materials 2023, Programme and the Book Of Abstracts, September 7 - 8, 2023, Banja Luka (2023):40-40,
https://hdl.handle.net/21.15107/rcub_cer_7115 .

Laser-induced graphene on cross-linked sodium alginate

Vićentić, Teodora; Greco, Immacolata; Iorio, Carlo Saverio; Mišković, Vanja; Bajuk-Bogdanović, Danica; Pašti, Igor; Radulović, Katarina; Klenk, S.; Stimpel-Lindner, Tanja; Duesberg, G. S.; Spasenović, Marko

(IOP Publishing, 2023)

TY  - JOUR
AU  - Vićentić, Teodora
AU  - Greco, Immacolata
AU  - Iorio, Carlo Saverio
AU  - Mišković, Vanja
AU  - Bajuk-Bogdanović, Danica
AU  - Pašti, Igor
AU  - Radulović, Katarina
AU  - Klenk, S.
AU  - Stimpel-Lindner, Tanja
AU  - Duesberg, G. S.
AU  - Spasenović, Marko
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7416
AB  - Laser-induced graphene (LIG) possesses desirable properties for numerous applications. However, LIG formation on biocompatible substrates is needed to further augment the integration of LIG-based technologies into nanobiotechnology. Here, LIG formation on cross-linked sodium alginate is reported. The LIG is systematically investigated, providing a comprehensive understanding of the physicochemical characteristics of the material. Raman spectroscopy, scanning electron microscopy with energy-dispersive x-ray analysis, x-ray diffraction, transmission electron microscopy, Fourier-transform infrared spectroscopy and x-ray photoelectron spectroscopy techniques confirm the successful generation of oxidized graphene on the surface of cross-linked sodium alginate. The influence of laser parameters and the amount of crosslinker incorporated into the alginate substrate is explored, revealing that lower laser speed, higher resolution, and increased CaCl2 content leads to LIG with lower electrical resistance. These findings could have significant implications for the fabrication of LIG on alginate with tailored conductive properties, but they could also play a guiding role for LIG formation on other biocompatible substrates.
PB  - IOP Publishing
T2  - Nanotechnology
T1  - Laser-induced graphene on cross-linked sodium alginate
VL  - 35
IS  - 11
SP  - 115103
DO  - 10.1088/1361-6528/ad143a
ER  - 
@article{
author = "Vićentić, Teodora and Greco, Immacolata and Iorio, Carlo Saverio and Mišković, Vanja and Bajuk-Bogdanović, Danica and Pašti, Igor and Radulović, Katarina and Klenk, S. and Stimpel-Lindner, Tanja and Duesberg, G. S. and Spasenović, Marko",
year = "2023",
abstract = "Laser-induced graphene (LIG) possesses desirable properties for numerous applications. However, LIG formation on biocompatible substrates is needed to further augment the integration of LIG-based technologies into nanobiotechnology. Here, LIG formation on cross-linked sodium alginate is reported. The LIG is systematically investigated, providing a comprehensive understanding of the physicochemical characteristics of the material. Raman spectroscopy, scanning electron microscopy with energy-dispersive x-ray analysis, x-ray diffraction, transmission electron microscopy, Fourier-transform infrared spectroscopy and x-ray photoelectron spectroscopy techniques confirm the successful generation of oxidized graphene on the surface of cross-linked sodium alginate. The influence of laser parameters and the amount of crosslinker incorporated into the alginate substrate is explored, revealing that lower laser speed, higher resolution, and increased CaCl2 content leads to LIG with lower electrical resistance. These findings could have significant implications for the fabrication of LIG on alginate with tailored conductive properties, but they could also play a guiding role for LIG formation on other biocompatible substrates.",
publisher = "IOP Publishing",
journal = "Nanotechnology",
title = "Laser-induced graphene on cross-linked sodium alginate",
volume = "35",
number = "11",
pages = "115103",
doi = "10.1088/1361-6528/ad143a"
}
Vićentić, T., Greco, I., Iorio, C. S., Mišković, V., Bajuk-Bogdanović, D., Pašti, I., Radulović, K., Klenk, S., Stimpel-Lindner, T., Duesberg, G. S.,& Spasenović, M.. (2023). Laser-induced graphene on cross-linked sodium alginate. in Nanotechnology
IOP Publishing., 35(11), 115103.
https://doi.org/10.1088/1361-6528/ad143a
Vićentić T, Greco I, Iorio CS, Mišković V, Bajuk-Bogdanović D, Pašti I, Radulović K, Klenk S, Stimpel-Lindner T, Duesberg GS, Spasenović M. Laser-induced graphene on cross-linked sodium alginate. in Nanotechnology. 2023;35(11):115103.
doi:10.1088/1361-6528/ad143a .
Vićentić, Teodora, Greco, Immacolata, Iorio, Carlo Saverio, Mišković, Vanja, Bajuk-Bogdanović, Danica, Pašti, Igor, Radulović, Katarina, Klenk, S., Stimpel-Lindner, Tanja, Duesberg, G. S., Spasenović, Marko, "Laser-induced graphene on cross-linked sodium alginate" in Nanotechnology, 35, no. 11 (2023):115103,
https://doi.org/10.1088/1361-6528/ad143a . .
1

Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis

Ajduković, Marija; Stevanović, Gordana; Marinović, Sanja; Mojović, Zorica; Banković, Predrag; Radulović, Katarina; Jović-Jovičić, Nataša

(MDPI, 2023)

TY  - JOUR
AU  - Ajduković, Marija
AU  - Stevanović, Gordana
AU  - Marinović, Sanja
AU  - Mojović, Zorica
AU  - Banković, Predrag
AU  - Radulović, Katarina
AU  - Jović-Jovičić, Nataša
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6712
AB  - The employment of compounds obtained from natural sources to produce adsorbents and their application in the elimination of antibiotics from industrial effluents have gained significant attention because of their low production cost and sustainability. Herein, chitosan (biopolymer) and smectite (abundant clay mineral) were used for the low-cost and eco-friendly synthesis of a new type of adsorbent. A low-energy-consumption hydrothermal process was applied to the synthesis of the chitosan-derived carbon–smectite nanocomposite with cobalt (H_Co/C-S). The produced nanocomposite was characterized using elemental analysis, ICP-OES, XRPD, low-temperature N2 adsorption–desorption isotherms, FTIR analysis, and point of zero charge. H_Co/C-S (SBET = 0.73 m2 g−1, d001 = 1.40 nm, pHPZC = 5.3) was evaluated as a ciprofloxacin adsorbent in aqueous solution. Experimental data were fitted with different kinetic models and interpreted by selected adsorption isotherms. The pseudo-second-order model was found to be the most appropriate, while ciprofloxacin adsorption onto H_Co/C-S was best described by the Redlich–Peterson isotherm (R2 = 0.985). The maximum adsorption capacity of H_Co/C-S, according to the Langmuir isotherm (R2 = 0.977), was 72.3 mg g−1. Desorption and thermodynamic studies were performed. The obtained results indicated that the new hierarchically designed H_Co/C-S has promising potential to be further tested for application in real wastewater treatment.
PB  - MDPI
T2  - Water
T1  - Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis
VL  - 15
IS  - 14
SP  - 2608
DO  - 10.3390/w15142608
ER  - 
@article{
author = "Ajduković, Marija and Stevanović, Gordana and Marinović, Sanja and Mojović, Zorica and Banković, Predrag and Radulović, Katarina and Jović-Jovičić, Nataša",
year = "2023",
abstract = "The employment of compounds obtained from natural sources to produce adsorbents and their application in the elimination of antibiotics from industrial effluents have gained significant attention because of their low production cost and sustainability. Herein, chitosan (biopolymer) and smectite (abundant clay mineral) were used for the low-cost and eco-friendly synthesis of a new type of adsorbent. A low-energy-consumption hydrothermal process was applied to the synthesis of the chitosan-derived carbon–smectite nanocomposite with cobalt (H_Co/C-S). The produced nanocomposite was characterized using elemental analysis, ICP-OES, XRPD, low-temperature N2 adsorption–desorption isotherms, FTIR analysis, and point of zero charge. H_Co/C-S (SBET = 0.73 m2 g−1, d001 = 1.40 nm, pHPZC = 5.3) was evaluated as a ciprofloxacin adsorbent in aqueous solution. Experimental data were fitted with different kinetic models and interpreted by selected adsorption isotherms. The pseudo-second-order model was found to be the most appropriate, while ciprofloxacin adsorption onto H_Co/C-S was best described by the Redlich–Peterson isotherm (R2 = 0.985). The maximum adsorption capacity of H_Co/C-S, according to the Langmuir isotherm (R2 = 0.977), was 72.3 mg g−1. Desorption and thermodynamic studies were performed. The obtained results indicated that the new hierarchically designed H_Co/C-S has promising potential to be further tested for application in real wastewater treatment.",
publisher = "MDPI",
journal = "Water",
title = "Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis",
volume = "15",
number = "14",
pages = "2608",
doi = "10.3390/w15142608"
}
Ajduković, M., Stevanović, G., Marinović, S., Mojović, Z., Banković, P., Radulović, K.,& Jović-Jovičić, N.. (2023). Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis. in Water
MDPI., 15(14), 2608.
https://doi.org/10.3390/w15142608
Ajduković M, Stevanović G, Marinović S, Mojović Z, Banković P, Radulović K, Jović-Jovičić N. Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis. in Water. 2023;15(14):2608.
doi:10.3390/w15142608 .
Ajduković, Marija, Stevanović, Gordana, Marinović, Sanja, Mojović, Zorica, Banković, Predrag, Radulović, Katarina, Jović-Jovičić, Nataša, "Ciprofloxacin Adsorption onto a Smectite–Chitosan-Derived Nanocomposite Obtained by Hydrothermal Synthesis" in Water, 15, no. 14 (2023):2608,
https://doi.org/10.3390/w15142608 . .
4
1

Characterization of heterogeneous sensing layers in graphene-based gas sensors

Andrić, Stevan; Jokić, Ivana; Frantlović, Miloš; Radulović, Katarina; Spasenović, Marko

(Belgrade : The Military Technical Institute, 2022)

