Anđelković, Ljubica

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Authority KeyName Variants
orcid::0000-0001-5971-5383
  • Anđelković, Ljubica (62)
Projects
Rational design and synthesis of biologically active and coordination compounds and functional materials, relevant for (bio)nanotechnology Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200026 (University of Belgrade, Institute of Chemistry, Technology and Metallurgy - IChTM)
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200017 (University of Belgrade, Institute of Nuclear Sciences 'Vinča', Belgrade-Vinča) Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200168 (University of Belgrade, Faculty of Chemistry)
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200116 (University of Belgrade, Faculty of Agriculture) Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200162 (University of Belgrade, Faculty of Physics)
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200288 (Innovation Center of the Faculty of Chemistry) Swiss National Science Foundation
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200126 (University of Belgrade, Faculty of Mining and Geology) German Academic Exchange Service (DAAD)
Diagnostics and Optimization of Plasma Sources Important for Applications Structure-properties relationships of natural and synthetic molecules and their metal complexes
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200053 (University of Belgrade, Institute for Multidisciplinary Research) Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200175 (Institute of Technical Sciences of SASA, Belgrade)
NOOM-SeC - Nano-objects in own matrix: Self composite National Institutes of Health (NIH) [R01-GM106443]
Serbian-German bilateral project [451-03-01038/2015-09/7] Startup for Science 2017/18
COST Action CM1305 - ECOSTBio (Explicit Control Over Spin-states in Technology and Biochemistry) COST Action "COnvergent Distributed Environment for Computational Spectroscopy (CODECS)'' - CM1002
DIUE of the Generalitat de Catalunya (Xarxa de Referencia en Quimica Teorica i Computacional) [2009SGR528] FEDER fund (European Fund for Regional Development) [UNGI08-4E-003]
ICREA Molecular properties and modifications of some respiratory and nutritional allergens
Application of advanced oxidation processes and nanostructured oxide materials for the removal of pollutants from the environment, development and optimisation of instrumental techniques for efficiency monitoring Interactions of natural products, their derivatives and coordination compounds with proteins and nucleic acids
Directed synthesis, structure and properties of multifunctional materials Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200024 (University of Belgrade, Institute of Physics, Belgrade-Zemun)
Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200088 (University of Kragujevac, Faculty of Agronomy, Čačak) Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 451-03-68/2020-14/200105 (University of Belgrade, Faculty of Mechanical Engineering)

Author's Bibliography

Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles

Anđelković, Ljubica; Šuljagić, Marija; Pavlović, Vladimir; Mirković, Miljana; Vrbica, Boško; Novaković, Irena; Stanković, Dalibor; Kremenović, Aleksandar; Uskoković, Vuk

(Elsevier, 2024)

TY  - JOUR
AU  - Anđelković, Ljubica
AU  - Šuljagić, Marija
AU  - Pavlović, Vladimir
AU  - Mirković, Miljana
AU  - Vrbica, Boško
AU  - Novaković, Irena
AU  - Stanković, Dalibor
AU  - Kremenović, Aleksandar
AU  - Uskoković, Vuk
PY  - 2024
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7552
AB  - Metals and metal oxides have subpar antibacterial activities compared to those of small-molecule antibiotics, yet there are hopes that with proper compositional and structural adjustments this gap might be bridged. In this study, titanium dioxide (TiO2) nanoparticles were mechanically activated and combined with particulate silver through simple reduction process elicited by UV irradiation and assisted with the ultrasound. The resulting powders in various combinations (Ag vs. no Ag, activated vs. non-activated) were characterized using a range of experimental techniques and assessed for their antibacterial activities. The preparation procedure presented in this work prevails over the disadvantages of many chemical routes, most critically by avoiding the use of toxic substances. The mechanical activation did not reduce the particle size or crystallinity of TiO2 nor did it consistently alter the bandgap, yet it enabled the doubling of the amount of silver incorporable into the material. Further, while both mechanical activation and the addition of silver in the amount not exceeding 0.5 wt% produced barely detectable structural changes in the material, they both augmented its antibacterial activity. The precursor TiO2 powder produced no inhibition zone against any of the four bacterial species tested, while the mechanical activation of TiO2 led to the formation of distinct inhibition zones against each of the four bacterial species tested. The addition of silver to activated TiO2 further widened the inhibition zones and it also imparted the antibacterial activity to non-activated TiO2. The boost in the antibacterial activity achieved by the short mechanical activation was of a similar magnitude as the boost obtained after the addition of silver. The antibacterial activity was not different for different species when no silver was added to the system. However, with the addition of silver, species selectivity was obtained, as the composites were more effective against the two Gram-negative species (Escherichia coli and Klebsiella pneumoniae) than against the two Gram-positive ones (Staphylococcus aureus and Bacillus subtilis). The antibacterial activity increased with the addition of silver in the broth assay, but it was mediocre compared to that detected in the agar assay, attesting to the poor dispersability of the powders and their best performance when the bacterial cells migrate to the composite surface than vice versa. The findings of this study give hope that with appropriate microstructural or compositional alterations, the antibacterial activity of metal oxide powders and inorganic materials in general can be made comparable to that of small-molecule antibiotics.
PB  - Elsevier
T2  - Colloids and Surfaces A: Physicochemical and Engineering Aspects
T1  - Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles
VL  - 691
SP  - 133890
DO  - 10.1016/j.colsurfa.2024.133890
ER  - 
@article{
author = "Anđelković, Ljubica and Šuljagić, Marija and Pavlović, Vladimir and Mirković, Miljana and Vrbica, Boško and Novaković, Irena and Stanković, Dalibor and Kremenović, Aleksandar and Uskoković, Vuk",
year = "2024",
abstract = "Metals and metal oxides have subpar antibacterial activities compared to those of small-molecule antibiotics, yet there are hopes that with proper compositional and structural adjustments this gap might be bridged. In this study, titanium dioxide (TiO2) nanoparticles were mechanically activated and combined with particulate silver through simple reduction process elicited by UV irradiation and assisted with the ultrasound. The resulting powders in various combinations (Ag vs. no Ag, activated vs. non-activated) were characterized using a range of experimental techniques and assessed for their antibacterial activities. The preparation procedure presented in this work prevails over the disadvantages of many chemical routes, most critically by avoiding the use of toxic substances. The mechanical activation did not reduce the particle size or crystallinity of TiO2 nor did it consistently alter the bandgap, yet it enabled the doubling of the amount of silver incorporable into the material. Further, while both mechanical activation and the addition of silver in the amount not exceeding 0.5 wt% produced barely detectable structural changes in the material, they both augmented its antibacterial activity. The precursor TiO2 powder produced no inhibition zone against any of the four bacterial species tested, while the mechanical activation of TiO2 led to the formation of distinct inhibition zones against each of the four bacterial species tested. The addition of silver to activated TiO2 further widened the inhibition zones and it also imparted the antibacterial activity to non-activated TiO2. The boost in the antibacterial activity achieved by the short mechanical activation was of a similar magnitude as the boost obtained after the addition of silver. The antibacterial activity was not different for different species when no silver was added to the system. However, with the addition of silver, species selectivity was obtained, as the composites were more effective against the two Gram-negative species (Escherichia coli and Klebsiella pneumoniae) than against the two Gram-positive ones (Staphylococcus aureus and Bacillus subtilis). The antibacterial activity increased with the addition of silver in the broth assay, but it was mediocre compared to that detected in the agar assay, attesting to the poor dispersability of the powders and their best performance when the bacterial cells migrate to the composite surface than vice versa. The findings of this study give hope that with appropriate microstructural or compositional alterations, the antibacterial activity of metal oxide powders and inorganic materials in general can be made comparable to that of small-molecule antibiotics.",
publisher = "Elsevier",
journal = "Colloids and Surfaces A: Physicochemical and Engineering Aspects",
title = "Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles",
volume = "691",
pages = "133890",
doi = "10.1016/j.colsurfa.2024.133890"
}
Anđelković, L., Šuljagić, M., Pavlović, V., Mirković, M., Vrbica, B., Novaković, I., Stanković, D., Kremenović, A.,& Uskoković, V.. (2024). Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles. in Colloids and Surfaces A: Physicochemical and Engineering Aspects
Elsevier., 691, 133890.
https://doi.org/10.1016/j.colsurfa.2024.133890
Anđelković L, Šuljagić M, Pavlović V, Mirković M, Vrbica B, Novaković I, Stanković D, Kremenović A, Uskoković V. Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles. in Colloids and Surfaces A: Physicochemical and Engineering Aspects. 2024;691:133890.
doi:10.1016/j.colsurfa.2024.133890 .
Anđelković, Ljubica, Šuljagić, Marija, Pavlović, Vladimir, Mirković, Miljana, Vrbica, Boško, Novaković, Irena, Stanković, Dalibor, Kremenović, Aleksandar, Uskoković, Vuk, "Mechanical activation and silver supplementation as determinants of the antibacterial activity of titanium dioxide nanoparticles" in Colloids and Surfaces A: Physicochemical and Engineering Aspects, 691 (2024):133890,
https://doi.org/10.1016/j.colsurfa.2024.133890 . .

The influence of strontium content and sintering temperature on monazite stability

Mirković, Miljana; Maletaškić, Jelena; Butulija, Svetlana; Anđelković, Ljubica; Šuljagić, Marija

(Association for ETRAN Society, 2024)

TY  - JOUR
AU  - Mirković, Miljana
AU  - Maletaškić, Jelena
AU  - Butulija, Svetlana
AU  - Anđelković, Ljubica
AU  - Šuljagić, Marija
PY  - 2024
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7551
AB  - This paper shows a simple way to synthesize a series of Ce1-xSrxPO4 ceramic materials using acetate solutions of Ce and Sr instead of nitrate which were used so far. For synthesis, the preparation method was used by simple mixing of acetate solutions of Ceand Sr(, with NaH2PO4 at room temperature, and the studied compositions were Ce1-xSrxPO4 (where x = 0, 0.1, 0.2, 0.3, 0.4, 0.5). The disintegration of Sr in monazite structures in different sintering temperature ranges from 600°C to 1000°C was investigated. The X-ray diffraction was used to track the evolution of the phase composition with thermal treatment. The morphology of sintered ceramics was obtained by scanning electron microscopy and vibrational bands of selected spectra were observed using the FT-IR method. Relative geometric density of selected samples was evaluated. The most favorable conditions for obtaining high-temperature Ce, Sr phosphate-based ceramic material are reported.
AB  - У овом раду је приказан једноставан начин да се синтетише серија Ce1-xSrxPO4 керамичких материјала коришћењем ацетатних раствора Ce и Sr уместо до сада коришћених нитрата. За синтезу је коришћен метод припреме једноставним мешањем раствора Ce(C2H3O2)3·xH2O), Sr(C2H3O2)2, и NaH2PO4 као прекурсора на собној температури, а испитивани састави су Ce1-xSrxPO4 (где је к = 0 , 0,1, 0,2, 0,3, 0,4, 0,5). Испитивана је дезинтеграција Sr у структурама моназита у различитим температурним распонима синтеровања од 600 °C до 1000 °C. Дифракција рендгенских зрака на праху (XRD) је коришћена за праћење еволуције фазног састава синтетисаних и синтерованих узорака. Морфологија синтероване керамике испитивана је скенирајућом електронском микроскопијом (СЕМ), а вибрациое траке одабраних спектра су испитане ФТИР методом. Згушњавање и еволуција микроструктуре су одређене коришћењем релативне геометријске густине одабраних узорака. Приказани су најповољнији услови за добијање високотемпературног керамичког материјала на бази Ce, Sr фосфата.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - The influence of strontium content and sintering temperature on monazite stability
VL  - 56
SP  - 115
EP  - 121
DO  - 10.2298/SOS220811024M
ER  - 
@article{
author = "Mirković, Miljana and Maletaškić, Jelena and Butulija, Svetlana and Anđelković, Ljubica and Šuljagić, Marija",
year = "2024",
abstract = "This paper shows a simple way to synthesize a series of Ce1-xSrxPO4 ceramic materials using acetate solutions of Ce and Sr instead of nitrate which were used so far. For synthesis, the preparation method was used by simple mixing of acetate solutions of Ceand Sr(, with NaH2PO4 at room temperature, and the studied compositions were Ce1-xSrxPO4 (where x = 0, 0.1, 0.2, 0.3, 0.4, 0.5). The disintegration of Sr in monazite structures in different sintering temperature ranges from 600°C to 1000°C was investigated. The X-ray diffraction was used to track the evolution of the phase composition with thermal treatment. The morphology of sintered ceramics was obtained by scanning electron microscopy and vibrational bands of selected spectra were observed using the FT-IR method. Relative geometric density of selected samples was evaluated. The most favorable conditions for obtaining high-temperature Ce, Sr phosphate-based ceramic material are reported., У овом раду је приказан једноставан начин да се синтетише серија Ce1-xSrxPO4 керамичких материјала коришћењем ацетатних раствора Ce и Sr уместо до сада коришћених нитрата. За синтезу је коришћен метод припреме једноставним мешањем раствора Ce(C2H3O2)3·xH2O), Sr(C2H3O2)2, и NaH2PO4 као прекурсора на собној температури, а испитивани састави су Ce1-xSrxPO4 (где је к = 0 , 0,1, 0,2, 0,3, 0,4, 0,5). Испитивана је дезинтеграција Sr у структурама моназита у различитим температурним распонима синтеровања од 600 °C до 1000 °C. Дифракција рендгенских зрака на праху (XRD) је коришћена за праћење еволуције фазног састава синтетисаних и синтерованих узорака. Морфологија синтероване керамике испитивана је скенирајућом електронском микроскопијом (СЕМ), а вибрациое траке одабраних спектра су испитане ФТИР методом. Згушњавање и еволуција микроструктуре су одређене коришћењем релативне геометријске густине одабраних узорака. Приказани су најповољнији услови за добијање високотемпературног керамичког материјала на бази Ce, Sr фосфата.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "The influence of strontium content and sintering temperature on monazite stability",
volume = "56",
pages = "115-121",
doi = "10.2298/SOS220811024M"
}
Mirković, M., Maletaškić, J., Butulija, S., Anđelković, L.,& Šuljagić, M.. (2024). The influence of strontium content and sintering temperature on monazite stability. in Science of Sintering
Association for ETRAN Society., 56, 115-121.
https://doi.org/10.2298/SOS220811024M
Mirković M, Maletaškić J, Butulija S, Anđelković L, Šuljagić M. The influence of strontium content and sintering temperature on monazite stability. in Science of Sintering. 2024;56:115-121.
doi:10.2298/SOS220811024M .
Mirković, Miljana, Maletaškić, Jelena, Butulija, Svetlana, Anđelković, Ljubica, Šuljagić, Marija, "The influence of strontium content and sintering temperature on monazite stability" in Science of Sintering, 56 (2024):115-121,
https://doi.org/10.2298/SOS220811024M . .

BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties

Šuljagić, Marija; Petronijević, Ivan; Mirković, Miljana; Kremenović, Aleksandar; Džunuzović, Adis; Pavlović, Vladimir B.; Kalezić-Glišović, Aleksandra; Anđelković, Ljubica

(MDPI, 2023)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Petronijević, Ivan
AU  - Mirković, Miljana
AU  - Kremenović, Aleksandar
AU  - Džunuzović, Adis
AU  - Pavlović, Vladimir B.
AU  - Kalezić-Glišović, Aleksandra
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5865
AB  - To investigate the influence of spinel structure and sintering temperature on the functional properties of BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface from acetylacetonate precursors. As-prepared powders were additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the detailed examination of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were investigated. The optimal phase composition in the BaTiO3/NiFe2O4 composite, sintered at 1150 °C, resulted in a wide frequency range stability. Additionally, particular phase composition indicates favorable properties such as low conductivity and ideal-like hysteresis loop behavior. The favorable properties of BaTiO3/NiFe2O4 make this particular composite an ideal material choice for further studies on applications of multi-ferroic devices.
PB  - MDPI
T2  - Inorganics
T1  - BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties
VL  - 11
IS  - 2
SP  - 51
DO  - 10.3390/inorganics11020051
ER  - 
@article{
author = "Šuljagić, Marija and Petronijević, Ivan and Mirković, Miljana and Kremenović, Aleksandar and Džunuzović, Adis and Pavlović, Vladimir B. and Kalezić-Glišović, Aleksandra and Anđelković, Ljubica",
year = "2023",
abstract = "To investigate the influence of spinel structure and sintering temperature on the functional properties of BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface from acetylacetonate precursors. As-prepared powders were additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the detailed examination of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were investigated. The optimal phase composition in the BaTiO3/NiFe2O4 composite, sintered at 1150 °C, resulted in a wide frequency range stability. Additionally, particular phase composition indicates favorable properties such as low conductivity and ideal-like hysteresis loop behavior. The favorable properties of BaTiO3/NiFe2O4 make this particular composite an ideal material choice for further studies on applications of multi-ferroic devices.",
publisher = "MDPI",
journal = "Inorganics",
title = "BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties",
volume = "11",
number = "2",
pages = "51",
doi = "10.3390/inorganics11020051"
}
Šuljagić, M., Petronijević, I., Mirković, M., Kremenović, A., Džunuzović, A., Pavlović, V. B., Kalezić-Glišović, A.,& Anđelković, L.. (2023). BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties. in Inorganics
MDPI., 11(2), 51.
https://doi.org/10.3390/inorganics11020051
Šuljagić M, Petronijević I, Mirković M, Kremenović A, Džunuzović A, Pavlović VB, Kalezić-Glišović A, Anđelković L. BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties. in Inorganics. 2023;11(2):51.
doi:10.3390/inorganics11020051 .
Šuljagić, Marija, Petronijević, Ivan, Mirković, Miljana, Kremenović, Aleksandar, Džunuzović, Adis, Pavlović, Vladimir B., Kalezić-Glišović, Aleksandra, Anđelković, Ljubica, "BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1) Composites Synthesized by Thermal Decomposition: Magnetic, Dielectric and Ferroelectric Properties" in Inorganics, 11, no. 2 (2023):51,
https://doi.org/10.3390/inorganics11020051 . .
2
2

BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties

Šuljagić, Marija; Petronijević, Ivan; Mirković, Miljana; Kremenović, Aleksandar; Džunuzović, Adis; Pavlović, Vladimir; Kalezić-Glišović, Aleksandra; Anđelković, Ljubica

(Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo, 2023)

TY  - CONF
AU  - Šuljagić, Marija
AU  - Petronijević, Ivan
AU  - Mirković, Miljana
AU  - Kremenović, Aleksandar
AU  - Džunuzović, Adis
AU  - Pavlović, Vladimir
AU  - Kalezić-Glišović, Aleksandra
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6328
AB  - In order to examine the influence of phase composition and sintering temperature on the functional properties of perovskite/spinel composites, BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The obtained powders were compressed to pellets and sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive investigation of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C, which resulted in a wide frequency range stability. Furthermore, particular phase composition led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior [1]. These functional properties of BaTiO3/NiFe2O4 make this composite a “material of choice“ for further studies on applications of multiferroic devices.
AB  - U cilju ispitivanja uticaja faznog sastava i temperature sinterovanja na funkcionalna svojstva perovskit/spinel kompozita BaTiO3/NixZn1−xFe2O4 (x = 0, 0,5, 1), NiFe2O4, ZnFe2O4, i Ni0,5Zn0,5Fe2O4 pripremljeni su in situ metodom termalne dekompozicije. U sintezi su korišćeni acetilacetonatni kompleksi kao prekursori. Dobijeni prahovi su komprimovani u tablete i sinterovani na 1150 °C i 1300 °C. Za detaljno ispitivanje faznog sastava i morfologije sintetisanih kompozita korišćene su metode rendgenske difrakcije praha (XRPD) i skenirajuće elektronske mikroskopije (SEM) spregnute sa energetsko disperzivnom spektroskopijom (EDS). Ispitivana su i magnetna, dielektrična i feroelektrična svojstva sinterovanih kompozita. Ustanovljeno je da optimalni fazni sastav pronađen kod kompozita BaTiO3/NiFe2O4 sinterovanog na 1150 °C dovodi do stabilnosti u širokom opsegu frekvencija. Optimalni fazni sastav pomenutog kompozita povoljno je uticao na funkcionalna svojstva kao što su niska provodnost i feroelektrično ponašenje koje se ogleda u zadovoljavajućem izgledu histerezisa [1]. Ova svojstva nedvosmisleno ukazuju da je kompozit BaTiO3/NiFe2O4 odgovarajući izbor za dalja istraživanja posvećena primeni multiferoičnih materijala.
PB  - Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo
C3  - 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija
T1  - BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties
T1  - Uticaj faznog sastava i temperature sinterovanja na fizička svojstva BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) kompozita sintetisanih metodom termalne dekompozicije
SP  - 36
EP  - 37
UR  - https://hdl.handle.net/21.15107/rcub_cer_6328
ER  - 
@conference{
author = "Šuljagić, Marija and Petronijević, Ivan and Mirković, Miljana and Kremenović, Aleksandar and Džunuzović, Adis and Pavlović, Vladimir and Kalezić-Glišović, Aleksandra and Anđelković, Ljubica",
year = "2023",
abstract = "In order to examine the influence of phase composition and sintering temperature on the functional properties of perovskite/spinel composites, BaTiO3/NixZn1−xFe2O4 (x = 0, 0.5, 1), NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The obtained powders were compressed to pellets and sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive investigation of phase composition and morphology. The magnetic, dielectric, and ferroelectric properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C, which resulted in a wide frequency range stability. Furthermore, particular phase composition led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior [1]. These functional properties of BaTiO3/NiFe2O4 make this composite a “material of choice“ for further studies on applications of multiferroic devices., U cilju ispitivanja uticaja faznog sastava i temperature sinterovanja na funkcionalna svojstva perovskit/spinel kompozita BaTiO3/NixZn1−xFe2O4 (x = 0, 0,5, 1), NiFe2O4, ZnFe2O4, i Ni0,5Zn0,5Fe2O4 pripremljeni su in situ metodom termalne dekompozicije. U sintezi su korišćeni acetilacetonatni kompleksi kao prekursori. Dobijeni prahovi su komprimovani u tablete i sinterovani na 1150 °C i 1300 °C. Za detaljno ispitivanje faznog sastava i morfologije sintetisanih kompozita korišćene su metode rendgenske difrakcije praha (XRPD) i skenirajuće elektronske mikroskopije (SEM) spregnute sa energetsko disperzivnom spektroskopijom (EDS). Ispitivana su i magnetna, dielektrična i feroelektrična svojstva sinterovanih kompozita. Ustanovljeno je da optimalni fazni sastav pronađen kod kompozita BaTiO3/NiFe2O4 sinterovanog na 1150 °C dovodi do stabilnosti u širokom opsegu frekvencija. Optimalni fazni sastav pomenutog kompozita povoljno je uticao na funkcionalna svojstva kao što su niska provodnost i feroelektrično ponašenje koje se ogleda u zadovoljavajućem izgledu histerezisa [1]. Ova svojstva nedvosmisleno ukazuju da je kompozit BaTiO3/NiFe2O4 odgovarajući izbor za dalja istraživanja posvećena primeni multiferoičnih materijala.",
publisher = "Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo",
journal = "28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija",
title = "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties, Uticaj faznog sastava i temperature sinterovanja na fizička svojstva BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) kompozita sintetisanih metodom termalne dekompozicije",
pages = "36-37",
url = "https://hdl.handle.net/21.15107/rcub_cer_6328"
}
Šuljagić, M., Petronijević, I., Mirković, M., Kremenović, A., Džunuzović, A., Pavlović, V., Kalezić-Glišović, A.,& Anđelković, L.. (2023). BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties. in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija
Belgrade, Serbia : Serbian Cristallographic Soceity / Beograd, Srbija : Srpsko kristalografsko društvo., 36-37.
https://hdl.handle.net/21.15107/rcub_cer_6328
Šuljagić M, Petronijević I, Mirković M, Kremenović A, Džunuzović A, Pavlović V, Kalezić-Glišović A, Anđelković L. BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties. in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija. 2023;:36-37.
https://hdl.handle.net/21.15107/rcub_cer_6328 .
Šuljagić, Marija, Petronijević, Ivan, Mirković, Miljana, Kremenović, Aleksandar, Džunuzović, Adis, Pavlović, Vladimir, Kalezić-Glišović, Aleksandra, Anđelković, Ljubica, "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition and sintering temperature on their physical properties" in 28th Conference of the Serbian Crystallographic Society - Abstracts, June 14–15th, 2023 Čačak, Serbia / XXVIII Konferencija Srpskog kristalografskog društva - Izvodi radova, Jun 14–15, 2023 Čačak, Srbija (2023):36-37,
https://hdl.handle.net/21.15107/rcub_cer_6328 .

Understanding the Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite Composites

Šuljagić, Marija; Kremenović, Aleksandar; Petronijević, Ivan; Džunuzović, Adis; Mirković, Miljana; Pavlović, Vladimir; Anđelković, Ljubica

(Association for ETRAN Society, 2023)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Kremenović, Aleksandar
AU  - Petronijević, Ivan
AU  - Džunuzović, Adis
AU  - Mirković, Miljana
AU  - Pavlović, Vladimir
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6643
AB  - To investigate the effect of synthesis procedure and sintering temperature on the functional properties of perovskite/spinel ceramics, BaTiO3/CoFe2O4 composites were prepared by thermal decomposition, coprecipitation, and microemulsion method, and sintered at 1150°C and 1300°C. The phase composition and morphology of as-prepared powders as well as sintered ceramics were thoroughly examined by X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS). The dielectric and ferroelectric measurements were performed in detail. Generally, the samples sintered at 1300°C had better performances than those sintered at 1150°C. The composite synthesized by thermal decomposition and sintered at 1300 °C stands out among other prepared BaTiO3/CoFe2O4 ceramics, owing to high stability in the wide frequency range and low leakage currents. The obtained results indicate that such composite might be successfully applied as a functional multiferroic.
AB  - У циљу испитивања утицаја методе синтезе као и температуре синтеровања на функционална својства керамике перовскитно/спинелне структуре, синтетисани су BaTiO3/CoFe2O4 композити методама термалне декомпозиције, копреципитације и микроемулзије, а затим синтеровани на 1150 °C и 1300 °C. Фазни састав и морфологија синтетисаних узорака детаљно су испитани пре и после синтеровања помоћу рендгенске дифракције на праху (XRPD) и скенирајуће електронске микроскпије (SEM) спрегнуте са елекрон дисперзивном спектроскопијом (EDS). Изведена су опсежна испитивања како диелектричних, тако и фероелектричних својстава датих композита. У већини случајева узорци синтеровани на 1300 °C показали су боља својства од узорака синтерованих на 1150 °C. Композит синтетисан методом термалне декомпозиције и синтерован на 1300 °C издваја се од осталих синтетисаних BaTiO3/CoFe2O4 узорака захваљујући великој стабилносту у широком фреквентном опсегу и малим струјама цурења. Добијени резултати недвосмислено указују да истакнути композит може бити успешно примењен као функционални мултифероик.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites
VL  - 55
SP  - 367
EP  - 381
DO  - 10.2298/SOS220512013S
ER  - 
@article{
author = "Šuljagić, Marija and Kremenović, Aleksandar and Petronijević, Ivan and Džunuzović, Adis and Mirković, Miljana and Pavlović, Vladimir and Anđelković, Ljubica",
year = "2023",
abstract = "To investigate the effect of synthesis procedure and sintering temperature on the functional properties of perovskite/spinel ceramics, BaTiO3/CoFe2O4 composites were prepared by thermal decomposition, coprecipitation, and microemulsion method, and sintered at 1150°C and 1300°C. The phase composition and morphology of as-prepared powders as well as sintered ceramics were thoroughly examined by X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS). The dielectric and ferroelectric measurements were performed in detail. Generally, the samples sintered at 1300°C had better performances than those sintered at 1150°C. The composite synthesized by thermal decomposition and sintered at 1300 °C stands out among other prepared BaTiO3/CoFe2O4 ceramics, owing to high stability in the wide frequency range and low leakage currents. The obtained results indicate that such composite might be successfully applied as a functional multiferroic., У циљу испитивања утицаја методе синтезе као и температуре синтеровања на функционална својства керамике перовскитно/спинелне структуре, синтетисани су BaTiO3/CoFe2O4 композити методама термалне декомпозиције, копреципитације и микроемулзије, а затим синтеровани на 1150 °C и 1300 °C. Фазни састав и морфологија синтетисаних узорака детаљно су испитани пре и после синтеровања помоћу рендгенске дифракције на праху (XRPD) и скенирајуће електронске микроскпије (SEM) спрегнуте са елекрон дисперзивном спектроскопијом (EDS). Изведена су опсежна испитивања како диелектричних, тако и фероелектричних својстава датих композита. У већини случајева узорци синтеровани на 1300 °C показали су боља својства од узорака синтерованих на 1150 °C. Композит синтетисан методом термалне декомпозиције и синтерован на 1300 °C издваја се од осталих синтетисаних BaTiO3/CoFe2O4 узорака захваљујући великој стабилносту у широком фреквентном опсегу и малим струјама цурења. Добијени резултати недвосмислено указују да истакнути композит може бити успешно примењен као функционални мултифероик.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites",
volume = "55",
pages = "367-381",
doi = "10.2298/SOS220512013S"
}
Šuljagić, M., Kremenović, A., Petronijević, I., Džunuzović, A., Mirković, M., Pavlović, V.,& Anđelković, L.. (2023). Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites. in Science of Sintering
Association for ETRAN Society., 55, 367-381.
https://doi.org/10.2298/SOS220512013S
Šuljagić M, Kremenović A, Petronijević I, Džunuzović A, Mirković M, Pavlović V, Anđelković L. Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites. in Science of Sintering. 2023;55:367-381.
doi:10.2298/SOS220512013S .
Šuljagić, Marija, Kremenović, Aleksandar, Petronijević, Ivan, Džunuzović, Adis, Mirković, Miljana, Pavlović, Vladimir, Anđelković, Ljubica, "Understanding the  Effect of Synthesis and Sintering Temperature on the Functional Properties of Barium Titanate/ Cobalt Ferrite  Composites" in Science of Sintering, 55 (2023):367-381,
https://doi.org/10.2298/SOS220512013S . .

Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties

Mirković, Miljana; Sknepnek, Aleksandra; Miletić, Dunja; Pavlović, Vladimir; Đukić, Dunja; Šuljagić, Marija; Anđelković, Ljubica

(Faculty of Technology, University of Novi Sad, Bul. cara Lazara 1, 21000 Novi Sad, Serbia, 2023)

TY  - CONF
AU  - Mirković, Miljana
AU  - Sknepnek, Aleksandra
AU  - Miletić, Dunja
AU  - Pavlović, Vladimir
AU  - Đukić, Dunja
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6783
AB  - Hydroxyapatite Ca10(PO4)6(OH)2 - HAp presents natural construction material for bones and teeth and therefore is considered biocompatible, and has various applications in fields such as biomedicine, drug delivery, and as a biomarker. Considering nanoceramics' high specific surface area and antimicrobial activity, they can be used as potential antimicrobial materials. Bacterial cellulose (BC) is a biopolymer that stands out in its biodegradability, biocompatibility, and high water retention capacity, but also lacks functional properties. The main goal of this study is to create a newly designed composite material with the functionalization of cellulose by hydroxyapatite with antimicrobial properties. Hydroxyapatite material was incorporated in wet cellulose during the precipitation synthesis reaction. Obtained BC-HAp material was structurally and phase investigated by the XRD method. The morphology of obtained material was done by SEM, and appropriate functional groups were determined by the FTIR method. According to antimicrobial results investigated composite is shown proper antimicrobial activity.
PB  - Faculty of Technology, University of Novi Sad, Bul. cara Lazara 1, 21000 Novi Sad, Serbia
C3  - Programme and book of abstracts / 15th ECerS Conference for Young Scientists in Ceramics, October 11-14, 2023, Novi Sad
T1  - Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties
SP  - 70
EP  - 70
UR  - https://hdl.handle.net/21.15107/rcub_cer_6783
ER  - 
@conference{
author = "Mirković, Miljana and Sknepnek, Aleksandra and Miletić, Dunja and Pavlović, Vladimir and Đukić, Dunja and Šuljagić, Marija and Anđelković, Ljubica",
year = "2023",
abstract = "Hydroxyapatite Ca10(PO4)6(OH)2 - HAp presents natural construction material for bones and teeth and therefore is considered biocompatible, and has various applications in fields such as biomedicine, drug delivery, and as a biomarker. Considering nanoceramics' high specific surface area and antimicrobial activity, they can be used as potential antimicrobial materials. Bacterial cellulose (BC) is a biopolymer that stands out in its biodegradability, biocompatibility, and high water retention capacity, but also lacks functional properties. The main goal of this study is to create a newly designed composite material with the functionalization of cellulose by hydroxyapatite with antimicrobial properties. Hydroxyapatite material was incorporated in wet cellulose during the precipitation synthesis reaction. Obtained BC-HAp material was structurally and phase investigated by the XRD method. The morphology of obtained material was done by SEM, and appropriate functional groups were determined by the FTIR method. According to antimicrobial results investigated composite is shown proper antimicrobial activity.",
publisher = "Faculty of Technology, University of Novi Sad, Bul. cara Lazara 1, 21000 Novi Sad, Serbia",
journal = "Programme and book of abstracts / 15th ECerS Conference for Young Scientists in Ceramics, October 11-14, 2023, Novi Sad",
title = "Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties",
pages = "70-70",
url = "https://hdl.handle.net/21.15107/rcub_cer_6783"
}
Mirković, M., Sknepnek, A., Miletić, D., Pavlović, V., Đukić, D., Šuljagić, M.,& Anđelković, L.. (2023). Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties. in Programme and book of abstracts / 15th ECerS Conference for Young Scientists in Ceramics, October 11-14, 2023, Novi Sad
Faculty of Technology, University of Novi Sad, Bul. cara Lazara 1, 21000 Novi Sad, Serbia., 70-70.
https://hdl.handle.net/21.15107/rcub_cer_6783
Mirković M, Sknepnek A, Miletić D, Pavlović V, Đukić D, Šuljagić M, Anđelković L. Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties. in Programme and book of abstracts / 15th ECerS Conference for Young Scientists in Ceramics, October 11-14, 2023, Novi Sad. 2023;:70-70.
https://hdl.handle.net/21.15107/rcub_cer_6783 .
Mirković, Miljana, Sknepnek, Aleksandra, Miletić, Dunja, Pavlović, Vladimir, Đukić, Dunja, Šuljagić, Marija, Anđelković, Ljubica, "Synthesis and characterization of cellulose-hydroxyapatite composite material with proper antimicrobial properties" in Programme and book of abstracts / 15th ECerS Conference for Young Scientists in Ceramics, October 11-14, 2023, Novi Sad (2023):70-70,
https://hdl.handle.net/21.15107/rcub_cer_6783 .

Hybrid Nanoscale Materials for Convergent Technologies

Pavlović, Vladimir B.; Vuković, G.; Nikolić, M.; Pavlović, Vera P.; Perić, M.; Nenadović, S.; Ivanović, M.; Mirković, M.; Đoković, V.; Knežević, S.; Šuljagić, Marija; Anđelković, Ljubica; Janićijević, Aleksandra; Kovačević, D.; Filipović, Suzana; Vujančević, Jelena; Vlahović, Branislav

(Belgrade : Serbian Ceramic Society, 2023)

TY  - CONF
AU  - Pavlović, Vladimir B.
AU  - Vuković, G.
AU  - Nikolić, M.
AU  - Pavlović, Vera P.
AU  - Perić, M.
AU  - Nenadović, S.
AU  - Ivanović, M.
AU  - Mirković, M.
AU  - Đoković, V.
AU  - Knežević, S.
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
AU  - Janićijević, Aleksandra
AU  - Kovačević, D.
AU  - Filipović, Suzana
AU  - Vujančević, Jelena
AU  - Vlahović, Branislav
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7363
AB  - The convergence of nano-, bio-, and information technologies is based on the understanding of complex hierarchical structures and systems, as well as on the material unity at the nanoscale and on technology integration from that scale. A growing interest in these technologies is a result of their potential to provide solutions to numerous societal challenges, such as advanced healthcare, environmental remediation, sustainable development, and adoption of cyber-physical systems based on the Internet of Things and the Internet of Systems. Taking into account that hybrid nanomaterials possess extraordinary physical and chemical properties derived from their size in the nanoscale, the aim of this work is to present the connection between processing parameters and multifunctional properties of nano scale hybrid materials, focusing on the study of ceramic-polymer structures before they can be nano-engineered into functional devices. The unique functionality of these nanostructures has enabled their applications in numerous devices such as: micro and nano-electro-mechanical systems (MEMS/NEMS), sensors, microactuators, surface acoustic wave devices, polymer electrolyte membrane fuel cells, switches, thermistors, resonators and filters, electrooptic devices, etc. In this study special attention has been paid to their applications in the fields of electronics, biotechnology, environmental protection and remediation.
PB  - Belgrade : Serbian Ceramic Society
C3  - Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application XI New Frontiers in Multifunctional Material Science and Processing, Serbian Academy of Sciences and Art Serbia, Belgrade,18-20.September 2023
T1  - Hybrid Nanoscale Materials for Convergent Technologies
SP  - 45
EP  - 45
UR  - https://hdl.handle.net/21.15107/rcub_cer_7363
ER  - 
@conference{
author = "Pavlović, Vladimir B. and Vuković, G. and Nikolić, M. and Pavlović, Vera P. and Perić, M. and Nenadović, S. and Ivanović, M. and Mirković, M. and Đoković, V. and Knežević, S. and Šuljagić, Marija and Anđelković, Ljubica and Janićijević, Aleksandra and Kovačević, D. and Filipović, Suzana and Vujančević, Jelena and Vlahović, Branislav",
year = "2023",
abstract = "The convergence of nano-, bio-, and information technologies is based on the understanding of complex hierarchical structures and systems, as well as on the material unity at the nanoscale and on technology integration from that scale. A growing interest in these technologies is a result of their potential to provide solutions to numerous societal challenges, such as advanced healthcare, environmental remediation, sustainable development, and adoption of cyber-physical systems based on the Internet of Things and the Internet of Systems. Taking into account that hybrid nanomaterials possess extraordinary physical and chemical properties derived from their size in the nanoscale, the aim of this work is to present the connection between processing parameters and multifunctional properties of nano scale hybrid materials, focusing on the study of ceramic-polymer structures before they can be nano-engineered into functional devices. The unique functionality of these nanostructures has enabled their applications in numerous devices such as: micro and nano-electro-mechanical systems (MEMS/NEMS), sensors, microactuators, surface acoustic wave devices, polymer electrolyte membrane fuel cells, switches, thermistors, resonators and filters, electrooptic devices, etc. In this study special attention has been paid to their applications in the fields of electronics, biotechnology, environmental protection and remediation.",
publisher = "Belgrade : Serbian Ceramic Society",
journal = "Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application XI New Frontiers in Multifunctional Material Science and Processing, Serbian Academy of Sciences and Art Serbia, Belgrade,18-20.September 2023",
title = "Hybrid Nanoscale Materials for Convergent Technologies",
pages = "45-45",
url = "https://hdl.handle.net/21.15107/rcub_cer_7363"
}
Pavlović, V. B., Vuković, G., Nikolić, M., Pavlović, V. P., Perić, M., Nenadović, S., Ivanović, M., Mirković, M., Đoković, V., Knežević, S., Šuljagić, M., Anđelković, L., Janićijević, A., Kovačević, D., Filipović, S., Vujančević, J.,& Vlahović, B.. (2023). Hybrid Nanoscale Materials for Convergent Technologies. in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application XI New Frontiers in Multifunctional Material Science and Processing, Serbian Academy of Sciences and Art Serbia, Belgrade,18-20.September 2023
Belgrade : Serbian Ceramic Society., 45-45.
https://hdl.handle.net/21.15107/rcub_cer_7363
Pavlović VB, Vuković G, Nikolić M, Pavlović VP, Perić M, Nenadović S, Ivanović M, Mirković M, Đoković V, Knežević S, Šuljagić M, Anđelković L, Janićijević A, Kovačević D, Filipović S, Vujančević J, Vlahović B. Hybrid Nanoscale Materials for Convergent Technologies. in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application XI New Frontiers in Multifunctional Material Science and Processing, Serbian Academy of Sciences and Art Serbia, Belgrade,18-20.September 2023. 2023;:45-45.
https://hdl.handle.net/21.15107/rcub_cer_7363 .
Pavlović, Vladimir B., Vuković, G., Nikolić, M., Pavlović, Vera P., Perić, M., Nenadović, S., Ivanović, M., Mirković, M., Đoković, V., Knežević, S., Šuljagić, Marija, Anđelković, Ljubica, Janićijević, Aleksandra, Kovačević, D., Filipović, Suzana, Vujančević, Jelena, Vlahović, Branislav, "Hybrid Nanoscale Materials for Convergent Technologies" in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application XI New Frontiers in Multifunctional Material Science and Processing, Serbian Academy of Sciences and Art Serbia, Belgrade,18-20.September 2023 (2023):45-45,
https://hdl.handle.net/21.15107/rcub_cer_7363 .

Lead Free Polymer Composites for Radiation Shielding

Perić, Marko; Vuković, George; Knežević, Sanja; Nikolić, Milan; Šuljagić, Marija; Anđelković, Ljubica; Nenadović, Snežana; Ivanović, Marija; Mirković, Miljana; Pavlović, Vladmir B.

(Bucharest: SRMNIM, 2023)

TY  - CONF
AU  - Perić, Marko
AU  - Vuković, George
AU  - Knežević, Sanja
AU  - Nikolić, Milan
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
AU  - Nenadović, Snežana
AU  - Ivanović, Marija
AU  - Mirković, Miljana
AU  - Pavlović, Vladmir B.
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6022
AB  - Radiation shielding is a crucial precautionary measure in decreasing the dose of exposure medical personnel experience. The physical dimensions of these shields, specifically thickness and shape, are dependent on the type of radiation, energy and specific radioactivity. Currently, the most common radiation shielding equipment is made of lead, tungsten or uranium. Although these heavy metals have favorable shielding properties against ionizing radiation, protective garments such as lead aprons are heavy to wear and can pose significant health risks. Taking this into account, the primary goal of this study is to understand the radiation shielding properties of lead-free polymer geopolymer-polyurethane based composites. The geopolymer was synthesized using an 80%-20% mixture of fly ash and a bio-polyol substrate which was subsequently homogenized using MDI44. As a result, 6 samples of the geopolymer-polyurethane based composites were fabricated of which 5 were 90%-10% compositions between the mixture and varying concentrations of BaSO4 and Bi2O3 respectively. The last sample consisted of the pure fly ash/bio-polyol mixture. XRF and ICP analysis was used to chemically characterize the fly ash. The composite structures were analyzed using XRD, while the microstructural morphology was investigated using SEM techniques. Utilizing an energy-dispersive x-ray spectrometer (EDS), elemental abundance and agglomerating behavior was analyzed for each composite variant. The X-ray attenuation measurements pointed out that the obtained composites have the potential for a design of lead-free protective clothing against X-ray shielding in medical applications.
PB  - Bucharest: SRMNIM
C3  - Abstracts E-Book, 10th Balkan Congress of Nuclear Medicine & 5th Romanian Congress of Nuclear Medicine, 15-18 March, 2023, Bucharest, Romania
T1  - Lead Free Polymer Composites for Radiation Shielding
SP  - 17
SP  - 17
UR  - https://hdl.handle.net/21.15107/rcub_cer_6022
ER  - 
@conference{
author = "Perić, Marko and Vuković, George and Knežević, Sanja and Nikolić, Milan and Šuljagić, Marija and Anđelković, Ljubica and Nenadović, Snežana and Ivanović, Marija and Mirković, Miljana and Pavlović, Vladmir B.",
year = "2023",
abstract = "Radiation shielding is a crucial precautionary measure in decreasing the dose of exposure medical personnel experience. The physical dimensions of these shields, specifically thickness and shape, are dependent on the type of radiation, energy and specific radioactivity. Currently, the most common radiation shielding equipment is made of lead, tungsten or uranium. Although these heavy metals have favorable shielding properties against ionizing radiation, protective garments such as lead aprons are heavy to wear and can pose significant health risks. Taking this into account, the primary goal of this study is to understand the radiation shielding properties of lead-free polymer geopolymer-polyurethane based composites. The geopolymer was synthesized using an 80%-20% mixture of fly ash and a bio-polyol substrate which was subsequently homogenized using MDI44. As a result, 6 samples of the geopolymer-polyurethane based composites were fabricated of which 5 were 90%-10% compositions between the mixture and varying concentrations of BaSO4 and Bi2O3 respectively. The last sample consisted of the pure fly ash/bio-polyol mixture. XRF and ICP analysis was used to chemically characterize the fly ash. The composite structures were analyzed using XRD, while the microstructural morphology was investigated using SEM techniques. Utilizing an energy-dispersive x-ray spectrometer (EDS), elemental abundance and agglomerating behavior was analyzed for each composite variant. The X-ray attenuation measurements pointed out that the obtained composites have the potential for a design of lead-free protective clothing against X-ray shielding in medical applications.",
publisher = "Bucharest: SRMNIM",
journal = "Abstracts E-Book, 10th Balkan Congress of Nuclear Medicine & 5th Romanian Congress of Nuclear Medicine, 15-18 March, 2023, Bucharest, Romania",
title = "Lead Free Polymer Composites for Radiation Shielding",
pages = "17-17",
url = "https://hdl.handle.net/21.15107/rcub_cer_6022"
}
Perić, M., Vuković, G., Knežević, S., Nikolić, M., Šuljagić, M., Anđelković, L., Nenadović, S., Ivanović, M., Mirković, M.,& Pavlović, V. B.. (2023). Lead Free Polymer Composites for Radiation Shielding. in Abstracts E-Book, 10th Balkan Congress of Nuclear Medicine & 5th Romanian Congress of Nuclear Medicine, 15-18 March, 2023, Bucharest, Romania
Bucharest: SRMNIM., 17.
https://hdl.handle.net/21.15107/rcub_cer_6022
Perić M, Vuković G, Knežević S, Nikolić M, Šuljagić M, Anđelković L, Nenadović S, Ivanović M, Mirković M, Pavlović VB. Lead Free Polymer Composites for Radiation Shielding. in Abstracts E-Book, 10th Balkan Congress of Nuclear Medicine & 5th Romanian Congress of Nuclear Medicine, 15-18 March, 2023, Bucharest, Romania. 2023;:17.
https://hdl.handle.net/21.15107/rcub_cer_6022 .
Perić, Marko, Vuković, George, Knežević, Sanja, Nikolić, Milan, Šuljagić, Marija, Anđelković, Ljubica, Nenadović, Snežana, Ivanović, Marija, Mirković, Miljana, Pavlović, Vladmir B., "Lead Free Polymer Composites for Radiation Shielding" in Abstracts E-Book, 10th Balkan Congress of Nuclear Medicine & 5th Romanian Congress of Nuclear Medicine, 15-18 March, 2023, Bucharest, Romania (2023):17,
https://hdl.handle.net/21.15107/rcub_cer_6022 .

Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study

Lazarević, Zorica; Anđelković, Ljubica; Šuljagić, Marija; Milutinović, Aleksandra; Ćurčić, Milica; Trajić, Jelena; Paunović, Novica; Romčević, Maja; Hadžić, Branka; Romčević, Nebojša

(INOE, Romania, 2023)

TY  - JOUR
AU  - Lazarević, Zorica
AU  - Anđelković, Ljubica
AU  - Šuljagić, Marija
AU  - Milutinović, Aleksandra
AU  - Ćurčić, Milica
AU  - Trajić, Jelena
AU  - Paunović, Novica
AU  - Romčević, Maja
AU  - Hadžić, Branka
AU  - Romčević, Nebojša
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6231
AB  - Nanocrystalline CoFe2O4 has been synthesized by various synthesis methods. The obtained monodomain nanoparticles are similar in sizes (15.8-19 nm), but with different internal stresses, size distributions and cation inversion coefficients (0.51 - 0.90) due to different synthesis routes. The structure and cation distribution are investigated by XRD diffraction analysis, Raman and FIR spectroscopy. Measurement of magnetization, i.e. coercivity, enable the calculation of the anisotropy coefficient K1 = (3.6-5.12)·105 J cm-3, which is very high in cobalt ferrite. The anisotropy coefficient directly depends on the nanoparticle size. It has been shown that magnetization linearly depends on the cation inversion, except in the sample with the largest nanoparticles (19 nm), where the more regular crystal structure prevails and higher values of magnetization were obtained. The average magnetic moments at 300 K are: μFe = 3.6μB and μCo = 2.5μB. It is obvious that with small adjustments in the synthesis, desirable nanoparticle properties can be obtained.
PB  - INOE, Romania
T2  - Optoelectronics and Advanced Materials – Rapid Communications
T1  - Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study
VL  - 17
IS  - 5-6
SP  - 247
EP  - 254
UR  - https://hdl.handle.net/21.15107/rcub_cer_6231
ER  - 
@article{
author = "Lazarević, Zorica and Anđelković, Ljubica and Šuljagić, Marija and Milutinović, Aleksandra and Ćurčić, Milica and Trajić, Jelena and Paunović, Novica and Romčević, Maja and Hadžić, Branka and Romčević, Nebojša",
year = "2023",
abstract = "Nanocrystalline CoFe2O4 has been synthesized by various synthesis methods. The obtained monodomain nanoparticles are similar in sizes (15.8-19 nm), but with different internal stresses, size distributions and cation inversion coefficients (0.51 - 0.90) due to different synthesis routes. The structure and cation distribution are investigated by XRD diffraction analysis, Raman and FIR spectroscopy. Measurement of magnetization, i.e. coercivity, enable the calculation of the anisotropy coefficient K1 = (3.6-5.12)·105 J cm-3, which is very high in cobalt ferrite. The anisotropy coefficient directly depends on the nanoparticle size. It has been shown that magnetization linearly depends on the cation inversion, except in the sample with the largest nanoparticles (19 nm), where the more regular crystal structure prevails and higher values of magnetization were obtained. The average magnetic moments at 300 K are: μFe = 3.6μB and μCo = 2.5μB. It is obvious that with small adjustments in the synthesis, desirable nanoparticle properties can be obtained.",
publisher = "INOE, Romania",
journal = "Optoelectronics and Advanced Materials – Rapid Communications",
title = "Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study",
volume = "17",
number = "5-6",
pages = "247-254",
url = "https://hdl.handle.net/21.15107/rcub_cer_6231"
}
Lazarević, Z., Anđelković, L., Šuljagić, M., Milutinović, A., Ćurčić, M., Trajić, J., Paunović, N., Romčević, M., Hadžić, B.,& Romčević, N.. (2023). Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study. in Optoelectronics and Advanced Materials – Rapid Communications
INOE, Romania., 17(5-6), 247-254.
https://hdl.handle.net/21.15107/rcub_cer_6231
Lazarević Z, Anđelković L, Šuljagić M, Milutinović A, Ćurčić M, Trajić J, Paunović N, Romčević M, Hadžić B, Romčević N. Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study. in Optoelectronics and Advanced Materials – Rapid Communications. 2023;17(5-6):247-254.
https://hdl.handle.net/21.15107/rcub_cer_6231 .
Lazarević, Zorica, Anđelković, Ljubica, Šuljagić, Marija, Milutinović, Aleksandra, Ćurčić, Milica, Trajić, Jelena, Paunović, Novica, Romčević, Maja, Hadžić, Branka, Romčević, Nebojša, "Vibrational and magnetic properties of nano-sized CoFe2O4 obtained by various synthesis techniques: a comparative study" in Optoelectronics and Advanced Materials – Rapid Communications, 17, no. 5-6 (2023):247-254,
https://hdl.handle.net/21.15107/rcub_cer_6231 .

Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels

Lazarević, Zorica; Milutinović, Aleksandra; Anđelković, Ljubica; Petrović, Milica; Hadžić, Branka; Romčević, Maja; Trajić, Jelena; Romčević, Nebojša

(Association for ETRAN Society, 2023)

TY  - JOUR
AU  - Lazarević, Zorica
AU  - Milutinović, Aleksandra
AU  - Anđelković, Ljubica
AU  - Petrović, Milica
AU  - Hadžić, Branka
AU  - Romčević, Maja
AU  - Trajić, Jelena
AU  - Romčević, Nebojša
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7212
AB  - ingle phase cobalt ferrite (CoFe2O4) with nanoparticles of similar sizes (15.7-19 nm) was obtained by different synthesis methods: coprecipitation, ultrasonically assisted coprecipitation, coprecipitation followed by mechanochemical treatment, microemulsion and microwave assisted hydrothermal synthesis. The obtained CoFe2O4 samples have been studied using a variety of characterization techniques: X-ray diffraction (XRD), Raman spectroscopy, far infrared (FIR) reflectivity and attenuated total reflectance (ATR) in combination with Fourier-transform infrared (FTIR) spectroscopy in mid IR spectra. Different methods of synthesis produced nanoparticles with different lattice constants, internal stresses and different cation inversion values. This is confirmed in the subtle changes in the Raman and IR spectra of different CoFe2O4 nano-powders. The Raman spectra of CoFe2O4 were compared with the spectra of other ferrites and some cubic oxide spinels in an attempt to evaluate the contribution of tetrahedral and octahedral oscillations in certain Raman modes.
AB  - Монофазни кобалт ферит са наночестицама сличних величина (15,7-19  нанометара) добијен је различитим методама синтезе: копреципитацијом,  ултразвучно потпомогнутом копреципитацијом, копреципитацијом праћеном  механохемијском синтезом, микроемулзијом и микроталасном хидротермалном  синтезом. Добијени узорци кобалт ферита су проучавани коришћењем различитих  техника карактеризације: дифракцијом рендгенских зрака на праху, Раман спектроскопијом, рефлексијом у далекој инфра-црвеној области (ИЦ) и методом  апсорпције при вишеструкој тоталној рефлексији у комбинацији са инфра-црвеном  спектроскопијом (АТР-ИЦ) у средњој инфра црвеној области. Различитим методама  синтезе добијене су наночестице са различитим константама решетке, унутрашњим  напрезањима и различитим вредностима инверзије катјона. Ово је потврђено у  суптилним променама у Раман и ИЦ спектрима различитих нано-прахова кобалт  ферита. Раман спектри кобалт ферита упоређени су са спектрима других ферита и  неких кубних оксидних спинела у покушају да се процени утицај удела  тетраедарских и октаедарских осцилација у одређеним Раман модовима.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels
T1  - Kарактеризација наночестица кобалт ферита добијених  различитим методама синтезе и поређење са Рамановим спектрима  других ферита и неких кубичних оксидних спинела
DO  - 10.2298/SOS230322035L
ER  - 
@article{
author = "Lazarević, Zorica and Milutinović, Aleksandra and Anđelković, Ljubica and Petrović, Milica and Hadžić, Branka and Romčević, Maja and Trajić, Jelena and Romčević, Nebojša",
year = "2023",
abstract = "ingle phase cobalt ferrite (CoFe2O4) with nanoparticles of similar sizes (15.7-19 nm) was obtained by different synthesis methods: coprecipitation, ultrasonically assisted coprecipitation, coprecipitation followed by mechanochemical treatment, microemulsion and microwave assisted hydrothermal synthesis. The obtained CoFe2O4 samples have been studied using a variety of characterization techniques: X-ray diffraction (XRD), Raman spectroscopy, far infrared (FIR) reflectivity and attenuated total reflectance (ATR) in combination with Fourier-transform infrared (FTIR) spectroscopy in mid IR spectra. Different methods of synthesis produced nanoparticles with different lattice constants, internal stresses and different cation inversion values. This is confirmed in the subtle changes in the Raman and IR spectra of different CoFe2O4 nano-powders. The Raman spectra of CoFe2O4 were compared with the spectra of other ferrites and some cubic oxide spinels in an attempt to evaluate the contribution of tetrahedral and octahedral oscillations in certain Raman modes., Монофазни кобалт ферит са наночестицама сличних величина (15,7-19  нанометара) добијен је различитим методама синтезе: копреципитацијом,  ултразвучно потпомогнутом копреципитацијом, копреципитацијом праћеном  механохемијском синтезом, микроемулзијом и микроталасном хидротермалном  синтезом. Добијени узорци кобалт ферита су проучавани коришћењем различитих  техника карактеризације: дифракцијом рендгенских зрака на праху, Раман спектроскопијом, рефлексијом у далекој инфра-црвеној области (ИЦ) и методом  апсорпције при вишеструкој тоталној рефлексији у комбинацији са инфра-црвеном  спектроскопијом (АТР-ИЦ) у средњој инфра црвеној области. Различитим методама  синтезе добијене су наночестице са различитим константама решетке, унутрашњим  напрезањима и различитим вредностима инверзије катјона. Ово је потврђено у  суптилним променама у Раман и ИЦ спектрима различитих нано-прахова кобалт  ферита. Раман спектри кобалт ферита упоређени су са спектрима других ферита и  неких кубних оксидних спинела у покушају да се процени утицај удела  тетраедарских и октаедарских осцилација у одређеним Раман модовима.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels, Kарактеризација наночестица кобалт ферита добијених  различитим методама синтезе и поређење са Рамановим спектрима  других ферита и неких кубичних оксидних спинела",
doi = "10.2298/SOS230322035L"
}
Lazarević, Z., Milutinović, A., Anđelković, L., Petrović, M., Hadžić, B., Romčević, M., Trajić, J.,& Romčević, N.. (2023). Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels. in Science of Sintering
Association for ETRAN Society..
https://doi.org/10.2298/SOS230322035L
Lazarević Z, Milutinović A, Anđelković L, Petrović M, Hadžić B, Romčević M, Trajić J, Romčević N. Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels. in Science of Sintering. 2023;.
doi:10.2298/SOS230322035L .
Lazarević, Zorica, Milutinović, Aleksandra, Anđelković, Ljubica, Petrović, Milica, Hadžić, Branka, Romčević, Maja, Trajić, Jelena, Romčević, Nebojša, "Characterization of cobalt ferrite nanoparticles obtained by various synthesis methods and comparison with the Raman spectra of other ferrites and some cubic oxide spinels" in Science of Sintering (2023),
https://doi.org/10.2298/SOS230322035L . .

BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties

Šuljagić, Marija; Anđelković, Ljubica

(Belgrade: Serbian Ceramic Society, 2023)

TY  - CONF
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6642
AB  - To examine the influence of phase composition on the magnetic, dielectric, and ferroelectric
properties of perovskite/spinel composites, NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in
situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The synthesized powders were compressed to pellets and additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive study of phase composition and morphology. The magnetic and electrical properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C. This resulted in wide frequency range stability of relative dielectric constant. Furthermore, optimal phase composition in BaTiO3/NiFe2O4 led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior. These functional properties of BaTiO3/NiFe2O4 make this composite a promising candidate for further studies on multiferroic properties.
PB  - Belgrade: Serbian Ceramic Society
C3  - Program and the Book of Abstracts, The Eleventh Serbian Ceramic Society Conference Advanced Ceramics and Application, September 18-20, 2023
T1  - BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties
SP  - 33
EP  - 33
UR  - https://hdl.handle.net/21.15107/rcub_cer_6642
ER  - 
@conference{
author = "Šuljagić, Marija and Anđelković, Ljubica",
year = "2023",
abstract = "To examine the influence of phase composition on the magnetic, dielectric, and ferroelectric
properties of perovskite/spinel composites, NiFe2O4, ZnFe2O4, and Ni0.5Zn0.5Fe2O4 were in
situ prepared by thermal decomposition onto BaTiO3 surface. Acetylacetonate complexes were used as the precursors. The synthesized powders were compressed to pellets and additionally sintered at 1150 °C and 1300 °C. X-ray powder diffraction (XRPD) and scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS) were used for the comprehensive study of phase composition and morphology. The magnetic and electrical properties were performed in detail. The optimal phase composition was found in the BaTiO3/NiFe2O4 composite sintered at 1150 °C. This resulted in wide frequency range stability of relative dielectric constant. Furthermore, optimal phase composition in BaTiO3/NiFe2O4 led to suitable properties such as low conductivity and ideal-like hysteresis loop behavior. These functional properties of BaTiO3/NiFe2O4 make this composite a promising candidate for further studies on multiferroic properties.",
publisher = "Belgrade: Serbian Ceramic Society",
journal = "Program and the Book of Abstracts, The Eleventh Serbian Ceramic Society Conference Advanced Ceramics and Application, September 18-20, 2023",
title = "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties",
pages = "33-33",
url = "https://hdl.handle.net/21.15107/rcub_cer_6642"
}
Šuljagić, M.,& Anđelković, L.. (2023). BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties. in Program and the Book of Abstracts, The Eleventh Serbian Ceramic Society Conference Advanced Ceramics and Application, September 18-20, 2023
Belgrade: Serbian Ceramic Society., 33-33.
https://hdl.handle.net/21.15107/rcub_cer_6642
Šuljagić M, Anđelković L. BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties. in Program and the Book of Abstracts, The Eleventh Serbian Ceramic Society Conference Advanced Ceramics and Application, September 18-20, 2023. 2023;:33-33.
https://hdl.handle.net/21.15107/rcub_cer_6642 .
Šuljagić, Marija, Anđelković, Ljubica, "BaTiO3/NixZn1-xFe2O4 (x =0, 0.5, 1) composites synthesized by thermal decomposition: The influence of phase composition on their magnetic and electrical properties" in Program and the Book of Abstracts, The Eleventh Serbian Ceramic Society Conference Advanced Ceramics and Application, September 18-20, 2023 (2023):33-33,
https://hdl.handle.net/21.15107/rcub_cer_6642 .

Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition

Šuljagić, Marija; Anđelković, Ljubica; Jeremić, Dejan

(Skopje: Society of the chemists and technologists of Macedonia, 2023)

TY  - CONF
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
AU  - Jeremić, Dejan
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6675
AB  - The cobalt oxide (Co3O4) is a very attractive material for optoelectronic applications due to the intense absorption of visible light and p-type semiconducting properties. On the other hand, conventional synthesis methods for its preparation could be either time- and energy-consuming or relying on toxic chemicals. To address this issue, spinel Co3O4 nanoparticles were prepared by a simple, facile, and eco-friendly method of synthesis. Such method is based on the thermal decomposition of hexaaquacobalt(II) D-camphor10-sulfonate at 900 °C. This synthesis route avoids the use of toxic organic solvents which overcomes the disadvantages of many combustion methods. In order to assess the potential use of synthesized powder, the characterization methods were performed in detail. The purity and semiconducting properties of the Co3O4 were confirmed by UV/Vis spectroscopy which indicated the presence of two band gaps (2.10 eV and 1.22 eV). A noteworthy improvement in the electron transfer kinetics with the addition of the prepared sample to the carbon-paste electrode led to an enhanced electrocatalytic performance. Such remarkable functional properties are suitable for a wide range of technological applications, open the way for the implementation of this preparation procedure for the synthesis of Co3O4 on a larger industrial scale.
PB  - Skopje: Society of the chemists and technologists of Macedonia
C3  - Book of abstracts, 26th Congress of the Society of Chemists and Technologists of Macedonia, September 20-23, 2023, Ohrid, Macedonia
T1  - Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition
SP  - 26
EP  - 26
UR  - https://hdl.handle.net/21.15107/rcub_cer_6675
ER  - 
@conference{
author = "Šuljagić, Marija and Anđelković, Ljubica and Jeremić, Dejan",
year = "2023",
abstract = "The cobalt oxide (Co3O4) is a very attractive material for optoelectronic applications due to the intense absorption of visible light and p-type semiconducting properties. On the other hand, conventional synthesis methods for its preparation could be either time- and energy-consuming or relying on toxic chemicals. To address this issue, spinel Co3O4 nanoparticles were prepared by a simple, facile, and eco-friendly method of synthesis. Such method is based on the thermal decomposition of hexaaquacobalt(II) D-camphor10-sulfonate at 900 °C. This synthesis route avoids the use of toxic organic solvents which overcomes the disadvantages of many combustion methods. In order to assess the potential use of synthesized powder, the characterization methods were performed in detail. The purity and semiconducting properties of the Co3O4 were confirmed by UV/Vis spectroscopy which indicated the presence of two band gaps (2.10 eV and 1.22 eV). A noteworthy improvement in the electron transfer kinetics with the addition of the prepared sample to the carbon-paste electrode led to an enhanced electrocatalytic performance. Such remarkable functional properties are suitable for a wide range of technological applications, open the way for the implementation of this preparation procedure for the synthesis of Co3O4 on a larger industrial scale.",
publisher = "Skopje: Society of the chemists and technologists of Macedonia",
journal = "Book of abstracts, 26th Congress of the Society of Chemists and Technologists of Macedonia, September 20-23, 2023, Ohrid, Macedonia",
title = "Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition",
pages = "26-26",
url = "https://hdl.handle.net/21.15107/rcub_cer_6675"
}
Šuljagić, M., Anđelković, L.,& Jeremić, D.. (2023). Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition. in Book of abstracts, 26th Congress of the Society of Chemists and Technologists of Macedonia, September 20-23, 2023, Ohrid, Macedonia
Skopje: Society of the chemists and technologists of Macedonia., 26-26.
https://hdl.handle.net/21.15107/rcub_cer_6675
Šuljagić M, Anđelković L, Jeremić D. Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition. in Book of abstracts, 26th Congress of the Society of Chemists and Technologists of Macedonia, September 20-23, 2023, Ohrid, Macedonia. 2023;:26-26.
https://hdl.handle.net/21.15107/rcub_cer_6675 .
Šuljagić, Marija, Anđelković, Ljubica, Jeremić, Dejan, "Semiconducting Co3O4 Nanocatalyst Prepared by Eco-Friendly Thermal Decomposition" in Book of abstracts, 26th Congress of the Society of Chemists and Technologists of Macedonia, September 20-23, 2023, Ohrid, Macedonia (2023):26-26,
https://hdl.handle.net/21.15107/rcub_cer_6675 .

Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions

Petronijević, Ivan; Dudić, Duško; Cerović, Dragana; Maletić, Slavica; Marinković, Filip; Pergal, Marija; Anđelković, Ljubica

(Wiley, 2023)

TY  - JOUR
AU  - Petronijević, Ivan
AU  - Dudić, Duško
AU  - Cerović, Dragana
AU  - Maletić, Slavica
AU  - Marinković, Filip
AU  - Pergal, Marija
AU  - Anđelković, Ljubica
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6198
AB  - The dielectric properties of nanocomposites based on isotactic polypropylene (iPP) and atactic polystyrene (aPS) obtained by novel, simple, and environmentally friendly treatment technique have been analyzed in this study. The best treatment conditions to obtain nanocomposites with embedded core-shell particles with enhanced dielectric properties were considered. Treatment of polymer matrices in water solution iron(II)-chloride had the most pronounced precipitation effect, that was directly related to the appearance of higher transition metal concentrations in the iPP and aPS matrices, in comparison to treatments in the other two transition metal salts, MnCl2 and NiCl2. Relative dielectric constant and loss tangent have been studied in the frequency range from 20 Hz to 9 MHz. Embedded core-shell nanoparticles (from 15 to 150 nm in diameter) in a very small amount (1.72E-8 mol/cm3 to 1.17E-5 mol/cm3) resulted in significant improvement (2.5% up to 9.1%) and stabilization of relative dielectric constant value toward higher frequencies and also lowering loss tangent in compare to starting polymer matrices. These properties indicate that materials obtained with the presented treatment technique can be applied as microelectronic packing and with further development of the method in order to obtain a higher concentration of metal ions as energy storage devices.
PB  - Wiley
T2  - Polymers for Advanced Technologies
T1  - Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions
SP  - 1
EP  - 10
DO  - 10.1002/pat.6110
ER  - 
@article{
author = "Petronijević, Ivan and Dudić, Duško and Cerović, Dragana and Maletić, Slavica and Marinković, Filip and Pergal, Marija and Anđelković, Ljubica",
year = "2023",
abstract = "The dielectric properties of nanocomposites based on isotactic polypropylene (iPP) and atactic polystyrene (aPS) obtained by novel, simple, and environmentally friendly treatment technique have been analyzed in this study. The best treatment conditions to obtain nanocomposites with embedded core-shell particles with enhanced dielectric properties were considered. Treatment of polymer matrices in water solution iron(II)-chloride had the most pronounced precipitation effect, that was directly related to the appearance of higher transition metal concentrations in the iPP and aPS matrices, in comparison to treatments in the other two transition metal salts, MnCl2 and NiCl2. Relative dielectric constant and loss tangent have been studied in the frequency range from 20 Hz to 9 MHz. Embedded core-shell nanoparticles (from 15 to 150 nm in diameter) in a very small amount (1.72E-8 mol/cm3 to 1.17E-5 mol/cm3) resulted in significant improvement (2.5% up to 9.1%) and stabilization of relative dielectric constant value toward higher frequencies and also lowering loss tangent in compare to starting polymer matrices. These properties indicate that materials obtained with the presented treatment technique can be applied as microelectronic packing and with further development of the method in order to obtain a higher concentration of metal ions as energy storage devices.",
publisher = "Wiley",
journal = "Polymers for Advanced Technologies",
title = "Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions",
pages = "1-10",
doi = "10.1002/pat.6110"
}
Petronijević, I., Dudić, D., Cerović, D., Maletić, S., Marinković, F., Pergal, M.,& Anđelković, L.. (2023). Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions. in Polymers for Advanced Technologies
Wiley., 1-10.
https://doi.org/10.1002/pat.6110
Petronijević I, Dudić D, Cerović D, Maletić S, Marinković F, Pergal M, Anđelković L. Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions. in Polymers for Advanced Technologies. 2023;:1-10.
doi:10.1002/pat.6110 .
Petronijević, Ivan, Dudić, Duško, Cerović, Dragana, Maletić, Slavica, Marinković, Filip, Pergal, Marija, Anđelković, Ljubica, "Dielectric properties of iPP and aPS nanocomposites with core-shell particles obtained by treatment in transition metal salt solutions" in Polymers for Advanced Technologies (2023):1-10,
https://doi.org/10.1002/pat.6110 . .

Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition

Anđelković, Ljubica; Šuljagić, Marija; Mirković, Miljana; Pavlović, Vera; Petronijević, Ivan; Stanković, Dalibor; Jeremić, Dejan; Uskoković, Vuk

(Elsevier, 2023)

TY  - JOUR
AU  - Anđelković, Ljubica
AU  - Šuljagić, Marija
AU  - Mirković, Miljana
AU  - Pavlović, Vera
AU  - Petronijević, Ivan
AU  - Stanković, Dalibor
AU  - Jeremić, Dejan
AU  - Uskoković, Vuk
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6199
AB  - The combination of an intense absorption of visible light and p-type semiconducting nature makes spinel cobalt oxide (Co3O4) a very attractive material for various optoelectronic applications. However, the traditional methods for its synthesis have been either time- and energy-consuming or relying on toxic chemicals. To solve this issue, a simple, facile, and eco-friendly method of synthesis was successfully developed to obtain spinel Co3O4 nanoparticles. The novel method for obtaining pure and monophasic Co3O4 reported here is based on the thermal decomposition of hexaaquacobalt(II) D-camphor10-sulfonate at 900 °C. This fast solid-state synthesis route overcomes the disadvantages of many combustion methods, most critically by avoiding the use of toxic organic solvents. The synthesized material was subjected to a detailed characterization to assess its potential for use as a nanocatalyst. The band gap measurements indicated the presence of two band gaps, one at 2.10 eV and another at 1.22 eV, confirming the purity and semiconducting properties of the sample. The electrochemical studies demonstrated a significant enhancement in the electron transfer kinetics with the addition of the synthesized Co3O4 to the carbon-paste electrode, leading to an enhanced electrocatalytic performance. These prominent functional properties, suitable for a wide range of technological applications, pave way for the implementation of the reported method for the synthesis of Co3O4 on a larger industrial scale.
PB  - Elsevier
T2  - Ceramics International
T1  - Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition
DO  - 10.1016/j.ceramint.2023.04.182
ER  - 
@article{
author = "Anđelković, Ljubica and Šuljagić, Marija and Mirković, Miljana and Pavlović, Vera and Petronijević, Ivan and Stanković, Dalibor and Jeremić, Dejan and Uskoković, Vuk",
year = "2023",
abstract = "The combination of an intense absorption of visible light and p-type semiconducting nature makes spinel cobalt oxide (Co3O4) a very attractive material for various optoelectronic applications. However, the traditional methods for its synthesis have been either time- and energy-consuming or relying on toxic chemicals. To solve this issue, a simple, facile, and eco-friendly method of synthesis was successfully developed to obtain spinel Co3O4 nanoparticles. The novel method for obtaining pure and monophasic Co3O4 reported here is based on the thermal decomposition of hexaaquacobalt(II) D-camphor10-sulfonate at 900 °C. This fast solid-state synthesis route overcomes the disadvantages of many combustion methods, most critically by avoiding the use of toxic organic solvents. The synthesized material was subjected to a detailed characterization to assess its potential for use as a nanocatalyst. The band gap measurements indicated the presence of two band gaps, one at 2.10 eV and another at 1.22 eV, confirming the purity and semiconducting properties of the sample. The electrochemical studies demonstrated a significant enhancement in the electron transfer kinetics with the addition of the synthesized Co3O4 to the carbon-paste electrode, leading to an enhanced electrocatalytic performance. These prominent functional properties, suitable for a wide range of technological applications, pave way for the implementation of the reported method for the synthesis of Co3O4 on a larger industrial scale.",
publisher = "Elsevier",
journal = "Ceramics International",
title = "Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition",
doi = "10.1016/j.ceramint.2023.04.182"
}
Anđelković, L., Šuljagić, M., Mirković, M., Pavlović, V., Petronijević, I., Stanković, D., Jeremić, D.,& Uskoković, V.. (2023). Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition. in Ceramics International
Elsevier..
https://doi.org/10.1016/j.ceramint.2023.04.182
Anđelković L, Šuljagić M, Mirković M, Pavlović V, Petronijević I, Stanković D, Jeremić D, Uskoković V. Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition. in Ceramics International. 2023;.
doi:10.1016/j.ceramint.2023.04.182 .
Anđelković, Ljubica, Šuljagić, Marija, Mirković, Miljana, Pavlović, Vera, Petronijević, Ivan, Stanković, Dalibor, Jeremić, Dejan, Uskoković, Vuk, "Semiconducting cobalt oxide nanocatalyst obtained through an eco-friendly thermal decomposition" in Ceramics International (2023),
https://doi.org/10.1016/j.ceramint.2023.04.182 . .

The influence of strontium content and sintering temperature on monazite stability

Mirković, Miljana; Maletaskić, Jelena; Butulija, Svetlana; Anđelković, Ljubica; Šuljagić, Marija

(Association for ETRAN Society, 2023)

TY  - JOUR
AU  - Mirković, Miljana
AU  - Maletaskić, Jelena
AU  - Butulija, Svetlana
AU  - Anđelković, Ljubica
AU  - Šuljagić, Marija
PY  - 2023
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/7211
AB  - This paper shows a simple way to synthesize a series of Ce1-xSrxPO4 ceramic materials using acetate solutions of Ce and Sr instead of nitrate which were used so far. For synthesis, the preparation method was used by simple mixing of acetate solutions of Ceand Sr(, with NaH2PO4 at room temperature, and the studied compositions were Ce1-xSrxPO4 (where x = 0, 0.1, 0.2, 0.3, 0.4, 0.5). The disintegration of Sr in monazite structures in different sintering temperature ranges from 600°C to 1000°C was investigated. The X-ray diffraction was used to track the evolution of the phase composition with thermal treatment. The morphology of sintered ceramics was obtained by scanning electron microscopy and vibrational bands of selected spectra were observed using the FT-IR method. Relative geometric density of selected samples was evaluated. The most favorable conditions for obtaining high-temperature Ce, Sr phosphate-based ceramic material are reported.
AB  - У овом раду је приказан једноставан начин да се синтетише серија Ce1-xSrxPO4 керамичких материјала коришћењем ацетатних раствора Ce и Sr уместо до сада  коришћених нитрата. За синтезу је коришћен метод припреме једноставним мешањем  раствора Ce(C2H3O2)3·xH2O), Sr(C2H3O2)2, и NaH2PO4 као прекурсора на собној  температури, а испитивани састави су Ce1-xSrxPO4 (где је к = 0 , 0,1, 0,2, 0,3, 0,4, 0,5).  Испитивана је дезинтеграција Sr у структурама моназита у различитим  температурним распонима синтеровања од 600 °C до 1000 °C. Дифракција рендгенских  зрака на праху (XRD) је коришћена за праћење еволуције фазног састава синтетисаних и  синтерованих узорака. Морфологија синтероване керамике испитивана је скенирајућом  електронском микроскопијом (СЕМ), а вибрациое траке одабраних спектра су испитане  ФТИР методом. Згушњавање и еволуција микроструктуре су одређене коришћењем  релативне геометријске густине одабраних узорака. Приказани су најповољнији услови за  добијање високотемпературног керамичког материјала на бази Ce, Sr фосфата.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - The influence of strontium content and sintering temperature on monazite stability
DO  - 10.2298/SOS220811024M
ER  - 
@article{
author = "Mirković, Miljana and Maletaskić, Jelena and Butulija, Svetlana and Anđelković, Ljubica and Šuljagić, Marija",
year = "2023",
abstract = "This paper shows a simple way to synthesize a series of Ce1-xSrxPO4 ceramic materials using acetate solutions of Ce and Sr instead of nitrate which were used so far. For synthesis, the preparation method was used by simple mixing of acetate solutions of Ceand Sr(, with NaH2PO4 at room temperature, and the studied compositions were Ce1-xSrxPO4 (where x = 0, 0.1, 0.2, 0.3, 0.4, 0.5). The disintegration of Sr in monazite structures in different sintering temperature ranges from 600°C to 1000°C was investigated. The X-ray diffraction was used to track the evolution of the phase composition with thermal treatment. The morphology of sintered ceramics was obtained by scanning electron microscopy and vibrational bands of selected spectra were observed using the FT-IR method. Relative geometric density of selected samples was evaluated. The most favorable conditions for obtaining high-temperature Ce, Sr phosphate-based ceramic material are reported., У овом раду је приказан једноставан начин да се синтетише серија Ce1-xSrxPO4 керамичких материјала коришћењем ацетатних раствора Ce и Sr уместо до сада  коришћених нитрата. За синтезу је коришћен метод припреме једноставним мешањем  раствора Ce(C2H3O2)3·xH2O), Sr(C2H3O2)2, и NaH2PO4 као прекурсора на собној  температури, а испитивани састави су Ce1-xSrxPO4 (где је к = 0 , 0,1, 0,2, 0,3, 0,4, 0,5).  Испитивана је дезинтеграција Sr у структурама моназита у различитим  температурним распонима синтеровања од 600 °C до 1000 °C. Дифракција рендгенских  зрака на праху (XRD) је коришћена за праћење еволуције фазног састава синтетисаних и  синтерованих узорака. Морфологија синтероване керамике испитивана је скенирајућом  електронском микроскопијом (СЕМ), а вибрациое траке одабраних спектра су испитане  ФТИР методом. Згушњавање и еволуција микроструктуре су одређене коришћењем  релативне геометријске густине одабраних узорака. Приказани су најповољнији услови за  добијање високотемпературног керамичког материјала на бази Ce, Sr фосфата.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "The influence of strontium content and sintering temperature on monazite stability",
doi = "10.2298/SOS220811024M"
}
Mirković, M., Maletaskić, J., Butulija, S., Anđelković, L.,& Šuljagić, M.. (2023). The influence of strontium content and sintering temperature on monazite stability. in Science of Sintering
Association for ETRAN Society..
https://doi.org/10.2298/SOS220811024M
Mirković M, Maletaskić J, Butulija S, Anđelković L, Šuljagić M. The influence of strontium content and sintering temperature on monazite stability. in Science of Sintering. 2023;.
doi:10.2298/SOS220811024M .
Mirković, Miljana, Maletaskić, Jelena, Butulija, Svetlana, Anđelković, Ljubica, Šuljagić, Marija, "The influence of strontium content and sintering temperature on monazite stability" in Science of Sintering (2023),
https://doi.org/10.2298/SOS220811024M . .

Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions

Đukić, Dunja; Krstić, Aleksandar; Jakovljević, Ksenija; Butulija, Svetlana; Anđelković, Ljubica; Pavlović, Vladimir; Mirković, Miljana

(MDPI, 2022)

TY  - JOUR
AU  - Đukić, Dunja
AU  - Krstić, Aleksandar
AU  - Jakovljević, Ksenija
AU  - Butulija, Svetlana
AU  - Anđelković, Ljubica
AU  - Pavlović, Vladimir
AU  - Mirković, Miljana
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4941
AB  - Newly designed mesoporous brushite-metakaolin-based geopolymer materials were examined with an idea for using this material as a potential adsorbent for Pb(II) removal from aqueous solutions. As a starting component for geopolymer synthesis, a natural raw kaolinite clay with the
addition of 2 wt.%, 4 wt.%, 6 wt.%, 8 wt.%, and 10 wt.% of pure brushite was used. Phase, structural,morphological, and adsorption properties of newly synthesized mesoporous brushite-metakaolin geopolymer materials were examined in detail by the means of XRPD, FTIR, SEM-EDS, BET/BJH, and ICP-OES methods. The ICP-OES results showed that the synthesized material samples with 2 wt.%, 4 wt.%, and 6 wt.% of brushite possess significant adsorption properties and the mechanisms of the adsorption process can be attributed to chemisorption. The most notable result is that brushite-metakaolin-geopolymer with 2 wt.% of brushite have the best efficiency removal, more than 85% of Pb(II).
PB  - MDPI
T2  - Sustainability
T1  - Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions
VL  - 14
IS  - 7
SP  - 4003
DO  - 10.3390/su14074003
ER  - 
@article{
author = "Đukić, Dunja and Krstić, Aleksandar and Jakovljević, Ksenija and Butulija, Svetlana and Anđelković, Ljubica and Pavlović, Vladimir and Mirković, Miljana",
year = "2022",
abstract = "Newly designed mesoporous brushite-metakaolin-based geopolymer materials were examined with an idea for using this material as a potential adsorbent for Pb(II) removal from aqueous solutions. As a starting component for geopolymer synthesis, a natural raw kaolinite clay with the
addition of 2 wt.%, 4 wt.%, 6 wt.%, 8 wt.%, and 10 wt.% of pure brushite was used. Phase, structural,morphological, and adsorption properties of newly synthesized mesoporous brushite-metakaolin geopolymer materials were examined in detail by the means of XRPD, FTIR, SEM-EDS, BET/BJH, and ICP-OES methods. The ICP-OES results showed that the synthesized material samples with 2 wt.%, 4 wt.%, and 6 wt.% of brushite possess significant adsorption properties and the mechanisms of the adsorption process can be attributed to chemisorption. The most notable result is that brushite-metakaolin-geopolymer with 2 wt.% of brushite have the best efficiency removal, more than 85% of Pb(II).",
publisher = "MDPI",
journal = "Sustainability",
title = "Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions",
volume = "14",
number = "7",
pages = "4003",
doi = "10.3390/su14074003"
}
Đukić, D., Krstić, A., Jakovljević, K., Butulija, S., Anđelković, L., Pavlović, V.,& Mirković, M.. (2022). Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions. in Sustainability
MDPI., 14(7), 4003.
https://doi.org/10.3390/su14074003
Đukić D, Krstić A, Jakovljević K, Butulija S, Anđelković L, Pavlović V, Mirković M. Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions. in Sustainability. 2022;14(7):4003.
doi:10.3390/su14074003 .
Đukić, Dunja, Krstić, Aleksandar, Jakovljević, Ksenija, Butulija, Svetlana, Anđelković, Ljubica, Pavlović, Vladimir, Mirković, Miljana, "Brushite-Metakaolin Composite Geopolymer Material as an Effective Adsorbent for Lead Removal from Aqueous Solutions" in Sustainability, 14, no. 7 (2022):4003,
https://doi.org/10.3390/su14074003 . .
2

Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites

Šuljagić, Marija; Milenković, Milica; Uskoković, Vuk; Mirković, Miljana; Vrbica, Boško; Pavlović, Vladimir B.; Živković-Radovanović, Vukosava; Stanković, Dalibor; Anđelković, Ljubica

(Elsevier, 2022)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Milenković, Milica
AU  - Uskoković, Vuk
AU  - Mirković, Miljana
AU  - Vrbica, Boško
AU  - Pavlović, Vladimir B.
AU  - Živković-Radovanović, Vukosava
AU  - Stanković, Dalibor
AU  - Anđelković, Ljubica
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5329
AB  - The emerging threat of bacterial resistance to antibiotics prompts the urgent search for biomaterials for the treatment of infectious disease. Here we report on the synthesis and characterization of a multiphasic nanocomposite comprising magnetic iron oxide and silver nanoparticles. The method of synthesis involved the combustion of a metalorganic complex and reduction of the silver ions that were exchanged and/or adsorbed on the surface of iron oxide. Different physical and chemical treatments coupled to the reduction process, including ultrasound and Lugol's iodine solution, respectively, homogenized the distribution of the silver nanoparticles on the iron oxide phase. Remarkably, using ascorbic acid as a reductant enhanced the magnetic properties of the material as a result of the reduction of the magnetic matrix alongside the silver cations. The treatment with ultrasound detached large amounts of silver from the iron oxide phase and resulted in the lowest amount of silver incorporated in the nanocomposite. Despite that, this treatment led to the highest antibacterial activity against both Gram-positive and Gram-negative strains, indicating that the homogeneity of the distribution of silver on the iron oxide matrix is a more important determinant of the antibacterial performance than the amount of silver incorporated in the material. At the same time, the treatment with Lugol's iodine equally increased the distribution homogeneity, but induced excessive ion exchange and crystal lattice substitutions, thereby adversely affecting the antibacterial performance. This has indicated that the mode of binding silver to iron oxide can compensate for the positive effects of homogeneous distribution with respect to the antibacterial performance.
PB  - Elsevier
T2  - Materials Today Communications
T1  - Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites
VL  - 32
SP  - 104157
DO  - 10.1016/j.mtcomm.2022.104157
ER  - 
@article{
author = "Šuljagić, Marija and Milenković, Milica and Uskoković, Vuk and Mirković, Miljana and Vrbica, Boško and Pavlović, Vladimir B. and Živković-Radovanović, Vukosava and Stanković, Dalibor and Anđelković, Ljubica",
year = "2022",
abstract = "The emerging threat of bacterial resistance to antibiotics prompts the urgent search for biomaterials for the treatment of infectious disease. Here we report on the synthesis and characterization of a multiphasic nanocomposite comprising magnetic iron oxide and silver nanoparticles. The method of synthesis involved the combustion of a metalorganic complex and reduction of the silver ions that were exchanged and/or adsorbed on the surface of iron oxide. Different physical and chemical treatments coupled to the reduction process, including ultrasound and Lugol's iodine solution, respectively, homogenized the distribution of the silver nanoparticles on the iron oxide phase. Remarkably, using ascorbic acid as a reductant enhanced the magnetic properties of the material as a result of the reduction of the magnetic matrix alongside the silver cations. The treatment with ultrasound detached large amounts of silver from the iron oxide phase and resulted in the lowest amount of silver incorporated in the nanocomposite. Despite that, this treatment led to the highest antibacterial activity against both Gram-positive and Gram-negative strains, indicating that the homogeneity of the distribution of silver on the iron oxide matrix is a more important determinant of the antibacterial performance than the amount of silver incorporated in the material. At the same time, the treatment with Lugol's iodine equally increased the distribution homogeneity, but induced excessive ion exchange and crystal lattice substitutions, thereby adversely affecting the antibacterial performance. This has indicated that the mode of binding silver to iron oxide can compensate for the positive effects of homogeneous distribution with respect to the antibacterial performance.",
publisher = "Elsevier",
journal = "Materials Today Communications",
title = "Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites",
volume = "32",
pages = "104157",
doi = "10.1016/j.mtcomm.2022.104157"
}
Šuljagić, M., Milenković, M., Uskoković, V., Mirković, M., Vrbica, B., Pavlović, V. B., Živković-Radovanović, V., Stanković, D.,& Anđelković, L.. (2022). Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites. in Materials Today Communications
Elsevier., 32, 104157.
https://doi.org/10.1016/j.mtcomm.2022.104157
Šuljagić M, Milenković M, Uskoković V, Mirković M, Vrbica B, Pavlović VB, Živković-Radovanović V, Stanković D, Anđelković L. Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites. in Materials Today Communications. 2022;32:104157.
doi:10.1016/j.mtcomm.2022.104157 .
Šuljagić, Marija, Milenković, Milica, Uskoković, Vuk, Mirković, Miljana, Vrbica, Boško, Pavlović, Vladimir B., Živković-Radovanović, Vukosava, Stanković, Dalibor, Anđelković, Ljubica, "Silver distribution and binding mode as key determinants of the antimicrobial performance of iron oxide/silver nanocomposites" in Materials Today Communications, 32 (2022):104157,
https://doi.org/10.1016/j.mtcomm.2022.104157 . .
2
2

Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials

Đukić, Dunja; Šuljagić, Marija; Anđelković, Ljubica; Pavlović, Vera; Bučevac, Dušan; Vrbica, Boško; Mirković, Miljana

(Association for ETRAN Society, 2022)

TY  - JOUR
AU  - Đukić, Dunja
AU  - Šuljagić, Marija
AU  - Anđelković, Ljubica
AU  - Pavlović, Vera
AU  - Bučevac, Dušan
AU  - Vrbica, Boško
AU  - Mirković, Miljana
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5332
AB  - The effect of Ca2+ amount and sintering temperature on mechanical properties of geopolymer-brushite (GPB) binders was investigated. Brushite and raw abandoned kaolinite clay thermally transformed into metakaolin were used for GPB synthesis. The complete phase and structural analyses were performed by X-ray powder diffraction, and Fourier transforms infrared spectroscopy (FT-IR). The pore-filling effect as a consequence of Ca2+ ions incorporation into the hybrid geopolymer networks improved the compressive strength. On the other hand, the chosen biscuit sintering at 800 and 900oC caused the phase transformation of brushite into calcium pyrophosphate, which negatively affected the compressive strength of such materials. The obtained results indicate that the usage of relatively high sintering temperatures is not always the necessary step for producing geopolymer-based types of cement with prominent mechanical properties.
AB  - U ovom radu ispitivan je uticaj količine dodatog brušita i temperature sinterovanja na mehanička svojstva geopolimer-brušit veziva. Kao
polazni materijali za sintezu korišćeni su kaolinitska glina i sintetisani brušit. Kompletna fazna i strukturna analiza izvršena je difrakcijom
rendgenskih zraka na prahu i infracrvenom spektroskopijom sa Furijeovom transformacijom. Efekat dodatka brušita u geopolimernu matricu poboljšao je pritisnu čvrstoću, dok je biskvitno pečenje izazvalo faznu transformaciju brušita u kalcijum pirofosfat što je negativno uticalo na pritisnu čvrstoću takvih materijala. Dobijeni rezultati ukazuju da korišćenje relativno visokih temperatura sinterovanja nije uvek neophodan korak za proizvodnju cementa na bazi geopolimera sa istaknutim mehaničkim svojstvima.
PB  - Association for ETRAN Society
T2  - Science of Sintering
T1  - Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials
VL  - 54
IS  - 3
SP  - 287
EP  - 294
DO  - 10.2298/SOS2203287D
ER  - 
@article{
author = "Đukić, Dunja and Šuljagić, Marija and Anđelković, Ljubica and Pavlović, Vera and Bučevac, Dušan and Vrbica, Boško and Mirković, Miljana",
year = "2022",
abstract = "The effect of Ca2+ amount and sintering temperature on mechanical properties of geopolymer-brushite (GPB) binders was investigated. Brushite and raw abandoned kaolinite clay thermally transformed into metakaolin were used for GPB synthesis. The complete phase and structural analyses were performed by X-ray powder diffraction, and Fourier transforms infrared spectroscopy (FT-IR). The pore-filling effect as a consequence of Ca2+ ions incorporation into the hybrid geopolymer networks improved the compressive strength. On the other hand, the chosen biscuit sintering at 800 and 900oC caused the phase transformation of brushite into calcium pyrophosphate, which negatively affected the compressive strength of such materials. The obtained results indicate that the usage of relatively high sintering temperatures is not always the necessary step for producing geopolymer-based types of cement with prominent mechanical properties., U ovom radu ispitivan je uticaj količine dodatog brušita i temperature sinterovanja na mehanička svojstva geopolimer-brušit veziva. Kao
polazni materijali za sintezu korišćeni su kaolinitska glina i sintetisani brušit. Kompletna fazna i strukturna analiza izvršena je difrakcijom
rendgenskih zraka na prahu i infracrvenom spektroskopijom sa Furijeovom transformacijom. Efekat dodatka brušita u geopolimernu matricu poboljšao je pritisnu čvrstoću, dok je biskvitno pečenje izazvalo faznu transformaciju brušita u kalcijum pirofosfat što je negativno uticalo na pritisnu čvrstoću takvih materijala. Dobijeni rezultati ukazuju da korišćenje relativno visokih temperatura sinterovanja nije uvek neophodan korak za proizvodnju cementa na bazi geopolimera sa istaknutim mehaničkim svojstvima.",
publisher = "Association for ETRAN Society",
journal = "Science of Sintering",
title = "Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials",
volume = "54",
number = "3",
pages = "287-294",
doi = "10.2298/SOS2203287D"
}
Đukić, D., Šuljagić, M., Anđelković, L., Pavlović, V., Bučevac, D., Vrbica, B.,& Mirković, M.. (2022). Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials. in Science of Sintering
Association for ETRAN Society., 54(3), 287-294.
https://doi.org/10.2298/SOS2203287D
Đukić D, Šuljagić M, Anđelković L, Pavlović V, Bučevac D, Vrbica B, Mirković M. Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials. in Science of Sintering. 2022;54(3):287-294.
doi:10.2298/SOS2203287D .
Đukić, Dunja, Šuljagić, Marija, Anđelković, Ljubica, Pavlović, Vera, Bučevac, Dušan, Vrbica, Boško, Mirković, Miljana, "Effect of Sintering Temperature and Calcium amount on Compressive Strength of Brushite-Metakaolin Polymer Materials" in Science of Sintering, 54, no. 3 (2022):287-294,
https://doi.org/10.2298/SOS2203287D . .

Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid

Šuljagić, Marija; Stanković, Dalibor; Mirković, M.; Pavlović, V.; Petronijević, I.; Jeremić, Dejan; Anđelković, Ljubica

(Springer, 2022)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Stanković, Dalibor
AU  - Mirković, M.
AU  - Pavlović, V.
AU  - Petronijević, I.
AU  - Jeremić, Dejan
AU  - Anđelković, Ljubica
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5618
AB  - Nickel ferrite nanoparticles were synthesized via thermal decomposition of β-diketonato complexes of nickel(II) and iron(III). The mechano-chemical activation of the complex precursors was used to ensure the increase in the reaction activity and consequently reduce thermal decomposition temperature. The prepared sample was thoroughly characterized by X-ray powder diffraction, FT-IR spectroscopy, scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS), and transmission electron microscopy (TEM). X-ray powder diffraction and FT-IR confirmed the spinel phase of the investigated powder. SEM and TEM revealed the ultrafine nature of nanosized polygonal particles, with a pronounced agglomeration effect. The capacity for electrocatalytic applications was examined using cyclic voltammetry (CV) and electrical impedance spectroscopy (EIS). Electrocatalytic measurements pointed out that the addition of 5% of nickel ferrite as a modifier to carbon paste electrode caused a current increase and a decrease of the EIS semicircle. Further increase in the amount of the modifier decreased heterogeneity of the electrode surface and served as excellent sensor for the detection of gallic acid in the concentration range from 1 to 10 µM with the detection limit of 0.27 µM. This unambiguously indicated the significant improvement in electrode transfer rate and better characteristics of the diffusion layer.
PB  - Springer
T2  - Russian Journal of Inorganic Chemistry
T1  - Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid
VL  - 67
IS  - S1
SP  - S13
EP  - S21
DO  - 10.1134/S003602362260201X
ER  - 
@article{
author = "Šuljagić, Marija and Stanković, Dalibor and Mirković, M. and Pavlović, V. and Petronijević, I. and Jeremić, Dejan and Anđelković, Ljubica",
year = "2022",
abstract = "Nickel ferrite nanoparticles were synthesized via thermal decomposition of β-diketonato complexes of nickel(II) and iron(III). The mechano-chemical activation of the complex precursors was used to ensure the increase in the reaction activity and consequently reduce thermal decomposition temperature. The prepared sample was thoroughly characterized by X-ray powder diffraction, FT-IR spectroscopy, scanning electron microscopy (SEM) coupled with electron dispersive spectroscopy (EDS), and transmission electron microscopy (TEM). X-ray powder diffraction and FT-IR confirmed the spinel phase of the investigated powder. SEM and TEM revealed the ultrafine nature of nanosized polygonal particles, with a pronounced agglomeration effect. The capacity for electrocatalytic applications was examined using cyclic voltammetry (CV) and electrical impedance spectroscopy (EIS). Electrocatalytic measurements pointed out that the addition of 5% of nickel ferrite as a modifier to carbon paste electrode caused a current increase and a decrease of the EIS semicircle. Further increase in the amount of the modifier decreased heterogeneity of the electrode surface and served as excellent sensor for the detection of gallic acid in the concentration range from 1 to 10 µM with the detection limit of 0.27 µM. This unambiguously indicated the significant improvement in electrode transfer rate and better characteristics of the diffusion layer.",
publisher = "Springer",
journal = "Russian Journal of Inorganic Chemistry",
title = "Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid",
volume = "67",
number = "S1",
pages = "S13-S21",
doi = "10.1134/S003602362260201X"
}
Šuljagić, M., Stanković, D., Mirković, M., Pavlović, V., Petronijević, I., Jeremić, D.,& Anđelković, L.. (2022). Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid. in Russian Journal of Inorganic Chemistry
Springer., 67(S1), S13-S21.
https://doi.org/10.1134/S003602362260201X
Šuljagić M, Stanković D, Mirković M, Pavlović V, Petronijević I, Jeremić D, Anđelković L. Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid. in Russian Journal of Inorganic Chemistry. 2022;67(S1):S13-S21.
doi:10.1134/S003602362260201X .
Šuljagić, Marija, Stanković, Dalibor, Mirković, M., Pavlović, V., Petronijević, I., Jeremić, Dejan, Anđelković, Ljubica, "Novel Solid-State Approach to Nickel Ferrite Electrocatalyst for the Detection of Gallic Acid" in Russian Journal of Inorganic Chemistry, 67, no. S1 (2022):S13-S21,
https://doi.org/10.1134/S003602362260201X . .
3
2

Structural characterization of titanate–ferrite composites

Šuljagić, Marija; Jeremić, Dejan; Nikolić, Aleksandar S.; Anđelković, Ljubica

(Portugal: PROTEOMASS Scientific Society, 2022)

TY  - CONF
AU  - Šuljagić, Marija
AU  - Jeremić, Dejan
AU  - Nikolić, Aleksandar S.
AU  - Anđelković, Ljubica
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5908
AB  - Barium titanate–nickel ferrite, barium titanate–zinc ferrite, and barium titanate–nickel-zinc ferrite composite powders prepared by thermal decomposition method were characterized by Raman spectroscopy, scanning electron microscopy (SEM), and X-Ray powder diffraction (XRPD). Obtained materials consisted of pure perovskite and spinel phases. Scanning electron microscopy analyses revealed that the morphology of investigated samples is not uniform, and aggregation of individual particles is a dominant process in all cases. Raman spectroscopy suggested that in the case of barium titanate–nickel ferrite, the coupling of two phases occurred and the core-shell structure was partially formed, while for barium titanate–zinc ferrite the coupling effect is less pronounced.
PB  - Portugal: PROTEOMASS Scientific Society
C3  - Book of Abstracts, 5th International Caparica Symposium on Nanoparticles, Nanomaterials and Applications, 24-27 January, 2022, Caparica, Portugal
T1  - Structural characterization of titanate–ferrite composites
SP  - 212
EP  - 212
UR  - https://hdl.handle.net/21.15107/rcub_cer_5908
ER  - 
@conference{
author = "Šuljagić, Marija and Jeremić, Dejan and Nikolić, Aleksandar S. and Anđelković, Ljubica",
year = "2022",
abstract = "Barium titanate–nickel ferrite, barium titanate–zinc ferrite, and barium titanate–nickel-zinc ferrite composite powders prepared by thermal decomposition method were characterized by Raman spectroscopy, scanning electron microscopy (SEM), and X-Ray powder diffraction (XRPD). Obtained materials consisted of pure perovskite and spinel phases. Scanning electron microscopy analyses revealed that the morphology of investigated samples is not uniform, and aggregation of individual particles is a dominant process in all cases. Raman spectroscopy suggested that in the case of barium titanate–nickel ferrite, the coupling of two phases occurred and the core-shell structure was partially formed, while for barium titanate–zinc ferrite the coupling effect is less pronounced.",
publisher = "Portugal: PROTEOMASS Scientific Society",
journal = "Book of Abstracts, 5th International Caparica Symposium on Nanoparticles, Nanomaterials and Applications, 24-27 January, 2022, Caparica, Portugal",
title = "Structural characterization of titanate–ferrite composites",
pages = "212-212",
url = "https://hdl.handle.net/21.15107/rcub_cer_5908"
}
Šuljagić, M., Jeremić, D., Nikolić, A. S.,& Anđelković, L.. (2022). Structural characterization of titanate–ferrite composites. in Book of Abstracts, 5th International Caparica Symposium on Nanoparticles, Nanomaterials and Applications, 24-27 January, 2022, Caparica, Portugal
Portugal: PROTEOMASS Scientific Society., 212-212.
https://hdl.handle.net/21.15107/rcub_cer_5908
Šuljagić M, Jeremić D, Nikolić AS, Anđelković L. Structural characterization of titanate–ferrite composites. in Book of Abstracts, 5th International Caparica Symposium on Nanoparticles, Nanomaterials and Applications, 24-27 January, 2022, Caparica, Portugal. 2022;:212-212.
https://hdl.handle.net/21.15107/rcub_cer_5908 .
Šuljagić, Marija, Jeremić, Dejan, Nikolić, Aleksandar S., Anđelković, Ljubica, "Structural characterization of titanate–ferrite composites" in Book of Abstracts, 5th International Caparica Symposium on Nanoparticles, Nanomaterials and Applications, 24-27 January, 2022, Caparica, Portugal (2022):212-212,
https://hdl.handle.net/21.15107/rcub_cer_5908 .

The phase content effect on the functional properties of BaTiO3/CoFe2O4 composites prepared by different synthetic methods

Anđelković, Ljubica

(Belgrade: Serbian Ceramic Society, 2022)

TY  - CONF
AU  - Anđelković, Ljubica
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/5910
AB  - The CoFe2O4 nanoparticles were in situ synthesized on commercial BaTiO3 by thermal decomposition, coprecipitation, and microemulsion method. After initial preparation  procedures, the obtained powders were sintered at 1150 °C and 1300 °C in a pellet form. The bare powders, as well as sintered pellets, were thoroughly characterized by X-ray powder  diffraction and scanning electron microscopy coupled with electron dispersive spectroscopy.  The impedance spectroscopy, dielectric, and ferroelectric measurements were used to get  deeper insight into electrical properties of prepared materials. Better dielectric properties were  achieved for samples sintered at 1300 °C, irrespective of chosen synthetic route. The different  phase content obtained by three chosen synthetic procedures influenced different electrical properties of the investigated samples. The sample prepared in a microemulsion manner and  sintered at 1300 °C showed the best dielectric performances which can be explained by the  highest amount of barioferrite-like phase and the lowest amount of undesired  centrosymmetric P4/mmm BaTiO3 phase. Although well-defined electric hysteresis loops  were not achieved, the sample synthesized by thermal decomposition showed electrical  hysteresis most similar to conventional hysteresis loop of ferroelectric materials owing to highest amount of BaTiO3 phase.
PB  - Belgrade: Serbian Ceramic Society
C3  - Program and the Book of Abstracts, The Tenth Serbian Ceramic Society Conference Advanced Ceramics and Application, September 26-27, 2022, Belgrade, Serbia
T1  - The phase content effect on the functional properties of BaTiO3/CoFe2O4  composites prepared by different synthetic methods
SP  - 43
EP  - 44
UR  - https://hdl.handle.net/21.15107/rcub_cer_5910
ER  - 
@conference{
author = "Anđelković, Ljubica",
year = "2022",
abstract = "The CoFe2O4 nanoparticles were in situ synthesized on commercial BaTiO3 by thermal decomposition, coprecipitation, and microemulsion method. After initial preparation  procedures, the obtained powders were sintered at 1150 °C and 1300 °C in a pellet form. The bare powders, as well as sintered pellets, were thoroughly characterized by X-ray powder  diffraction and scanning electron microscopy coupled with electron dispersive spectroscopy.  The impedance spectroscopy, dielectric, and ferroelectric measurements were used to get  deeper insight into electrical properties of prepared materials. Better dielectric properties were  achieved for samples sintered at 1300 °C, irrespective of chosen synthetic route. The different  phase content obtained by three chosen synthetic procedures influenced different electrical properties of the investigated samples. The sample prepared in a microemulsion manner and  sintered at 1300 °C showed the best dielectric performances which can be explained by the  highest amount of barioferrite-like phase and the lowest amount of undesired  centrosymmetric P4/mmm BaTiO3 phase. Although well-defined electric hysteresis loops  were not achieved, the sample synthesized by thermal decomposition showed electrical  hysteresis most similar to conventional hysteresis loop of ferroelectric materials owing to highest amount of BaTiO3 phase.",
publisher = "Belgrade: Serbian Ceramic Society",
journal = "Program and the Book of Abstracts, The Tenth Serbian Ceramic Society Conference Advanced Ceramics and Application, September 26-27, 2022, Belgrade, Serbia",
title = "The phase content effect on the functional properties of BaTiO3/CoFe2O4  composites prepared by different synthetic methods",
pages = "43-44",
url = "https://hdl.handle.net/21.15107/rcub_cer_5910"
}
Anđelković, L.. (2022). The phase content effect on the functional properties of BaTiO3/CoFe2O4  composites prepared by different synthetic methods. in Program and the Book of Abstracts, The Tenth Serbian Ceramic Society Conference Advanced Ceramics and Application, September 26-27, 2022, Belgrade, Serbia
Belgrade: Serbian Ceramic Society., 43-44.
https://hdl.handle.net/21.15107/rcub_cer_5910
Anđelković L. The phase content effect on the functional properties of BaTiO3/CoFe2O4  composites prepared by different synthetic methods. in Program and the Book of Abstracts, The Tenth Serbian Ceramic Society Conference Advanced Ceramics and Application, September 26-27, 2022, Belgrade, Serbia. 2022;:43-44.
https://hdl.handle.net/21.15107/rcub_cer_5910 .
Anđelković, Ljubica, "The phase content effect on the functional properties of BaTiO3/CoFe2O4  composites prepared by different synthetic methods" in Program and the Book of Abstracts, The Tenth Serbian Ceramic Society Conference Advanced Ceramics and Application, September 26-27, 2022, Belgrade, Serbia (2022):43-44,
https://hdl.handle.net/21.15107/rcub_cer_5910 .

Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application

Petronijević, Ivan; Dudić, Duško; Cerović, Dragana; Maletić, Slavica; Marinković, Filip; Pergal, Marija; Anđelković, Ljubica

(Belgrade : SANU, 2022)

TY  - CONF
AU  - Petronijević, Ivan
AU  - Dudić, Duško
AU  - Cerović, Dragana
AU  - Maletić, Slavica
AU  - Marinković, Filip
AU  - Pergal, Marija
AU  - Anđelković, Ljubica
PY  - 2022
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/6023
AB  - Polymer nanocomposites are prepared by a simple and environmentally friendly technique. First, sheets of isotactic polypropylene (iPP) and atactic polystyrene (aPS) were prepared by compression molding with Servitec Polystat Press 200 T at 473.15 K and 3.0 MPa pressure followed by quenching in water at room temperature. The polymer sheets thus prepared were then immersed separately in three saturated salt water solutions (MnCl2, FeCl2, and NiCl2), at two temperatures (23ºC and 90ºC), and under influence of two DC electrical potentials (+4 kV, and ground potential). Count profiles and generated images of TOF – SIMS records have shown that higher temperature treatment (90ºC) and positive potential (+4kV) have given the highest count of iron ions and better distribution and dispersion of nanoparticles in polymer matrices. Also, the measured concentration of transition metals by ICP-OES confirmed higher concentrations of metals in nanocomposites obtained by these treatment conditions. It was stated that iron(II)-chloride had the highest concentration in iPP and aPS matrices in comparison to the other two transition salts. TEM micrographs showed spherically-shaped cores in the core-shell system and agglomerated particles of irregular shape. Encapsulation of iron cores prevented nanoparticles
from agglomeration. The cores of the investigated particles were probably iron oxides and/or hydroxides that occurred during the hydrolysis of iron salts in deionized water solution. Dielectric properties of obtained nanodielectrics were investigated. Relative dielectric constant and loss tangent has been studied in the frequency range from 20 Hz to 9 MHz. It was shown that adding the small amount of core-shell nanoparticles (from 15 nm to 150 nm in diameter) in a very small amount (1.72E-8 mol/cm3 to 1.17E-5 mol/cm3) are resulted in significant improvement and stabilization of relative dielectric constant value and also lowering loss tangent in compare to starting polymer matrices.These dielectric properties were marked as suitable for nanodielectric application for high speed and high dencity microelectronic packaging.
PB  - Belgrade : SANU
C3  - The Book of Abstracts, The 11th International Conference of the Balkan Physical Union, 28 August - 1 September, 2022, Belgrade, Serbia
T1  - Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application
SP  - 130
EP  - 130
UR  - https://hdl.handle.net/21.15107/rcub_cer_6023
ER  - 
@conference{
author = "Petronijević, Ivan and Dudić, Duško and Cerović, Dragana and Maletić, Slavica and Marinković, Filip and Pergal, Marija and Anđelković, Ljubica",
year = "2022",
abstract = "Polymer nanocomposites are prepared by a simple and environmentally friendly technique. First, sheets of isotactic polypropylene (iPP) and atactic polystyrene (aPS) were prepared by compression molding with Servitec Polystat Press 200 T at 473.15 K and 3.0 MPa pressure followed by quenching in water at room temperature. The polymer sheets thus prepared were then immersed separately in three saturated salt water solutions (MnCl2, FeCl2, and NiCl2), at two temperatures (23ºC and 90ºC), and under influence of two DC electrical potentials (+4 kV, and ground potential). Count profiles and generated images of TOF – SIMS records have shown that higher temperature treatment (90ºC) and positive potential (+4kV) have given the highest count of iron ions and better distribution and dispersion of nanoparticles in polymer matrices. Also, the measured concentration of transition metals by ICP-OES confirmed higher concentrations of metals in nanocomposites obtained by these treatment conditions. It was stated that iron(II)-chloride had the highest concentration in iPP and aPS matrices in comparison to the other two transition salts. TEM micrographs showed spherically-shaped cores in the core-shell system and agglomerated particles of irregular shape. Encapsulation of iron cores prevented nanoparticles
from agglomeration. The cores of the investigated particles were probably iron oxides and/or hydroxides that occurred during the hydrolysis of iron salts in deionized water solution. Dielectric properties of obtained nanodielectrics were investigated. Relative dielectric constant and loss tangent has been studied in the frequency range from 20 Hz to 9 MHz. It was shown that adding the small amount of core-shell nanoparticles (from 15 nm to 150 nm in diameter) in a very small amount (1.72E-8 mol/cm3 to 1.17E-5 mol/cm3) are resulted in significant improvement and stabilization of relative dielectric constant value and also lowering loss tangent in compare to starting polymer matrices.These dielectric properties were marked as suitable for nanodielectric application for high speed and high dencity microelectronic packaging.",
publisher = "Belgrade : SANU",
journal = "The Book of Abstracts, The 11th International Conference of the Balkan Physical Union, 28 August - 1 September, 2022, Belgrade, Serbia",
title = "Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application",
pages = "130-130",
url = "https://hdl.handle.net/21.15107/rcub_cer_6023"
}
Petronijević, I., Dudić, D., Cerović, D., Maletić, S., Marinković, F., Pergal, M.,& Anđelković, L.. (2022). Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application. in The Book of Abstracts, The 11th International Conference of the Balkan Physical Union, 28 August - 1 September, 2022, Belgrade, Serbia
Belgrade : SANU., 130-130.
https://hdl.handle.net/21.15107/rcub_cer_6023
Petronijević I, Dudić D, Cerović D, Maletić S, Marinković F, Pergal M, Anđelković L. Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application. in The Book of Abstracts, The 11th International Conference of the Balkan Physical Union, 28 August - 1 September, 2022, Belgrade, Serbia. 2022;:130-130.
https://hdl.handle.net/21.15107/rcub_cer_6023 .
Petronijević, Ivan, Dudić, Duško, Cerović, Dragana, Maletić, Slavica, Marinković, Filip, Pergal, Marija, Anđelković, Ljubica, "Polymer nanocomposites filled with core-shell nanoparticles for nanodielectric application" in The Book of Abstracts, The 11th International Conference of the Balkan Physical Union, 28 August - 1 September, 2022, Belgrade, Serbia (2022):130-130,
https://hdl.handle.net/21.15107/rcub_cer_6023 .