TY  - CONF
AU  - Andrić, Stevan
AU  - Jokić, Ivana
AU  - Frantlović, Miloš
AU  - Radulović, Katarina
AU  - Spasenović, Marko
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5825
AB  - Graphene-based sensors have a great potential for applications in public and personal health protection, including defense and security fields. However, sensitivity and selectivity of such sensors are inherently dependent on adsorption properties of the graphene sensing layer, which is typically of heterogeneous morphology and/or of heterogeneous chemical composition due to intentionally introduced functionalizing elements or spontaneously adsorbed molecules during sensor fabrication or operation. Therefore, characterization and optimization of sensing layers is extremely important for achieving high sensing performance. In this work, we present a method for characterization of the heterogeneous sensing layer by using the frequency domain analysis of the sensor output signal. The method is based on the mathematical model we devised. Here, the model is presented in detail for the case of a surface with three types of adsorption sites, and then the method is applied for extraction of parameters that characterize adsorption properties of a graphene sensing layer.
PB  - Belgrade : The Military Technical Institute
C3  - Proceedings - 10th International Scientific Conference on Defensive Technologies, OTEH 2022, 13-14 October 2022, Belgrade, Serbia
T1  - Characterization of heterogeneous sensing layers in graphene-based gas sensors
UR  - https://hdl.handle.net/21.15107/rcub_cer_5825
ER  - 
@conference{
author = "Andrić, Stevan and Jokić, Ivana and Frantlović, Miloš and Radulović, Katarina and Spasenović, Marko",
year = "2022",
abstract = "Graphene-based sensors have a great potential for applications in public and personal health protection, including defense and security fields. However, sensitivity and selectivity of such sensors are inherently dependent on adsorption properties of the graphene sensing layer, which is typically of heterogeneous morphology and/or of heterogeneous chemical composition due to intentionally introduced functionalizing elements or spontaneously adsorbed molecules during sensor fabrication or operation. Therefore, characterization and optimization of sensing layers is extremely important for achieving high sensing performance. In this work, we present a method for characterization of the heterogeneous sensing layer by using the frequency domain analysis of the sensor output signal. The method is based on the mathematical model we devised. Here, the model is presented in detail for the case of a surface with three types of adsorption sites, and then the method is applied for extraction of parameters that characterize adsorption properties of a graphene sensing layer.",
publisher = "Belgrade : The Military Technical Institute",
journal = "Proceedings - 10th International Scientific Conference on Defensive Technologies, OTEH 2022, 13-14 October 2022, Belgrade, Serbia",
title = "Characterization of heterogeneous sensing layers in graphene-based gas sensors",
url = "https://hdl.handle.net/21.15107/rcub_cer_5825"
}
Andrić, S., Jokić, I., Frantlović, M., Radulović, K.,& Spasenović, M.. (2022). Characterization of heterogeneous sensing layers in graphene-based gas sensors. in Proceedings - 10th International Scientific Conference on Defensive Technologies, OTEH 2022, 13-14 October 2022, Belgrade, Serbia
Belgrade : The Military Technical Institute..
https://hdl.handle.net/21.15107/rcub_cer_5825
Andrić S, Jokić I, Frantlović M, Radulović K, Spasenović M. Characterization of heterogeneous sensing layers in graphene-based gas sensors. in Proceedings - 10th International Scientific Conference on Defensive Technologies, OTEH 2022, 13-14 October 2022, Belgrade, Serbia. 2022;.
https://hdl.handle.net/21.15107/rcub_cer_5825 .
Andrić, Stevan, Jokić, Ivana, Frantlović, Miloš, Radulović, Katarina, Spasenović, Marko, "Characterization of heterogeneous sensing layers in graphene-based gas sensors" in Proceedings - 10th International Scientific Conference on Defensive Technologies, OTEH 2022, 13-14 October 2022, Belgrade, Serbia (2022),
https://hdl.handle.net/21.15107/rcub_cer_5825 .

Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water

Stevanović, Gordana; Jović-Jovičić, Nataša; Krstić, Jugoslav; Milutinović Nikolić, Aleksandra; Milovanović, Biljana; Radulović, Katarina; Ajduković, Marija

(Society of Physical Chemists of Serbia, 2021)

TY  - CONF
AU  - Stevanović, Gordana
AU  - Jović-Jovičić, Nataša
AU  - Krstić, Jugoslav
AU  - Milutinović Nikolić, Aleksandra
AU  - Milovanović, Biljana
AU  - Radulović, Katarina
AU  - Ajduković, Marija
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6683
AB  - In this work cobalt supported on chitosan-derived carbon-smectite composite catalyst was synthetized using impregnation-carbonization method (Co/cCh-S). The carbonization temperature was 400 °C. The obtained catalyst was tested as peroxymonosulfate (in form of Oxone®) activator for the food dye tartrazine degradation. The textural properties were obtained using low temperature N2 physisorption. The calculated textural parameters of the Co/cCh-S catalyst were compared with properties of the carbonized chitosane-smectite composite (cCh-S). The catalytic tests confirmed that neither Oxone® without catalyst nor cCh-S were unable to activate Oxone®. The catalyst Co/cCh-S was found to be effective for tartrazine degradation in presence of Oxone®.
PB  - Society of Physical Chemists of Serbia
C3  - Proceedings - 15th International Conference on Fundamental and Applied Aspects of Physical Chemistry, Physical Chemistry 2021, September 20-24 2021, Belgrade, Serbia
T1  - Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water
VL  - I
SP  - 151
EP  - 154
UR  - https://hdl.handle.net/21.15107/rcub_cer_6683
ER  - 
@conference{
author = "Stevanović, Gordana and Jović-Jovičić, Nataša and Krstić, Jugoslav and Milutinović Nikolić, Aleksandra and Milovanović, Biljana and Radulović, Katarina and Ajduković, Marija",
year = "2021",
abstract = "In this work cobalt supported on chitosan-derived carbon-smectite composite catalyst was synthetized using impregnation-carbonization method (Co/cCh-S). The carbonization temperature was 400 °C. The obtained catalyst was tested as peroxymonosulfate (in form of Oxone®) activator for the food dye tartrazine degradation. The textural properties were obtained using low temperature N2 physisorption. The calculated textural parameters of the Co/cCh-S catalyst were compared with properties of the carbonized chitosane-smectite composite (cCh-S). The catalytic tests confirmed that neither Oxone® without catalyst nor cCh-S were unable to activate Oxone®. The catalyst Co/cCh-S was found to be effective for tartrazine degradation in presence of Oxone®.",
publisher = "Society of Physical Chemists of Serbia",
journal = "Proceedings - 15th International Conference on Fundamental and Applied Aspects of Physical Chemistry, Physical Chemistry 2021, September 20-24 2021, Belgrade, Serbia",
title = "Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water",
volume = "I",
pages = "151-154",
url = "https://hdl.handle.net/21.15107/rcub_cer_6683"
}
Stevanović, G., Jović-Jovičić, N., Krstić, J., Milutinović Nikolić, A., Milovanović, B., Radulović, K.,& Ajduković, M.. (2021). Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water. in Proceedings - 15th International Conference on Fundamental and Applied Aspects of Physical Chemistry, Physical Chemistry 2021, September 20-24 2021, Belgrade, Serbia
Society of Physical Chemists of Serbia., I, 151-154.
https://hdl.handle.net/21.15107/rcub_cer_6683
Stevanović G, Jović-Jovičić N, Krstić J, Milutinović Nikolić A, Milovanović B, Radulović K, Ajduković M. Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water. in Proceedings - 15th International Conference on Fundamental and Applied Aspects of Physical Chemistry, Physical Chemistry 2021, September 20-24 2021, Belgrade, Serbia. 2021;I:151-154.
https://hdl.handle.net/21.15107/rcub_cer_6683 .
Stevanović, Gordana, Jović-Jovičić, Nataša, Krstić, Jugoslav, Milutinović Nikolić, Aleksandra, Milovanović, Biljana, Radulović, Katarina, Ajduković, Marija, "Cobalt supported chitosan-derived carbon-smectite composite for catalytic activation of peroxymonosulfate in water" in Proceedings - 15th International Conference on Fundamental and Applied Aspects of Physical Chemistry, Physical Chemistry 2021, September 20-24 2021, Belgrade, Serbia, I (2021):151-154,
https://hdl.handle.net/21.15107/rcub_cer_6683 .

Full-self-powered humidity sensor based on electrochemical aluminum–water reaction

Bošković, Marko V.; Šljukić, Biljana; Vasiljević-Radović, Dana; Radulović, Katarina; Rašljić Rafajilović, Milena; Frantlović, Miloš; Sarajlić, Milija

(MDPI, 2021)

TY  - JOUR
AU  - Bošković, Marko V.
AU  - Šljukić, Biljana
AU  - Vasiljević-Radović, Dana
AU  - Radulović, Katarina
AU  - Rašljić Rafajilović, Milena
AU  - Frantlović, Miloš
AU  - Sarajlić, Milija
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4697
AB  - A detailed examination of the principle of operation behind the functioning of the full-self-powered humidity sensor is presented. The sensor has been realized as a structure consisting of an interdigitated capacitor with aluminum thin-film digits. In this work, the details of its fabrication and activation are described in detail. The performed XRD, FTIR, SEM, AFM, and EIS analyses, as well as noise measurements, revealed that the dominant process of electricity generation is the electrochemical reaction between the sensor’s aluminum electrodes and the water from humid air in the presence of oxygen, which was the main goal of this work. The response of the sensor to human breath is also presented as a demonstration of its possible practical application.
PB  - MDPI
T2  - Sensors
T1  - Full-self-powered humidity sensor based on electrochemical aluminum–water reaction
VL  - 21
IS  - 10
SP  - 3486
DO  - 10.3390/s21103486
ER  - 
@article{
author = "Bošković, Marko V. and Šljukić, Biljana and Vasiljević-Radović, Dana and Radulović, Katarina and Rašljić Rafajilović, Milena and Frantlović, Miloš and Sarajlić, Milija",
year = "2021",
abstract = "A detailed examination of the principle of operation behind the functioning of the full-self-powered humidity sensor is presented. The sensor has been realized as a structure consisting of an interdigitated capacitor with aluminum thin-film digits. In this work, the details of its fabrication and activation are described in detail. The performed XRD, FTIR, SEM, AFM, and EIS analyses, as well as noise measurements, revealed that the dominant process of electricity generation is the electrochemical reaction between the sensor’s aluminum electrodes and the water from humid air in the presence of oxygen, which was the main goal of this work. The response of the sensor to human breath is also presented as a demonstration of its possible practical application.",
publisher = "MDPI",
journal = "Sensors",
title = "Full-self-powered humidity sensor based on electrochemical aluminum–water reaction",
volume = "21",
number = "10",
pages = "3486",
doi = "10.3390/s21103486"
}
Bošković, M. V., Šljukić, B., Vasiljević-Radović, D., Radulović, K., Rašljić Rafajilović, M., Frantlović, M.,& Sarajlić, M.. (2021). Full-self-powered humidity sensor based on electrochemical aluminum–water reaction. in Sensors
MDPI., 21(10), 3486.
https://doi.org/10.3390/s21103486
Bošković MV, Šljukić B, Vasiljević-Radović D, Radulović K, Rašljić Rafajilović M, Frantlović M, Sarajlić M. Full-self-powered humidity sensor based on electrochemical aluminum–water reaction. in Sensors. 2021;21(10):3486.
doi:10.3390/s21103486 .
Bošković, Marko V., Šljukić, Biljana, Vasiljević-Radović, Dana, Radulović, Katarina, Rašljić Rafajilović, Milena, Frantlović, Miloš, Sarajlić, Milija, "Full-self-powered humidity sensor based on electrochemical aluminum–water reaction" in Sensors, 21, no. 10 (2021):3486,
https://doi.org/10.3390/s21103486 . .
5
4

Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion

Jokić, Ivana; Jakšić, Olga; Frantlović, Miloš; Jakšić, Zoran; Radulović, Katarina

(IOP Publishing, 2021)

TY  - JOUR
AU  - Jokić, Ivana
AU  - Jakšić, Olga
AU  - Frantlović, Miloš
AU  - Jakšić, Zoran
AU  - Radulović, Katarina
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4726
AB  - Highly sensitive detection of biological analytes by plasmonic sensors is based on analyte adsorption, which modifies the effective refractive index (RI) at the medium-sensor interface. The main issue with such sensors is the non-ideal sensor selectivity (manifested in multiple analyte adsorption), while sample depletion (significant at low analyte concentrations) also causes a deviation of the sensor response from the expected time dependence. Mathematical modelling of sensor response, presented in this work, simultaneously tackles these two issues that may cause erroneous interpretation of measurement results. Two mathematical models that address the problem of limited selectivity are utilized to analyse the sensor response: the linear (pseudo-first order) model, commonly used for interpretation of measurements, and the nonlinear (second order) model that takes into account analyte depletion in the sensor chamber. While the nonlinear model has a virtue of generality, the advantages of the linear model are its simplicity and a well-established procedure for the analysis of experimental results. However, the linear model can exhibit large errors in the case of significant analyte depletion. Until now, the influence of analyte depletion on the linear model fidelity has not been studied for multianalyte adsorption. In this paper, we quantify the difference between the RI changes predicted by the two models of two-analyte competitive adsorption, and establish the conditions that justify the use of the linear model. The validity of these conditions is confirmed by numerically solving the exact nonlinear model equations. The conditions enable making an objective decision whether it is safe to use the linear model for detection of ultralow analyte concentrations, or the nonlinear model must be used in order to avoid false-positive/false-negative detection results and analyte quantification errors. The results are applicable in adsorption-based chemical/biological sensing in complex samples, as well as for the new generation single-element multianalyte plasmonic sensors.
PB  - IOP Publishing
T2  - Measurement Science and Technology
T1  - Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion
VL  - 32
IS  - 9
DO  - 10.1088/1361-6501/abfe85
ER  - 
@article{
author = "Jokić, Ivana and Jakšić, Olga and Frantlović, Miloš and Jakšić, Zoran and Radulović, Katarina",
year = "2021",
abstract = "Highly sensitive detection of biological analytes by plasmonic sensors is based on analyte adsorption, which modifies the effective refractive index (RI) at the medium-sensor interface. The main issue with such sensors is the non-ideal sensor selectivity (manifested in multiple analyte adsorption), while sample depletion (significant at low analyte concentrations) also causes a deviation of the sensor response from the expected time dependence. Mathematical modelling of sensor response, presented in this work, simultaneously tackles these two issues that may cause erroneous interpretation of measurement results. Two mathematical models that address the problem of limited selectivity are utilized to analyse the sensor response: the linear (pseudo-first order) model, commonly used for interpretation of measurements, and the nonlinear (second order) model that takes into account analyte depletion in the sensor chamber. While the nonlinear model has a virtue of generality, the advantages of the linear model are its simplicity and a well-established procedure for the analysis of experimental results. However, the linear model can exhibit large errors in the case of significant analyte depletion. Until now, the influence of analyte depletion on the linear model fidelity has not been studied for multianalyte adsorption. In this paper, we quantify the difference between the RI changes predicted by the two models of two-analyte competitive adsorption, and establish the conditions that justify the use of the linear model. The validity of these conditions is confirmed by numerically solving the exact nonlinear model equations. The conditions enable making an objective decision whether it is safe to use the linear model for detection of ultralow analyte concentrations, or the nonlinear model must be used in order to avoid false-positive/false-negative detection results and analyte quantification errors. The results are applicable in adsorption-based chemical/biological sensing in complex samples, as well as for the new generation single-element multianalyte plasmonic sensors.",
publisher = "IOP Publishing",
journal = "Measurement Science and Technology",
title = "Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion",
volume = "32",
number = "9",
doi = "10.1088/1361-6501/abfe85"
}
Jokić, I., Jakšić, O., Frantlović, M., Jakšić, Z.,& Radulović, K.. (2021). Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion. in Measurement Science and Technology
IOP Publishing., 32(9).
https://doi.org/10.1088/1361-6501/abfe85
Jokić I, Jakšić O, Frantlović M, Jakšić Z, Radulović K. Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion. in Measurement Science and Technology. 2021;32(9).
doi:10.1088/1361-6501/abfe85 .
Jokić, Ivana, Jakšić, Olga, Frantlović, Miloš, Jakšić, Zoran, Radulović, Katarina, "Modelling of plasmonic biosensor temporal response influenced by competitive adsorption and analyte depletion" in Measurement Science and Technology, 32, no. 9 (2021),
https://doi.org/10.1088/1361-6501/abfe85 . .
2

Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors

Jokić, Ivana; Đurić, Zoran G.; Radulović, Katarina; Frantlović, Miloš; Milovanović, Gradimir V.; Krstajić, Predrag

(MDPI, 2021)

TY  - JOUR
AU  - Jokić, Ivana
AU  - Đurić, Zoran G.
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Milovanović, Gradimir V.
AU  - Krstajić, Predrag
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4826
AB  - In order to improve the interpretation of measurement results and to achieve the optimal performance of microfluidic biosensors, advanced mathematical models of their time response and noise are needed. The random nature of adsorption–desorption and mass transfer (MT) processes that generate the sensor response makes the sensor output signal inherently stochastic and necessi-tates the use of a stochastic approach in sensor response analysis. We present a stochastic model of the sensor time response, which takes into account the coupling of adsorption–desorption and MT processes. It is used for the analysis of response kinetics and ultimate noise performance of protein biosensors. We show that slow MT not only decelerates the response kinetics, but also increases the noise and decreases the sensor’s maximal achievable signal‐to‐noise ratio, thus degrading the ultimate sensor performance, including the minimal detectable/quantifiable analyte concentration. The results illustrate the significance of the presented model for the correct interpretation of measurement data, for the estimation of sensors’ noise performance metrics important for reliable analyte detection/quantification, as well as for sensor optimization in terms of the lower detection/quanti-fication limit. They are also incentives for the further investigation of the MT influence in nanoscale sensors, as a possible cause of false‐negative results in analyte detection experiments.
PB  - MDPI
T2  - Biosensors
T1  - Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors
VL  - 11
IS  - 6
SP  - 194
DO  - 10.3390/bios11060194
ER  - 
@article{
author = "Jokić, Ivana and Đurić, Zoran G. and Radulović, Katarina and Frantlović, Miloš and Milovanović, Gradimir V. and Krstajić, Predrag",
year = "2021",
abstract = "In order to improve the interpretation of measurement results and to achieve the optimal performance of microfluidic biosensors, advanced mathematical models of their time response and noise are needed. The random nature of adsorption–desorption and mass transfer (MT) processes that generate the sensor response makes the sensor output signal inherently stochastic and necessi-tates the use of a stochastic approach in sensor response analysis. We present a stochastic model of the sensor time response, which takes into account the coupling of adsorption–desorption and MT processes. It is used for the analysis of response kinetics and ultimate noise performance of protein biosensors. We show that slow MT not only decelerates the response kinetics, but also increases the noise and decreases the sensor’s maximal achievable signal‐to‐noise ratio, thus degrading the ultimate sensor performance, including the minimal detectable/quantifiable analyte concentration. The results illustrate the significance of the presented model for the correct interpretation of measurement data, for the estimation of sensors’ noise performance metrics important for reliable analyte detection/quantification, as well as for sensor optimization in terms of the lower detection/quanti-fication limit. They are also incentives for the further investigation of the MT influence in nanoscale sensors, as a possible cause of false‐negative results in analyte detection experiments.",
publisher = "MDPI",
journal = "Biosensors",
title = "Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors",
volume = "11",
number = "6",
pages = "194",
doi = "10.3390/bios11060194"
}
Jokić, I., Đurić, Z. G., Radulović, K., Frantlović, M., Milovanović, G. V.,& Krstajić, P.. (2021). Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors. in Biosensors
MDPI., 11(6), 194.
https://doi.org/10.3390/bios11060194
Jokić I, Đurić ZG, Radulović K, Frantlović M, Milovanović GV, Krstajić P. Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors. in Biosensors. 2021;11(6):194.
doi:10.3390/bios11060194 .
Jokić, Ivana, Đurić, Zoran G., Radulović, Katarina, Frantlović, Miloš, Milovanović, Gradimir V., Krstajić, Predrag, "Stochastic time response and ultimate noise performance of adsorption‐based microfluidic biosensors" in Biosensors, 11, no. 6 (2021):194,
https://doi.org/10.3390/bios11060194 . .
2
2
2

Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects.

Rašljić Rafajilović, Milena; Radulović, Katarina; Smiljanić, Milče M.; Lazić, Žarko; Jakšić, Zoran; Stanisavljev, Dragomir; Vasiljević-Radović, Dana

(MDPI, 2020)

TY  - JOUR
AU  - Rašljić Rafajilović, Milena
AU  - Radulović, Katarina
AU  - Smiljanić, Milče M.
AU  - Lazić, Žarko
AU  - Jakšić, Zoran
AU  - Stanisavljev, Dragomir
AU  - Vasiljević-Radović, Dana
PY  - 2020
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4009
AB  - We present the design, simulation, fabrication and characterization of monolithically
integrated high resistivity p-type boron-di used silicon two-zone heaters in a model high temperature
microreactor intended for nanoparticle fabrication. We used a finite element method for simulations
of the heaters’ operation and performance. Our experimental model reactor structure consisted of
a silicon wafer anodically bonded to a Pyrex glass wafer with an isotropically etched serpentine
microchannels network. We fabricated two separate spiral heaters with di erent temperatures,
mutually thermally isolated by barrier apertures etched throughout the silicon wafer. The heaters
were characterized by electric measurements and by infrared thermal vision. The obtained results
show that our proposed procedure for the heater fabrication is robust, stable and controllable, with a
decreased sensitivity to random variations of fabrication process parameters. Compared to metallic or
polysilicon heaters typically integrated into microreactors, our approach o ers improved control over
heater characteristics through adjustment of the Boron doping level and profile. Our microreactor is
intended to produce titanium dioxide nanoparticles, but it could be also used to fabricate nanoparticles
in di erent materials as well, with various parameters and geometries. Our method can be generally
applied to other high-temperature microsystems.
PB  - MDPI
T2  - Micromachines
T1  - Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects.
VL  - 11
IS  - 9
SP  - 818
DO  - 10.3390/mi11090818
ER  - 
@article{
author = "Rašljić Rafajilović, Milena and Radulović, Katarina and Smiljanić, Milče M. and Lazić, Žarko and Jakšić, Zoran and Stanisavljev, Dragomir and Vasiljević-Radović, Dana",
year = "2020",
abstract = "We present the design, simulation, fabrication and characterization of monolithically
integrated high resistivity p-type boron-di used silicon two-zone heaters in a model high temperature
microreactor intended for nanoparticle fabrication. We used a finite element method for simulations
of the heaters’ operation and performance. Our experimental model reactor structure consisted of
a silicon wafer anodically bonded to a Pyrex glass wafer with an isotropically etched serpentine
microchannels network. We fabricated two separate spiral heaters with di erent temperatures,
mutually thermally isolated by barrier apertures etched throughout the silicon wafer. The heaters
were characterized by electric measurements and by infrared thermal vision. The obtained results
show that our proposed procedure for the heater fabrication is robust, stable and controllable, with a
decreased sensitivity to random variations of fabrication process parameters. Compared to metallic or
polysilicon heaters typically integrated into microreactors, our approach o ers improved control over
heater characteristics through adjustment of the Boron doping level and profile. Our microreactor is
intended to produce titanium dioxide nanoparticles, but it could be also used to fabricate nanoparticles
in di erent materials as well, with various parameters and geometries. Our method can be generally
applied to other high-temperature microsystems.",
publisher = "MDPI",
journal = "Micromachines",
title = "Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects.",
volume = "11",
number = "9",
pages = "818",
doi = "10.3390/mi11090818"
}
Rašljić Rafajilović, M., Radulović, K., Smiljanić, M. M., Lazić, Ž., Jakšić, Z., Stanisavljev, D.,& Vasiljević-Radović, D.. (2020). Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects.. in Micromachines
MDPI., 11(9), 818.
https://doi.org/10.3390/mi11090818
Rašljić Rafajilović M, Radulović K, Smiljanić MM, Lazić Ž, Jakšić Z, Stanisavljev D, Vasiljević-Radović D. Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects.. in Micromachines. 2020;11(9):818.
doi:10.3390/mi11090818 .
Rašljić Rafajilović, Milena, Radulović, Katarina, Smiljanić, Milče M., Lazić, Žarko, Jakšić, Zoran, Stanisavljev, Dragomir, Vasiljević-Radović, Dana, "Monolithically Integrated Diffused Silicon Two-Zone Heaters for Silicon-Pyrex Glass Microreactors for Production of Nanoparticles: Heat Exchange Aspects." in Micromachines, 11, no. 9 (2020):818,
https://doi.org/10.3390/mi11090818 . .
4
2
4

The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling

Jakšić, Olga; Jokić, Ivana; Jakšić, Zoran; Mladenović, Ivana; Radulović, Katarina; Frantlović, Miloš

(Springer Nature, 2020)

TY  - JOUR
AU  - Jakšić, Olga
AU  - Jokić, Ivana
AU  - Jakšić, Zoran
AU  - Mladenović, Ivana
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
PY  - 2020
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3493
AB  - In order to allow for multiscale modeling of complex systems we focus on various approaches to modeling binary adsorption. We consider multiple methods of  modeling the temporal response of general plasmonic sensors. We start from the analytical approach. The kinetics of adsorption and desorption is modeled both as a first order reaction and as a second order reaction. The criteria for their validity and the choice between them in the case of two-component adsorption are established. Due to the nonlinearities of the second order reactions and the lack of their analytical solutions, computer aided modeling is considered next, also in multiple ways: the employment of numerical solvers, fitting of experimental results, the stochastic simulation algorithms and the employment of artificial neural networks (ANN). The examples we present illustrate the advantages and disadvantages of the particular approaches. The goal is to aid the concurrent multiscale modeling of adsorption-based devices. Machine learning in ANN performed here is used to estimate the equilibrium values of adsorbed quantities. The obtained results show that to train an ANN for the estimation of the equilibrium adsorption quantities the Levenberg-Marquardt and the Bayesian regularization algorithms are less efficient than the quasi-Newton BFGS (Broyden-Fletcher-Goldfarb-Shanno) algorithm.
PB  - Springer Nature
T2  - Applied Physics A
T1  - The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling
VL  - 126
SP  - 342
DO  - 10.1007/s00339-020-03524-3
ER  - 
@article{
author = "Jakšić, Olga and Jokić, Ivana and Jakšić, Zoran and Mladenović, Ivana and Radulović, Katarina and Frantlović, Miloš",
year = "2020",
abstract = "In order to allow for multiscale modeling of complex systems we focus on various approaches to modeling binary adsorption. We consider multiple methods of  modeling the temporal response of general plasmonic sensors. We start from the analytical approach. The kinetics of adsorption and desorption is modeled both as a first order reaction and as a second order reaction. The criteria for their validity and the choice between them in the case of two-component adsorption are established. Due to the nonlinearities of the second order reactions and the lack of their analytical solutions, computer aided modeling is considered next, also in multiple ways: the employment of numerical solvers, fitting of experimental results, the stochastic simulation algorithms and the employment of artificial neural networks (ANN). The examples we present illustrate the advantages and disadvantages of the particular approaches. The goal is to aid the concurrent multiscale modeling of adsorption-based devices. Machine learning in ANN performed here is used to estimate the equilibrium values of adsorbed quantities. The obtained results show that to train an ANN for the estimation of the equilibrium adsorption quantities the Levenberg-Marquardt and the Bayesian regularization algorithms are less efficient than the quasi-Newton BFGS (Broyden-Fletcher-Goldfarb-Shanno) algorithm.",
publisher = "Springer Nature",
journal = "Applied Physics A",
title = "The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling",
volume = "126",
pages = "342",
doi = "10.1007/s00339-020-03524-3"
}
Jakšić, O., Jokić, I., Jakšić, Z., Mladenović, I., Radulović, K.,& Frantlović, M.. (2020). The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling. in Applied Physics A
Springer Nature., 126, 342.
https://doi.org/10.1007/s00339-020-03524-3
Jakšić O, Jokić I, Jakšić Z, Mladenović I, Radulović K, Frantlović M. The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling. in Applied Physics A. 2020;126:342.
doi:10.1007/s00339-020-03524-3 .
Jakšić, Olga, Jokić, Ivana, Jakšić, Zoran, Mladenović, Ivana, Radulović, Katarina, Frantlović, Miloš, "The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling" in Applied Physics A, 126 (2020):342,
https://doi.org/10.1007/s00339-020-03524-3 . .
1
3
2
3

The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling

Jakšić, Olga; Jokić, Ivana; Jakšić, Zoran; Mladenović, Ivana; Radulović, Katarina; Frantlović, Miloš

(Springer Nature, 2020)

TY  - JOUR
AU  - Jakšić, Olga
AU  - Jokić, Ivana
AU  - Jakšić, Zoran
AU  - Mladenović, Ivana
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
PY  - 2020
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3494
AB  - In order to allow for multiscale modeling of complex systems we focus on various approaches to modeling binary adsorption. We consider multiple methods of  modeling the temporal response of general plasmonic sensors. We start from the analytical approach. The kinetics of adsorption and desorption is modeled both as a first order reaction and as a second order reaction. The criteria for their validity and the choice between them in the case of two-component adsorption are established. Due to the nonlinearities of the second order reactions and the lack of their analytical solutions, computer aided modeling is considered next, also in multiple ways: the employment of numerical solvers, fitting of experimental results, the stochastic simulation algorithms and the employment of artificial neural networks (ANN). The examples we present illustrate the advantages and disadvantages of the particular approaches. The goal is to aid the concurrent multiscale modeling of adsorption-based devices. Machine learning in ANN performed here is used to estimate the equilibrium values of adsorbed quantities. The obtained results show that to train an ANN for the estimation of the equilibrium adsorption quantities the Levenberg-Marquardt and the Bayesian regularization algorithms are less efficient than the quasi-Newton BFGS (Broyden-Fletcher-Goldfarb-Shanno) algorithm.
PB  - Springer Nature
T2  - Applied Physics A
T1  - The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling
VL  - 126
SP  - 342
DO  - 10.1007/s00339-020-03524-3
ER  - 
@article{
author = "Jakšić, Olga and Jokić, Ivana and Jakšić, Zoran and Mladenović, Ivana and Radulović, Katarina and Frantlović, Miloš",
year = "2020",
abstract = "In order to allow for multiscale modeling of complex systems we focus on various approaches to modeling binary adsorption. We consider multiple methods of  modeling the temporal response of general plasmonic sensors. We start from the analytical approach. The kinetics of adsorption and desorption is modeled both as a first order reaction and as a second order reaction. The criteria for their validity and the choice between them in the case of two-component adsorption are established. Due to the nonlinearities of the second order reactions and the lack of their analytical solutions, computer aided modeling is considered next, also in multiple ways: the employment of numerical solvers, fitting of experimental results, the stochastic simulation algorithms and the employment of artificial neural networks (ANN). The examples we present illustrate the advantages and disadvantages of the particular approaches. The goal is to aid the concurrent multiscale modeling of adsorption-based devices. Machine learning in ANN performed here is used to estimate the equilibrium values of adsorbed quantities. The obtained results show that to train an ANN for the estimation of the equilibrium adsorption quantities the Levenberg-Marquardt and the Bayesian regularization algorithms are less efficient than the quasi-Newton BFGS (Broyden-Fletcher-Goldfarb-Shanno) algorithm.",
publisher = "Springer Nature",
journal = "Applied Physics A",
title = "The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling",
volume = "126",
pages = "342",
doi = "10.1007/s00339-020-03524-3"
}
Jakšić, O., Jokić, I., Jakšić, Z., Mladenović, I., Radulović, K.,& Frantlović, M.. (2020). The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling. in Applied Physics A
Springer Nature., 126, 342.
https://doi.org/10.1007/s00339-020-03524-3
Jakšić O, Jokić I, Jakšić Z, Mladenović I, Radulović K, Frantlović M. The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling. in Applied Physics A. 2020;126:342.
doi:10.1007/s00339-020-03524-3 .
Jakšić, Olga, Jokić, Ivana, Jakšić, Zoran, Mladenović, Ivana, Radulović, Katarina, Frantlović, Miloš, "The time response of plasmonic sensors due to binary adsorption: analytical versus numerical modeling" in Applied Physics A, 126 (2020):342,
https://doi.org/10.1007/s00339-020-03524-3 . .
1
3
2
3

Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase

Vuković, Marina; Dinić, Ivana; Nikolić, Marko G.; Marinković, Bojan A.; Costa, Antonio Mario Leal Martins; Radulović, Katarina; Milošević, Olivera; Mančić, Lidija

(Springer, 2020)

TY  - JOUR
AU  - Vuković, Marina
AU  - Dinić, Ivana
AU  - Nikolić, Marko G.
AU  - Marinković, Bojan A.
AU  - Costa, Antonio Mario Leal Martins
AU  - Radulović, Katarina
AU  - Milošević, Olivera
AU  - Mančić, Lidija
PY  - 2020
UR  - https://doi.org/10.1007/s12034-019-1975-1
UR  - http://dais.sanu.ac.rs/123456789/6911
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3324
AB  - Up-converting NaYF4:Yb,Er nanoparticles were obtained by polymer-assisted solvothermal synthesis using a common solution of hydrated RE nitrates in ethanol or ethylene glycol. It was shown that polymer choice (polyacrylic acid—PAA, polyvinylpyrrolidone—PVP and chitosan—CS) controls the size and shape of NaYF4:Yb,Er nanoparticles, while the solvent type and pH value affect their crystallinity. Consequently, the spherical nanoparticles of a cubic (α) phase, the average size of which ranged from 60 to 140 nm, were obtained either when PVP/ethanol or PVP/ethylene glycol were used solely during synthesis, whereas NaOH addition induced hexagonal (β) phase nucleation. The formation of the hierarchically organized spherical aggregates and nanofoils was observed when CS and PAA were used during synthesis, respectively. The average crystallite size, microstrain, doping level, lattice parameters, as well as, the presence of the certain ligands on the particle surface were determined and correlated with the intensity of visible-light emission observed under 980 nm laser-diode excitation.
PB  - Springer
T2  - Bulletin of Materials Science
T1  - Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase
VL  - 43
IS  - 1
SP  - 2
DO  - 10.1007/s12034-019-1975-1
ER  - 
@article{
author = "Vuković, Marina and Dinić, Ivana and Nikolić, Marko G. and Marinković, Bojan A. and Costa, Antonio Mario Leal Martins and Radulović, Katarina and Milošević, Olivera and Mančić, Lidija",
year = "2020",
abstract = "Up-converting NaYF4:Yb,Er nanoparticles were obtained by polymer-assisted solvothermal synthesis using a common solution of hydrated RE nitrates in ethanol or ethylene glycol. It was shown that polymer choice (polyacrylic acid—PAA, polyvinylpyrrolidone—PVP and chitosan—CS) controls the size and shape of NaYF4:Yb,Er nanoparticles, while the solvent type and pH value affect their crystallinity. Consequently, the spherical nanoparticles of a cubic (α) phase, the average size of which ranged from 60 to 140 nm, were obtained either when PVP/ethanol or PVP/ethylene glycol were used solely during synthesis, whereas NaOH addition induced hexagonal (β) phase nucleation. The formation of the hierarchically organized spherical aggregates and nanofoils was observed when CS and PAA were used during synthesis, respectively. The average crystallite size, microstrain, doping level, lattice parameters, as well as, the presence of the certain ligands on the particle surface were determined and correlated with the intensity of visible-light emission observed under 980 nm laser-diode excitation.",
publisher = "Springer",
journal = "Bulletin of Materials Science",
title = "Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase",
volume = "43",
number = "1",
pages = "2",
doi = "10.1007/s12034-019-1975-1"
}
Vuković, M., Dinić, I., Nikolić, M. G., Marinković, B. A., Costa, A. M. L. M., Radulović, K., Milošević, O.,& Mančić, L.. (2020). Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase. in Bulletin of Materials Science
Springer., 43(1), 2.
https://doi.org/10.1007/s12034-019-1975-1
Vuković M, Dinić I, Nikolić MG, Marinković BA, Costa AMLM, Radulović K, Milošević O, Mančić L. Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase. in Bulletin of Materials Science. 2020;43(1):2.
doi:10.1007/s12034-019-1975-1 .
Vuković, Marina, Dinić, Ivana, Nikolić, Marko G., Marinković, Bojan A., Costa, Antonio Mario Leal Martins, Radulović, Katarina, Milošević, Olivera, Mančić, Lidija, "Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase" in Bulletin of Materials Science, 43, no. 1 (2020):2,
https://doi.org/10.1007/s12034-019-1975-1 . .
5
2
5

Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase

Vuković, Marina; Dinić, Ivana; Nikolić, Marko G.; Marinković, Bojan A.; Costa, Antonio Mario Leal Martins; Radulović, Katarina; Milošević, Olivera; Mančić, Lidija

(Springer, 2020)

TY  - JOUR
AU  - Vuković, Marina
AU  - Dinić, Ivana
AU  - Nikolić, Marko G.
AU  - Marinković, Bojan A.
AU  - Costa, Antonio Mario Leal Martins
AU  - Radulović, Katarina
AU  - Milošević, Olivera
AU  - Mančić, Lidija
PY  - 2020
UR  - https://doi.org/10.1007/s12034-019-1975-1
UR  - http://dais.sanu.ac.rs/123456789/6912
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3323
AB  - Up-converting NaYF4:Yb,Er nanoparticles were obtained by polymer-assisted solvothermal synthesis using a common solution of hydrated RE nitrates in ethanol or ethylene glycol. It was shown that polymer choice (polyacrylic acid—PAA, polyvinylpyrrolidone—PVP and chitosan—CS) controls the size and shape of NaYF4:Yb,Er nanoparticles, while the solvent type and pH value affect their crystallinity. Consequently, the spherical nanoparticles of a cubic (α) phase, the average size of which ranged from 60 to 140 nm, were obtained either when PVP/ethanol or PVP/ethylene glycol were used solely during synthesis, whereas NaOH addition induced hexagonal (β) phase nucleation. The formation of the hierarchically organized spherical aggregates and nanofoils was observed when CS and PAA were used during synthesis, respectively. The average crystallite size, microstrain, doping level, lattice parameters, as well as, the presence of the certain ligands on the particle surface were determined and correlated with the intensity of visible-light emission observed under 980 nm laser-diode excitation.
PB  - Springer
T2  - Bulletin of Materials Science
T1  - Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase
VL  - 43
IS  - 1
SP  - 2
DO  - 10.1007/s12034-019-1975-1
ER  - 
@article{
author = "Vuković, Marina and Dinić, Ivana and Nikolić, Marko G. and Marinković, Bojan A. and Costa, Antonio Mario Leal Martins and Radulović, Katarina and Milošević, Olivera and Mančić, Lidija",
year = "2020",
abstract = "Up-converting NaYF4:Yb,Er nanoparticles were obtained by polymer-assisted solvothermal synthesis using a common solution of hydrated RE nitrates in ethanol or ethylene glycol. It was shown that polymer choice (polyacrylic acid—PAA, polyvinylpyrrolidone—PVP and chitosan—CS) controls the size and shape of NaYF4:Yb,Er nanoparticles, while the solvent type and pH value affect their crystallinity. Consequently, the spherical nanoparticles of a cubic (α) phase, the average size of which ranged from 60 to 140 nm, were obtained either when PVP/ethanol or PVP/ethylene glycol were used solely during synthesis, whereas NaOH addition induced hexagonal (β) phase nucleation. The formation of the hierarchically organized spherical aggregates and nanofoils was observed when CS and PAA were used during synthesis, respectively. The average crystallite size, microstrain, doping level, lattice parameters, as well as, the presence of the certain ligands on the particle surface were determined and correlated with the intensity of visible-light emission observed under 980 nm laser-diode excitation.",
publisher = "Springer",
journal = "Bulletin of Materials Science",
title = "Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase",
volume = "43",
number = "1",
pages = "2",
doi = "10.1007/s12034-019-1975-1"
}
Vuković, M., Dinić, I., Nikolić, M. G., Marinković, B. A., Costa, A. M. L. M., Radulović, K., Milošević, O.,& Mančić, L.. (2020). Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase. in Bulletin of Materials Science
Springer., 43(1), 2.
https://doi.org/10.1007/s12034-019-1975-1
Vuković M, Dinić I, Nikolić MG, Marinković BA, Costa AMLM, Radulović K, Milošević O, Mančić L. Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase. in Bulletin of Materials Science. 2020;43(1):2.
doi:10.1007/s12034-019-1975-1 .
Vuković, Marina, Dinić, Ivana, Nikolić, Marko G., Marinković, Bojan A., Costa, Antonio Mario Leal Martins, Radulović, Katarina, Milošević, Olivera, Mančić, Lidija, "Effects of different polymers and solvents on crystallization of the NaYF4:Yb/Er phase" in Bulletin of Materials Science, 43, no. 1 (2020):2,
https://doi.org/10.1007/s12034-019-1975-1 . .
5
2
5

Microselectromechanical system (MEMS) based microfluidic platforms

Vasiljević-Radović, Dana; Rašljić, Milena; Smiljanić, Milče M.; Lazić, Žarko; Radulović, Katarina; Cvetanović-Zobenica, Katarina

(Belgrade : ETRAN Society / Beograd : Društvo za ETRAN, 2019)

TY  - CONF
AU  - Vasiljević-Radović, Dana
AU  - Rašljić, Milena
AU  - Smiljanić, Milče M.
AU  - Lazić, Žarko
AU  - Radulović, Katarina
AU  - Cvetanović-Zobenica, Katarina
PY  - 2019
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7420
AB  - In this work an overview of Micro Electromechanical
Systems (MEMS)-based microfluidic platforms for
different applications is presented. Microfluidics refers
to a set of technologies that control the flow of liquids or
gases through miniaturized systems in typical amounts of
nano- and pico- liters. Microfluidic devices are
characterized by microchannels with characteristic
dimensions in the micrometer range. The main
techniques, technologies and materials used for
fabrication of MEMS microfluidic devices and systems
are presented. The used materials and their properties are
very important for the final characteristics and
functionalities of devices. As an example, the design and
fabrication of our opto-fluidic lab-on-a-chip device based
on silicon and pyrex glass is given.
PB  - Belgrade : ETRAN Society / Beograd : Društvo za ETRAN
C3  - Proceedings of papers - (Ic) ETRAN 6th International Conference on Electrical, Electronical and Computing Engineering, June 03-06 2019, Silver Lake, Serbia
T1  - Microselectromechanical system (MEMS) based microfluidic platforms
SP  - 570
EP  - 570
UR  - https://hdl.handle.net/21.15107/rcub_cer_7420
ER  - 
@conference{
author = "Vasiljević-Radović, Dana and Rašljić, Milena and Smiljanić, Milče M. and Lazić, Žarko and Radulović, Katarina and Cvetanović-Zobenica, Katarina",
year = "2019",
abstract = "In this work an overview of Micro Electromechanical
Systems (MEMS)-based microfluidic platforms for
different applications is presented. Microfluidics refers
to a set of technologies that control the flow of liquids or
gases through miniaturized systems in typical amounts of
nano- and pico- liters. Microfluidic devices are
characterized by microchannels with characteristic
dimensions in the micrometer range. The main
techniques, technologies and materials used for
fabrication of MEMS microfluidic devices and systems
are presented. The used materials and their properties are
very important for the final characteristics and
functionalities of devices. As an example, the design and
fabrication of our opto-fluidic lab-on-a-chip device based
on silicon and pyrex glass is given.",
publisher = "Belgrade : ETRAN Society / Beograd : Društvo za ETRAN",
journal = "Proceedings of papers - (Ic) ETRAN 6th International Conference on Electrical, Electronical and Computing Engineering, June 03-06 2019, Silver Lake, Serbia",
title = "Microselectromechanical system (MEMS) based microfluidic platforms",
pages = "570-570",
url = "https://hdl.handle.net/21.15107/rcub_cer_7420"
}
Vasiljević-Radović, D., Rašljić, M., Smiljanić, M. M., Lazić, Ž., Radulović, K.,& Cvetanović-Zobenica, K.. (2019). Microselectromechanical system (MEMS) based microfluidic platforms. in Proceedings of papers - (Ic) ETRAN 6th International Conference on Electrical, Electronical and Computing Engineering, June 03-06 2019, Silver Lake, Serbia
Belgrade : ETRAN Society / Beograd : Društvo za ETRAN., 570-570.
https://hdl.handle.net/21.15107/rcub_cer_7420
Vasiljević-Radović D, Rašljić M, Smiljanić MM, Lazić Ž, Radulović K, Cvetanović-Zobenica K. Microselectromechanical system (MEMS) based microfluidic platforms. in Proceedings of papers - (Ic) ETRAN 6th International Conference on Electrical, Electronical and Computing Engineering, June 03-06 2019, Silver Lake, Serbia. 2019;:570-570.
https://hdl.handle.net/21.15107/rcub_cer_7420 .
Vasiljević-Radović, Dana, Rašljić, Milena, Smiljanić, Milče M., Lazić, Žarko, Radulović, Katarina, Cvetanović-Zobenica, Katarina, "Microselectromechanical system (MEMS) based microfluidic platforms" in Proceedings of papers - (Ic) ETRAN 6th International Conference on Electrical, Electronical and Computing Engineering, June 03-06 2019, Silver Lake, Serbia (2019):570-570,
https://hdl.handle.net/21.15107/rcub_cer_7420 .

A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing

Stevanović, Jelena; Lazić, Žarko; Smiljanić, Milče M.; Radulović, Katarina; Randjelović, Danijela; Frantlović, Miloš; Sarajlić, Milija

(Belgrade : ETRAN Society, 2019)

TY  - CONF
AU  - Stevanović, Jelena
AU  - Lazić, Žarko
AU  - Smiljanić, Milče M.
AU  - Radulović, Katarina
AU  - Randjelović, Danijela
AU  - Frantlović, Miloš
AU  - Sarajlić, Milija
PY  - 2019
UR  - https://www.etran.rs/2019/IcETRAN/About_Conference/
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4007
AB  - A consideration study for the application of the pressure sensor SP-12 developed and produced by ICTM CMT as an ultrasound sensor is given. The interaction of ultrasound with the sensor’s membrane was analytically described, but for the initial examination of its performance, Finite Elements Method simulation was applied. The sensor SP-12 has eigenfrequencies in the range from 200 kHz to the frequencies higher than 2 MHz. The amplitude of the output signal, which is proportional to Von Mises stress, is highest for the lowest frequency, and it exponentially decreases as the eigenfrequencies increase. This makes the sensor suitable for the ultrasound measurements in the range of hundreds of kHz
PB  - Belgrade : ETRAN Society
PB  - Belgrade : Akademska misao
C3  - Proceedings - 6th International Conference on Electrical, Electronics and Computing Engineering, IcETRAN 2019
T1  - A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing
UR  - https://hdl.handle.net/21.15107/rcub_cer_4007
ER  - 
@conference{
author = "Stevanović, Jelena and Lazić, Žarko and Smiljanić, Milče M. and Radulović, Katarina and Randjelović, Danijela and Frantlović, Miloš and Sarajlić, Milija",
year = "2019",
abstract = "A consideration study for the application of the pressure sensor SP-12 developed and produced by ICTM CMT as an ultrasound sensor is given. The interaction of ultrasound with the sensor’s membrane was analytically described, but for the initial examination of its performance, Finite Elements Method simulation was applied. The sensor SP-12 has eigenfrequencies in the range from 200 kHz to the frequencies higher than 2 MHz. The amplitude of the output signal, which is proportional to Von Mises stress, is highest for the lowest frequency, and it exponentially decreases as the eigenfrequencies increase. This makes the sensor suitable for the ultrasound measurements in the range of hundreds of kHz",
publisher = "Belgrade : ETRAN Society, Belgrade : Akademska misao",
journal = "Proceedings - 6th International Conference on Electrical, Electronics and Computing Engineering, IcETRAN 2019",
title = "A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing",
url = "https://hdl.handle.net/21.15107/rcub_cer_4007"
}
Stevanović, J., Lazić, Ž., Smiljanić, M. M., Radulović, K., Randjelović, D., Frantlović, M.,& Sarajlić, M.. (2019). A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing. in Proceedings - 6th International Conference on Electrical, Electronics and Computing Engineering, IcETRAN 2019
Belgrade : ETRAN Society..
https://hdl.handle.net/21.15107/rcub_cer_4007
Stevanović J, Lazić Ž, Smiljanić MM, Radulović K, Randjelović D, Frantlović M, Sarajlić M. A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing. in Proceedings - 6th International Conference on Electrical, Electronics and Computing Engineering, IcETRAN 2019. 2019;.
https://hdl.handle.net/21.15107/rcub_cer_4007 .
Stevanović, Jelena, Lazić, Žarko, Smiljanić, Milče M., Radulović, Katarina, Randjelović, Danijela, Frantlović, Miloš, Sarajlić, Milija, "A consideration of the use of ICTM SP-12 pressure sensor for ultrasound sensing" in Proceedings - 6th International Conference on Electrical, Electronics and Computing Engineering, IcETRAN 2019 (2019),
https://hdl.handle.net/21.15107/rcub_cer_4007 .

Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters

Mladenović, Ivana; Lamovec, Jelena; Jović, Vesna; Obradov, Marko; Radulović, Katarina; Vasiljević-Radović, Dana; Radojević, Vesna

(Institute of Electrical and Electronics Engineers (IEEE), 2019)

TY  - CONF
AU  - Mladenović, Ivana
AU  - Lamovec, Jelena
AU  - Jović, Vesna
AU  - Obradov, Marko
AU  - Radulović, Katarina
AU  - Vasiljević-Radović, Dana
AU  - Radojević, Vesna
PY  - 2019
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3227
AB  - Copper coatings are produced on silicon wafer by electrodeposition (ED) for various cathode current densities. The resulting composite systems consist of 10 μm monolayered copper films electrodeposited from sulphate bath on Si wafers with sputtered layers of Cr/Au. Hardness measurements were performed to evaluate properties of the composites. The composite hardness (H c ) was characterized using Vickers microindentation test. Then, an artificial neural network (ANN) model was used to study the relationship between the parameters of metallic composite and their hardness. Two experimental values: applied load during indentation test and current density during the ED process were used as the inputs to the neural network. Finally, the results of the composite hardness (experimental and predicted) were used to estimate the film hardness (H f ) of copper for each variations of the current density. This article shows that ANN is an useful tool in modeling composite hardness change with variation of experimental parameters predicting hardness change of composite Si/Cu with average error of 6 %. Using created ANN model it is possible to predict microhardness of Cu film for current density or indentation load for which we do not have experimental data.
PB  - Institute of Electrical and Electronics Engineers (IEEE)
C3  - 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
T1  - Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters
SP  - 133
EP  - 136
DO  - 10.1109/MIEL.2019.8889610
ER  - 
@conference{
author = "Mladenović, Ivana and Lamovec, Jelena and Jović, Vesna and Obradov, Marko and Radulović, Katarina and Vasiljević-Radović, Dana and Radojević, Vesna",
year = "2019",
abstract = "Copper coatings are produced on silicon wafer by electrodeposition (ED) for various cathode current densities. The resulting composite systems consist of 10 μm monolayered copper films electrodeposited from sulphate bath on Si wafers with sputtered layers of Cr/Au. Hardness measurements were performed to evaluate properties of the composites. The composite hardness (H c ) was characterized using Vickers microindentation test. Then, an artificial neural network (ANN) model was used to study the relationship between the parameters of metallic composite and their hardness. Two experimental values: applied load during indentation test and current density during the ED process were used as the inputs to the neural network. Finally, the results of the composite hardness (experimental and predicted) were used to estimate the film hardness (H f ) of copper for each variations of the current density. This article shows that ANN is an useful tool in modeling composite hardness change with variation of experimental parameters predicting hardness change of composite Si/Cu with average error of 6 %. Using created ANN model it is possible to predict microhardness of Cu film for current density or indentation load for which we do not have experimental data.",
publisher = "Institute of Electrical and Electronics Engineers (IEEE)",
journal = "2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings",
title = "Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters",
pages = "133-136",
doi = "10.1109/MIEL.2019.8889610"
}
Mladenović, I., Lamovec, J., Jović, V., Obradov, M., Radulović, K., Vasiljević-Radović, D.,& Radojević, V.. (2019). Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
Institute of Electrical and Electronics Engineers (IEEE)., 133-136.
https://doi.org/10.1109/MIEL.2019.8889610
Mladenović I, Lamovec J, Jović V, Obradov M, Radulović K, Vasiljević-Radović D, Radojević V. Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings. 2019;:133-136.
doi:10.1109/MIEL.2019.8889610 .
Mladenović, Ivana, Lamovec, Jelena, Jović, Vesna, Obradov, Marko, Radulović, Katarina, Vasiljević-Radović, Dana, Radojević, Vesna, "Artificial Neural Network for Composite Hardness Modeling of Cu/Si Systems Fabricated Using Various Electrodeposition Parameters" in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings (2019):133-136,
https://doi.org/10.1109/MIEL.2019.8889610 . .
1
1

Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures

Jokić, Ivana; Đurić, Zoran G.; Radulović, Katarina; Frantlović, Miloš; Krstajić, Predrag

(Institute of Electrical and Electronics Engineers (IEEE), 2019)

TY  - CONF
AU  - Jokić, Ivana
AU  - Đurić, Zoran G.
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Krstajić, Predrag
PY  - 2019
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3256
AB  - Real-time in situ operation of bio/chemical sensors assumes detection of chemical substances or biological specimens in samples of complex composition. Since sensor selectivity cannot be ideal, adsorption of particles other than target particles inevitably occur on the sensing surface. That affects the sensor response and its intrinsic fluctuations which are caused by stochastic fluctuations of the numbers of adsorbed particles of all the adsorbing substances. In microfluidic sensors, such response fluctuations are a result of coupled adsorption, desorption and mass transfer (convection and diffusion) processes of analyte particles. Analysis of these fluctuations is important because they constitute the adsorption-desorption noise, which limits the sensing performance. In this work we perform the analysis of fluctuations by using a stochastic model of sensor response after the steady state is reached, in the case of two-analyte adsorption, considering mass transfer processes. The results enable estimation of the ultimate sensing performance of adsorption-based microfluidic bio/chemical sensors of different sensing areas, operating in bianalyte mixture environments.
PB  - Institute of Electrical and Electronics Engineers (IEEE)
C3  - 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
T1  - Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures
SP  - 161
EP  - 164
DO  - 10.1109/MIEL.2019.8889579
ER  - 
@conference{
author = "Jokić, Ivana and Đurić, Zoran G. and Radulović, Katarina and Frantlović, Miloš and Krstajić, Predrag",
year = "2019",
abstract = "Real-time in situ operation of bio/chemical sensors assumes detection of chemical substances or biological specimens in samples of complex composition. Since sensor selectivity cannot be ideal, adsorption of particles other than target particles inevitably occur on the sensing surface. That affects the sensor response and its intrinsic fluctuations which are caused by stochastic fluctuations of the numbers of adsorbed particles of all the adsorbing substances. In microfluidic sensors, such response fluctuations are a result of coupled adsorption, desorption and mass transfer (convection and diffusion) processes of analyte particles. Analysis of these fluctuations is important because they constitute the adsorption-desorption noise, which limits the sensing performance. In this work we perform the analysis of fluctuations by using a stochastic model of sensor response after the steady state is reached, in the case of two-analyte adsorption, considering mass transfer processes. The results enable estimation of the ultimate sensing performance of adsorption-based microfluidic bio/chemical sensors of different sensing areas, operating in bianalyte mixture environments.",
publisher = "Institute of Electrical and Electronics Engineers (IEEE)",
journal = "2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings",
title = "Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures",
pages = "161-164",
doi = "10.1109/MIEL.2019.8889579"
}
Jokić, I., Đurić, Z. G., Radulović, K., Frantlović, M.,& Krstajić, P.. (2019). Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
Institute of Electrical and Electronics Engineers (IEEE)., 161-164.
https://doi.org/10.1109/MIEL.2019.8889579
Jokić I, Đurić ZG, Radulović K, Frantlović M, Krstajić P. Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings. 2019;:161-164.
doi:10.1109/MIEL.2019.8889579 .
Jokić, Ivana, Đurić, Zoran G., Radulović, Katarina, Frantlović, Miloš, Krstajić, Predrag, "Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures" in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings (2019):161-164,
https://doi.org/10.1109/MIEL.2019.8889579 . .

Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors

Jokić, Ivana; Radulović, Katarina; Frantlović, Miloš; Đurić, Zoran G.; Cvetanović Zobenica, Katarina; Krstajić, Predrag

(Belgrade : ETRAN, 2019)

TY  - CONF
AU  - Jokić, Ivana
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Đurić, Zoran G.
AU  - Cvetanović Zobenica, Katarina
AU  - Krstajić, Predrag
PY  - 2019
UR  - http://dais.sanu.ac.rs/123456789/6961
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3326
AB  - Detection limits in microfluidic chemical and biological sensors, which determine the range of analyte concentrations reliably detectable by the sensor, are important sensor parameters. The lower limit of detection, defined as the lowest concentration that can be distinguished from noise, has its minimum determined by the fundamental adsorption-desorption (AD) noise, inevitable in adsorption-based devices. In this work, we analyze this fundamental detection limit, particularly considering the influence of mass transfer processes in microfluidic devices. For that purpose, we derive the expression for the sensor’s signal-to-noise ratio (SNR), which takes into account the AD noise, and then the equation for the minimal analyte concentration at which the SNR has a sufficiently high value for reliable analyte detection. Subsequently, we analyze the mass transfer influence on the sensor’s maximal achievable signal-to-noise ratio and on the fundamental detection limit. The results of the analysis show a significant mass transfer influence on these important sensor performance metrics. They also provide guidelines for achieving the sensor’s best possible detection performance through the optimization of the sensor design and operating conditions.
PB  - Belgrade : ETRAN
PB  - Belgrade :Academic Mind
C3  - Proceedings of Papers – 6th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2019, Silver Lake, Serbia, June 03 – 06, 2019 / Zbornik radova - 63. Konferencija za elektroniku, telekomunikacije, računarstvo, automatiku i nuklearnu tehniku, Srebrno jezero, 03 – 06. juna, 2019. godine
T1  - Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors
SP  - 571
EP  - 574
UR  - https://hdl.handle.net/21.15107/rcub_dais_6961
ER  - 
@conference{
author = "Jokić, Ivana and Radulović, Katarina and Frantlović, Miloš and Đurić, Zoran G. and Cvetanović Zobenica, Katarina and Krstajić, Predrag",
year = "2019",
abstract = "Detection limits in microfluidic chemical and biological sensors, which determine the range of analyte concentrations reliably detectable by the sensor, are important sensor parameters. The lower limit of detection, defined as the lowest concentration that can be distinguished from noise, has its minimum determined by the fundamental adsorption-desorption (AD) noise, inevitable in adsorption-based devices. In this work, we analyze this fundamental detection limit, particularly considering the influence of mass transfer processes in microfluidic devices. For that purpose, we derive the expression for the sensor’s signal-to-noise ratio (SNR), which takes into account the AD noise, and then the equation for the minimal analyte concentration at which the SNR has a sufficiently high value for reliable analyte detection. Subsequently, we analyze the mass transfer influence on the sensor’s maximal achievable signal-to-noise ratio and on the fundamental detection limit. The results of the analysis show a significant mass transfer influence on these important sensor performance metrics. They also provide guidelines for achieving the sensor’s best possible detection performance through the optimization of the sensor design and operating conditions.",
publisher = "Belgrade : ETRAN, Belgrade :Academic Mind",
journal = "Proceedings of Papers – 6th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2019, Silver Lake, Serbia, June 03 – 06, 2019 / Zbornik radova - 63. Konferencija za elektroniku, telekomunikacije, računarstvo, automatiku i nuklearnu tehniku, Srebrno jezero, 03 – 06. juna, 2019. godine",
title = "Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors",
pages = "571-574",
url = "https://hdl.handle.net/21.15107/rcub_dais_6961"
}
Jokić, I., Radulović, K., Frantlović, M., Đurić, Z. G., Cvetanović Zobenica, K.,& Krstajić, P.. (2019). Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors. in Proceedings of Papers – 6th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2019, Silver Lake, Serbia, June 03 – 06, 2019 / Zbornik radova - 63. Konferencija za elektroniku, telekomunikacije, računarstvo, automatiku i nuklearnu tehniku, Srebrno jezero, 03 – 06. juna, 2019. godine
Belgrade : ETRAN., 571-574.
https://hdl.handle.net/21.15107/rcub_dais_6961
Jokić I, Radulović K, Frantlović M, Đurić ZG, Cvetanović Zobenica K, Krstajić P. Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors. in Proceedings of Papers – 6th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2019, Silver Lake, Serbia, June 03 – 06, 2019 / Zbornik radova - 63. Konferencija za elektroniku, telekomunikacije, računarstvo, automatiku i nuklearnu tehniku, Srebrno jezero, 03 – 06. juna, 2019. godine. 2019;:571-574.
https://hdl.handle.net/21.15107/rcub_dais_6961 .
Jokić, Ivana, Radulović, Katarina, Frantlović, Miloš, Đurić, Zoran G., Cvetanović Zobenica, Katarina, Krstajić, Predrag, "Analysis of the Fundamental Detection Limit in Microfluidic Chemical and Biological Sensors" in Proceedings of Papers – 6th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2019, Silver Lake, Serbia, June 03 – 06, 2019 / Zbornik radova - 63. Konferencija za elektroniku, telekomunikacije, računarstvo, automatiku i nuklearnu tehniku, Srebrno jezero, 03 – 06. juna, 2019. godine (2019):571-574,
https://hdl.handle.net/21.15107/rcub_dais_6961 .

Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures

Jokić, Ivana; Đurić, Zoran G.; Radulović, Katarina; Frantlović, Miloš; Krstajić, Predrag

(Institute of Electrical and Electronics Engineers (IEEE), 2019)

TY  - CONF
AU  - Jokić, Ivana
AU  - Đurić, Zoran G.
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Krstajić, Predrag
PY  - 2019
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4866
AB  - Real-time in situ operation of bio/chemical sensors assumes detection of chemical substances or biological specimens in samples of complex composition. Since sensor selectivity cannot be ideal, adsorption of particles other than target particles inevitably occur on the sensing surface. That affects the sensor response and its intrinsic fluctuations which are caused by stochastic fluctuations of the numbers of adsorbed particles of all the adsorbing substances. In microfluidic sensors, such response fluctuations are a result of coupled adsorption, desorption and mass transfer (convection and diffusion) processes of analyte particles. Analysis of these fluctuations is important because they constitute the adsorption-desorption noise, which limits the sensing performance. In this work we perform the analysis of fluctuations by using a stochastic model of sensor response after the steady state is reached, in the case of two-analyte adsorption, considering mass transfer processes. The results enable estimation of the ultimate sensing performance of adsorption-based microfluidic bio/chemical sensors of different sensing areas, operating in bianalyte mixture environments.
PB  - Institute of Electrical and Electronics Engineers (IEEE)
C3  - 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
T1  - Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures
SP  - 161
EP  - 164
DO  - 10.1109/MIEL.2019.8889579
ER  - 
@conference{
author = "Jokić, Ivana and Đurić, Zoran G. and Radulović, Katarina and Frantlović, Miloš and Krstajić, Predrag",
year = "2019",
abstract = "Real-time in situ operation of bio/chemical sensors assumes detection of chemical substances or biological specimens in samples of complex composition. Since sensor selectivity cannot be ideal, adsorption of particles other than target particles inevitably occur on the sensing surface. That affects the sensor response and its intrinsic fluctuations which are caused by stochastic fluctuations of the numbers of adsorbed particles of all the adsorbing substances. In microfluidic sensors, such response fluctuations are a result of coupled adsorption, desorption and mass transfer (convection and diffusion) processes of analyte particles. Analysis of these fluctuations is important because they constitute the adsorption-desorption noise, which limits the sensing performance. In this work we perform the analysis of fluctuations by using a stochastic model of sensor response after the steady state is reached, in the case of two-analyte adsorption, considering mass transfer processes. The results enable estimation of the ultimate sensing performance of adsorption-based microfluidic bio/chemical sensors of different sensing areas, operating in bianalyte mixture environments.",
publisher = "Institute of Electrical and Electronics Engineers (IEEE)",
journal = "2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings",
title = "Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures",
pages = "161-164",
doi = "10.1109/MIEL.2019.8889579"
}
Jokić, I., Đurić, Z. G., Radulović, K., Frantlović, M.,& Krstajić, P.. (2019). Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings
Institute of Electrical and Electronics Engineers (IEEE)., 161-164.
https://doi.org/10.1109/MIEL.2019.8889579
Jokić I, Đurić ZG, Radulović K, Frantlović M, Krstajić P. Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures. in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings. 2019;:161-164.
doi:10.1109/MIEL.2019.8889579 .
Jokić, Ivana, Đurić, Zoran G., Radulović, Katarina, Frantlović, Miloš, Krstajić, Predrag, "Analysis of Intrinsic Stochastic Fluctuations of the Time Response of Adsorption-Based Microfluidic Bio/Chemical Sensors: the Case of Bianalyte Mixtures" in 2019 IEEE 31st International Conference on Microelectronics, MIEL 2019 - Proceedings (2019):161-164,
https://doi.org/10.1109/MIEL.2019.8889579 . .

Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors

Rašljić, Milena; Smiljanić, Milče M.; Lazić, Žarko; Radulović, Katarina; Cvetanović Zobenica, Katarina; Vasiljević-Radović, Dana

(Belgrade : ETRAN Society, 2018)

TY  - CONF
AU  - Rašljić, Milena
AU  - Smiljanić, Milče M.
AU  - Lazić, Žarko
AU  - Radulović, Katarina
AU  - Cvetanović Zobenica, Katarina
AU  - Vasiljević-Radović, Dana
PY  - 2018
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5730
AB  - In this paper it is shown how we fabricated two types of heaters for microreactors which are used in synthesis of TiO2 nanoparticles. We used standard photolithographic processes to design gold and p-type heaters diffused in n-type silicon substrate. Heaters are designed to be integrated part of microreactors. The temperature necessary for synthesis of TiO2 nanoparticles is achieved with both types of heaters. P-type diffused heaters are shown better in terms of power
consumption.
PB  - Belgrade : ETRAN Society
C3  - Proceedings of Papers – 5th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2018, 11-14.06.2018, Palić
T1  - Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors
SP  - 953
EP  - 956
UR  - https://hdl.handle.net/21.15107/rcub_cer_5730
ER  - 
@conference{
author = "Rašljić, Milena and Smiljanić, Milče M. and Lazić, Žarko and Radulović, Katarina and Cvetanović Zobenica, Katarina and Vasiljević-Radović, Dana",
year = "2018",
abstract = "In this paper it is shown how we fabricated two types of heaters for microreactors which are used in synthesis of TiO2 nanoparticles. We used standard photolithographic processes to design gold and p-type heaters diffused in n-type silicon substrate. Heaters are designed to be integrated part of microreactors. The temperature necessary for synthesis of TiO2 nanoparticles is achieved with both types of heaters. P-type diffused heaters are shown better in terms of power
consumption.",
publisher = "Belgrade : ETRAN Society",
journal = "Proceedings of Papers – 5th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2018, 11-14.06.2018, Palić",
title = "Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors",
pages = "953-956",
url = "https://hdl.handle.net/21.15107/rcub_cer_5730"
}
Rašljić, M., Smiljanić, M. M., Lazić, Ž., Radulović, K., Cvetanović Zobenica, K.,& Vasiljević-Radović, D.. (2018). Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors. in Proceedings of Papers – 5th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2018, 11-14.06.2018, Palić
Belgrade : ETRAN Society., 953-956.
https://hdl.handle.net/21.15107/rcub_cer_5730
Rašljić M, Smiljanić MM, Lazić Ž, Radulović K, Cvetanović Zobenica K, Vasiljević-Radović D. Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors. in Proceedings of Papers – 5th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2018, 11-14.06.2018, Palić. 2018;:953-956.
https://hdl.handle.net/21.15107/rcub_cer_5730 .
Rašljić, Milena, Smiljanić, Milče M., Lazić, Žarko, Radulović, Katarina, Cvetanović Zobenica, Katarina, Vasiljević-Radović, Dana, "Two types of integrated heaters for synthesis of TiO2 nanoparticles in microreactors" in Proceedings of Papers – 5th International Conference on Electrical, Electronic and Computing Engineering, IcETRAN 2018, 11-14.06.2018, Palić (2018):953-956,
https://hdl.handle.net/21.15107/rcub_cer_5730 .

Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors

Jokić, Ivana; Đurić, Zoran G.; Radulović, Katarina; Frantlović, Miloš; Krstajić, Predrag; Cvetanović Zobenica, Katarina

(ETRAN, 2018)

TY  - CONF
AU  - Jokić, Ivana
AU  - Đurić, Zoran G.
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Krstajić, Predrag
AU  - Cvetanović Zobenica, Katarina
PY  - 2018
UR  - https://www.etran.rs/2018/IcETRAN/News/IcETRAN%20sumarni%20program%20sekcija_Ver.%204.3%20(1).pdf
UR  - http://dais.sanu.ac.rs/123456789/4630
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/2859
AB  - In this paper we first give a short review of two stochastic models describing both the expected value and variance of the random number of adsorbed particles in microfluidic adsorption-based chemical and biological sensors. One model takes into account the influence of coupling of stochastic adsorptiondesorption processes and mass transfer on the change of the number of adsorbed particles, while the other neglects the influence of mass transfer. Subsequently, by using the two models, we perform the analysis of the expected value and variance, as well as the sensor's signal-to-noise ratio, after reaching the steady state of all transient processes. We compare the results obtained by using the different models, and determine conditions for their application. We estimate the influences of the sensing surface area and the concentration of target particles on statistical parameters of sensor response and signal-to-noise ratio, considering the cases where mass transfer is significant, and those where it is not. We particularly analyze the mass transfer influence on the expected value, variance and signal-to-noise ratio. Such analysis does not exist in the available literature. The presented analysis yields new knowledge about the stochastic response of adsorption-based sensors, and it is significant for their optimization in order to achieve reliable analyte detection and improved sensing performance.
PB  - ETRAN
C3  - IcETRAN & ETRAN 2018, Palić 11-14. 06. 2018: Program
T1  - Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors
UR  - https://hdl.handle.net/21.15107/rcub_dais_4630
ER  - 
@conference{
author = "Jokić, Ivana and Đurić, Zoran G. and Radulović, Katarina and Frantlović, Miloš and Krstajić, Predrag and Cvetanović Zobenica, Katarina",
year = "2018",
abstract = "In this paper we first give a short review of two stochastic models describing both the expected value and variance of the random number of adsorbed particles in microfluidic adsorption-based chemical and biological sensors. One model takes into account the influence of coupling of stochastic adsorptiondesorption processes and mass transfer on the change of the number of adsorbed particles, while the other neglects the influence of mass transfer. Subsequently, by using the two models, we perform the analysis of the expected value and variance, as well as the sensor's signal-to-noise ratio, after reaching the steady state of all transient processes. We compare the results obtained by using the different models, and determine conditions for their application. We estimate the influences of the sensing surface area and the concentration of target particles on statistical parameters of sensor response and signal-to-noise ratio, considering the cases where mass transfer is significant, and those where it is not. We particularly analyze the mass transfer influence on the expected value, variance and signal-to-noise ratio. Such analysis does not exist in the available literature. The presented analysis yields new knowledge about the stochastic response of adsorption-based sensors, and it is significant for their optimization in order to achieve reliable analyte detection and improved sensing performance.",
publisher = "ETRAN",
journal = "IcETRAN & ETRAN 2018, Palić 11-14. 06. 2018: Program",
title = "Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors",
url = "https://hdl.handle.net/21.15107/rcub_dais_4630"
}
Jokić, I., Đurić, Z. G., Radulović, K., Frantlović, M., Krstajić, P.,& Cvetanović Zobenica, K.. (2018). Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors. in IcETRAN & ETRAN 2018, Palić 11-14. 06. 2018: Program
ETRAN..
https://hdl.handle.net/21.15107/rcub_dais_4630
Jokić I, Đurić ZG, Radulović K, Frantlović M, Krstajić P, Cvetanović Zobenica K. Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors. in IcETRAN & ETRAN 2018, Palić 11-14. 06. 2018: Program. 2018;.
https://hdl.handle.net/21.15107/rcub_dais_4630 .
Jokić, Ivana, Đurić, Zoran G., Radulović, Katarina, Frantlović, Miloš, Krstajić, Predrag, Cvetanović Zobenica, Katarina, "Steady-state analysis of stochastic time response of chemical and biological microfluidic sensors" in IcETRAN & ETRAN 2018, Palić 11-14. 06. 2018: Program (2018),
https://hdl.handle.net/21.15107/rcub_dais_4630 .

MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise

Jokić, Ivana; Radulović, Katarina; Frantlović, Miloš; Đurić, Zoran; Krstajić, Predrag

(Belgrade : The Military Technical Institute, 2018)

TY  - CONF
AU  - Jokić, Ivana
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
AU  - Đurić, Zoran
AU  - Krstajić, Predrag
PY  - 2018
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5709
AB  - We analyze the time response of MEMS/NEMS sensors of chemical and biological agents and its noise, by using two mathematical models. One of them is commonly used in the literature on MEMS/NEMS adsorption-based chemical and biological sensors, while the other one, which is more elaborate, and takes into account additional relevant physical processes, has been developed by us. We also investigate the limits of applicability of the two models as a function of the target substance concentration, especially having in mind the decrease of the minimal detectable concentration in the new sensor generation.
PB  - Belgrade : The Military Technical Institute
C3  - Proceedings - 8th International Scientific Conference of Defensive Technologies, OTEH 2018, 11-12.10.2018, Belgrade
T1  - MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise
UR  - https://hdl.handle.net/21.15107/rcub_cer_5709
ER  - 
@conference{
author = "Jokić, Ivana and Radulović, Katarina and Frantlović, Miloš and Đurić, Zoran and Krstajić, Predrag",
year = "2018",
abstract = "We analyze the time response of MEMS/NEMS sensors of chemical and biological agents and its noise, by using two mathematical models. One of them is commonly used in the literature on MEMS/NEMS adsorption-based chemical and biological sensors, while the other one, which is more elaborate, and takes into account additional relevant physical processes, has been developed by us. We also investigate the limits of applicability of the two models as a function of the target substance concentration, especially having in mind the decrease of the minimal detectable concentration in the new sensor generation.",
publisher = "Belgrade : The Military Technical Institute",
journal = "Proceedings - 8th International Scientific Conference of Defensive Technologies, OTEH 2018, 11-12.10.2018, Belgrade",
title = "MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise",
url = "https://hdl.handle.net/21.15107/rcub_cer_5709"
}
Jokić, I., Radulović, K., Frantlović, M., Đurić, Z.,& Krstajić, P.. (2018). MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise. in Proceedings - 8th International Scientific Conference of Defensive Technologies, OTEH 2018, 11-12.10.2018, Belgrade
Belgrade : The Military Technical Institute..
https://hdl.handle.net/21.15107/rcub_cer_5709
Jokić I, Radulović K, Frantlović M, Đurić Z, Krstajić P. MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise. in Proceedings - 8th International Scientific Conference of Defensive Technologies, OTEH 2018, 11-12.10.2018, Belgrade. 2018;.
https://hdl.handle.net/21.15107/rcub_cer_5709 .
Jokić, Ivana, Radulović, Katarina, Frantlović, Miloš, Đurić, Zoran, Krstajić, Predrag, "MEMS/NEMS sensors of chemical and biological agents: applicability of different models for stedy-state analysis of sensor time response and noise" in Proceedings - 8th International Scientific Conference of Defensive Technologies, OTEH 2018, 11-12.10.2018, Belgrade (2018),
https://hdl.handle.net/21.15107/rcub_cer_5709 .

Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes

Jokić, Ivana; Đurić, Zoran G.; Radulović, Katarina; Frantlović, Miloš

(MDPI, 2018)

TY  - CONF
AU  - Jokić, Ivana
AU  - Đurić, Zoran G.
AU  - Radulović, Katarina
AU  - Frantlović, Miloš
PY  - 2018
UR  - https://www.mdpi.com/2504-3900/2/13/991
UR  - http://dais.sanu.ac.rs/123456789/4715
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/2607
AB  - A model of stochastic time response of adsorption-based microfluidic biosensors is presented, that considers the competitive adsorption-desorption process coupled with mass transfer of two analytes. By using the model we analyze the expected value of the adsorbed particles number of each analyte, which determine the sensor response kinetics. The comparison with the case when only one analyte exists is used for investigation of the influence of competitive adsorption on the sensor response. The response kinetics analyzed by using the stochastic model is compared with the kinetics predicted by the deterministic response model. The results are useful for optimization of micro/nanosensors intended for detection of substances in ultra-low concentrations in complex samples.
PB  - MDPI
C3  - Proceedings, Volume 2, Eurosensors 2018
T1  - Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes
VL  - 2
IS  - 13
SP  - 991
DO  - 10.3390/proceedings2130991
ER  - 
@conference{
author = "Jokić, Ivana and Đurić, Zoran G. and Radulović, Katarina and Frantlović, Miloš",
year = "2018",
abstract = "A model of stochastic time response of adsorption-based microfluidic biosensors is presented, that considers the competitive adsorption-desorption process coupled with mass transfer of two analytes. By using the model we analyze the expected value of the adsorbed particles number of each analyte, which determine the sensor response kinetics. The comparison with the case when only one analyte exists is used for investigation of the influence of competitive adsorption on the sensor response. The response kinetics analyzed by using the stochastic model is compared with the kinetics predicted by the deterministic response model. The results are useful for optimization of micro/nanosensors intended for detection of substances in ultra-low concentrations in complex samples.",
publisher = "MDPI",
journal = "Proceedings, Volume 2, Eurosensors 2018",
title = "Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes",
volume = "2",
number = "13",
pages = "991",
doi = "10.3390/proceedings2130991"
}
Jokić, I., Đurić, Z. G., Radulović, K.,& Frantlović, M.. (2018). Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes. in Proceedings, Volume 2, Eurosensors 2018
MDPI., 2(13), 991.
https://doi.org/10.3390/proceedings2130991
Jokić I, Đurić ZG, Radulović K, Frantlović M. Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes. in Proceedings, Volume 2, Eurosensors 2018. 2018;2(13):991.
doi:10.3390/proceedings2130991 .
Jokić, Ivana, Đurić, Zoran G., Radulović, Katarina, Frantlović, Miloš, "Analysis of Stochastic Time Response of Microfluidic Biosensors in the Case of Competitive Adsorption of Two Analytes" in Proceedings, Volume 2, Eurosensors 2018, 2, no. 13 (2018):991,
https://doi.org/10.3390/proceedings2130991 . .
2