The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods

Šuljagić, Marija; Vulić, Predrag; Jeremić, Dejan; Pavlović, Vladimir B.; Filipović, Suzana; Kilanski, Lukasz; Lewinska, Sabina; Slawska-Waniewska, Anna; Milenković, Milica R.; Nikolić, Aleksandar S.; Anđelković, Ljubica

(Elsevier, 2021)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Vulić, Predrag
AU  - Jeremić, Dejan
AU  - Pavlović, Vladimir B.
AU  - Filipović, Suzana
AU  - Kilanski, Lukasz
AU  - Lewinska, Sabina
AU  - Slawska-Waniewska, Anna
AU  - Milenković, Milica R.
AU  - Nikolić, Aleksandar S.
AU  - Anđelković, Ljubica
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/3715
AB  - To investigate the magnetic behavior of starch-coated cobalt ferrites, well-established synthetic methods, i.e., coprecipitation, mechanochemical, ultrasonically assisted coprecipitation, microemulsion, and microwave-assisted hydrothermal syntheses were chosen for their preparation. The obtained materials had pure single-phase spinel structures. Scanning and transmission electron microscopy analyses revealed that the morphology of the samples is not uniform, and particle aggregation is a dominant process. Fourier transform infrared spectra and thermogravimetric analysis confirmed the presence of starch in all–coated samples. The unusually higher saturation magnetization of starch-coated samples than their as-prepared analogs, obtained by coprecipitation, ultrasonically assisted coprecipitation, and microwave-assisted hydrothermal methods, might be explained by the Ostwald ripening mechanism induced by the coating process. A decrease in magnetization was noticed for the starch-functionalized nanomaterials synthesized by mechanochemical and microemulsion methods, in comparison to their as-prepared analogs, i.e., the size distribution of such nanoparticles is narrow, and the average diameter of the grains is near critical for the Ostwald ripening process.
PB  - Elsevier
T2  - Materials Research Bulletin
T1  - The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods
VL  - 134
SP  - 111117
DO  - 10.1016/j.materresbull.2020.111117
ER  - 
@article{
author = "Šuljagić, Marija and Vulić, Predrag and Jeremić, Dejan and Pavlović, Vladimir B. and Filipović, Suzana and Kilanski, Lukasz and Lewinska, Sabina and Slawska-Waniewska, Anna and Milenković, Milica R. and Nikolić, Aleksandar S. and Anđelković, Ljubica",
year = "2021",
abstract = "To investigate the magnetic behavior of starch-coated cobalt ferrites, well-established synthetic methods, i.e., coprecipitation, mechanochemical, ultrasonically assisted coprecipitation, microemulsion, and microwave-assisted hydrothermal syntheses were chosen for their preparation. The obtained materials had pure single-phase spinel structures. Scanning and transmission electron microscopy analyses revealed that the morphology of the samples is not uniform, and particle aggregation is a dominant process. Fourier transform infrared spectra and thermogravimetric analysis confirmed the presence of starch in all–coated samples. The unusually higher saturation magnetization of starch-coated samples than their as-prepared analogs, obtained by coprecipitation, ultrasonically assisted coprecipitation, and microwave-assisted hydrothermal methods, might be explained by the Ostwald ripening mechanism induced by the coating process. A decrease in magnetization was noticed for the starch-functionalized nanomaterials synthesized by mechanochemical and microemulsion methods, in comparison to their as-prepared analogs, i.e., the size distribution of such nanoparticles is narrow, and the average diameter of the grains is near critical for the Ostwald ripening process.",
publisher = "Elsevier",
journal = "Materials Research Bulletin",
title = "The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods",
volume = "134",
pages = "111117",
doi = "10.1016/j.materresbull.2020.111117"
}
Šuljagić, M., Vulić, P., Jeremić, D., Pavlović, V. B., Filipović, S., Kilanski, L., Lewinska, S., Slawska-Waniewska, A., Milenković, M. R., Nikolić, A. S.,& Anđelković, L.. (2021). The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods. in Materials Research Bulletin
Elsevier., 134, 111117.
https://doi.org/10.1016/j.materresbull.2020.111117
Šuljagić M, Vulić P, Jeremić D, Pavlović VB, Filipović S, Kilanski L, Lewinska S, Slawska-Waniewska A, Milenković MR, Nikolić AS, Anđelković L. The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods. in Materials Research Bulletin. 2021;134:111117.
doi:10.1016/j.materresbull.2020.111117 .
Šuljagić, Marija, Vulić, Predrag, Jeremić, Dejan, Pavlović, Vladimir B., Filipović, Suzana, Kilanski, Lukasz, Lewinska, Sabina, Slawska-Waniewska, Anna, Milenković, Milica R., Nikolić, Aleksandar S., Anđelković, Ljubica, "The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods" in Materials Research Bulletin, 134 (2021):111117,
https://doi.org/10.1016/j.materresbull.2020.111117 . .
19
5
18

Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction

Filipović, Suzana; Obradović, Nina; Anđelković, Ljubica; Olćan, Dragan; Petrović, Jovana; Mirković, Miljana; Pavlović, Vladimir; Jeremić, Dejan; Vlahović, Branislav; Đorđević, Antonije

(Belgrade : International Institute for the Science of Sintering, 2021)

TY  - JOUR
AU  - Filipović, Suzana
AU  - Obradović, Nina
AU  - Anđelković, Ljubica
AU  - Olćan, Dragan
AU  - Petrović, Jovana
AU  - Mirković, Miljana
AU  - Pavlović, Vladimir
AU  - Jeremić, Dejan
AU  - Vlahović, Branislav
AU  - Đorđević, Antonije
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4356
AB  - Solid-state reaction between BaTiO3 and Fe2O3 was used to produce a multiferroic heterostructure composite. Commercial BaTiO3 and Fe(NO3)3•9H2O were suspended in ethanol for 30 minutes in an ultrasound bath. The prepared mixture was thermally processed at 300 oC for 6 h. Sintering at 1300 oC for 1 h resulted in a mixture of different phases, BaTiO3, BaFe12O19 and Ba12Ti28Fe15O84, which were confirmed by x-ray powder diffraction. A dense microstructure with a small volume fraction of closed porosity was indicated by the scanning electron microscopy, while a homogeneous distribution of Fe ions over BaTiO3 phase was visible from energy dispersive spectroscopy mapping. Doping of BaTiO3 with Fe2O3 resulted in formation of magnetic hexaferrite phases, as confirmed by dielectric measurements that showed a broadened maximum of the permittivity measured as a function of temperature.
PB  - Belgrade : International Institute for the Science of Sintering
T2  - Science of Sintering
T1  - Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction
VL  - 53
SP  - 1
EP  - 8
DO  - 10.2298/SOS2101001F
ER  - 
@article{
author = "Filipović, Suzana and Obradović, Nina and Anđelković, Ljubica and Olćan, Dragan and Petrović, Jovana and Mirković, Miljana and Pavlović, Vladimir and Jeremić, Dejan and Vlahović, Branislav and Đorđević, Antonije",
year = "2021",
abstract = "Solid-state reaction between BaTiO3 and Fe2O3 was used to produce a multiferroic heterostructure composite. Commercial BaTiO3 and Fe(NO3)3•9H2O were suspended in ethanol for 30 minutes in an ultrasound bath. The prepared mixture was thermally processed at 300 oC for 6 h. Sintering at 1300 oC for 1 h resulted in a mixture of different phases, BaTiO3, BaFe12O19 and Ba12Ti28Fe15O84, which were confirmed by x-ray powder diffraction. A dense microstructure with a small volume fraction of closed porosity was indicated by the scanning electron microscopy, while a homogeneous distribution of Fe ions over BaTiO3 phase was visible from energy dispersive spectroscopy mapping. Doping of BaTiO3 with Fe2O3 resulted in formation of magnetic hexaferrite phases, as confirmed by dielectric measurements that showed a broadened maximum of the permittivity measured as a function of temperature.",
publisher = "Belgrade : International Institute for the Science of Sintering",
journal = "Science of Sintering",
title = "Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction",
volume = "53",
pages = "1-8",
doi = "10.2298/SOS2101001F"
}
Filipović, S., Obradović, N., Anđelković, L., Olćan, D., Petrović, J., Mirković, M., Pavlović, V., Jeremić, D., Vlahović, B.,& Đorđević, A.. (2021). Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction. in Science of Sintering
Belgrade : International Institute for the Science of Sintering., 53, 1-8.
https://doi.org/10.2298/SOS2101001F
Filipović S, Obradović N, Anđelković L, Olćan D, Petrović J, Mirković M, Pavlović V, Jeremić D, Vlahović B, Đorđević A. Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction. in Science of Sintering. 2021;53:1-8.
doi:10.2298/SOS2101001F .
Filipović, Suzana, Obradović, Nina, Anđelković, Ljubica, Olćan, Dragan, Petrović, Jovana, Mirković, Miljana, Pavlović, Vladimir, Jeremić, Dejan, Vlahović, Branislav, Đorđević, Antonije, "Multiferroic Heterostructure BaTiO3/ε-Fe2O3 Composite Obtained by in situ Reaction" in Science of Sintering, 53 (2021):1-8,
https://doi.org/10.2298/SOS2101001F . .
2
1

The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods

Šuljagić, Marija; Vulić, Predrag; Jeremić, Dejan; Pavlović, Vladimir B.; Filipović, Suzana; Kilanski, Lukasz; Lewinska, Sabina; Slawska-Waniewska, Anna; Milenković, Milica R.; Nikolić, Aleksandar S.; Anđelković, Ljubica

(Elsevier, 2021)

TY  - JOUR
AU  - Šuljagić, Marija
AU  - Vulić, Predrag
AU  - Jeremić, Dejan
AU  - Pavlović, Vladimir B.
AU  - Filipović, Suzana
AU  - Kilanski, Lukasz
AU  - Lewinska, Sabina
AU  - Slawska-Waniewska, Anna
AU  - Milenković, Milica R.
AU  - Nikolić, Aleksandar S.
AU  - Anđelković, Ljubica
PY  - 2021
UR  - https://cer.ihtm.bg.ac.rs/handle/123456789/4557
AB  - To investigate the magnetic behavior of starch-coated cobalt ferrites, well-established synthetic methods, i.e., coprecipitation, mechanochemical, ultrasonically assisted coprecipitation, microemulsion, and microwave-assisted hydrothermal syntheses were chosen for their preparation. The obtained materials had pure single-phase spinel structures. Scanning and transmission electron microscopy analyses revealed that the morphology of the samples is not uniform, and particle aggregation is a dominant process. Fourier transform infrared spectra and thermogravimetric analysis confirmed the presence of starch in all–coated samples. The unusually higher saturation magnetization of starch-coated samples than their as-prepared analogs, obtained by coprecipitation, ultrasonically assisted coprecipitation, and microwave-assisted hydrothermal methods, might be explained by the Ostwald ripening mechanism induced by the coating process. A decrease in magnetization was noticed for the starch-functionalized nanomaterials synthesized by mechanochemical and microemulsion methods, in comparison to their as-prepared analogs, i.e., the size distribution of such nanoparticles is narrow, and the average diameter of the grains is near critical for the Ostwald ripening process.
PB  - Elsevier
T2  - Materials Research Bulletin
T1  - The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods
VL  - 134
SP  - 111117
DO  - 10.1016/j.materresbull.2020.111117
ER  - 
@article{
author = "Šuljagić, Marija and Vulić, Predrag and Jeremić, Dejan and Pavlović, Vladimir B. and Filipović, Suzana and Kilanski, Lukasz and Lewinska, Sabina and Slawska-Waniewska, Anna and Milenković, Milica R. and Nikolić, Aleksandar S. and Anđelković, Ljubica",
year = "2021",
abstract = "To investigate the magnetic behavior of starch-coated cobalt ferrites, well-established synthetic methods, i.e., coprecipitation, mechanochemical, ultrasonically assisted coprecipitation, microemulsion, and microwave-assisted hydrothermal syntheses were chosen for their preparation. The obtained materials had pure single-phase spinel structures. Scanning and transmission electron microscopy analyses revealed that the morphology of the samples is not uniform, and particle aggregation is a dominant process. Fourier transform infrared spectra and thermogravimetric analysis confirmed the presence of starch in all–coated samples. The unusually higher saturation magnetization of starch-coated samples than their as-prepared analogs, obtained by coprecipitation, ultrasonically assisted coprecipitation, and microwave-assisted hydrothermal methods, might be explained by the Ostwald ripening mechanism induced by the coating process. A decrease in magnetization was noticed for the starch-functionalized nanomaterials synthesized by mechanochemical and microemulsion methods, in comparison to their as-prepared analogs, i.e., the size distribution of such nanoparticles is narrow, and the average diameter of the grains is near critical for the Ostwald ripening process.",
publisher = "Elsevier",
journal = "Materials Research Bulletin",
title = "The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods",
volume = "134",
pages = "111117",
doi = "10.1016/j.materresbull.2020.111117"
}
Šuljagić, M., Vulić, P., Jeremić, D., Pavlović, V. B., Filipović, S., Kilanski, L., Lewinska, S., Slawska-Waniewska, A., Milenković, M. R., Nikolić, A. S.,& Anđelković, L.. (2021). The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods. in Materials Research Bulletin
Elsevier., 134, 111117.
https://doi.org/10.1016/j.materresbull.2020.111117
Šuljagić M, Vulić P, Jeremić D, Pavlović VB, Filipović S, Kilanski L, Lewinska S, Slawska-Waniewska A, Milenković MR, Nikolić AS, Anđelković L. The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods. in Materials Research Bulletin. 2021;134:111117.
doi:10.1016/j.materresbull.2020.111117 .
Šuljagić, Marija, Vulić, Predrag, Jeremić, Dejan, Pavlović, Vladimir B., Filipović, Suzana, Kilanski, Lukasz, Lewinska, Sabina, Slawska-Waniewska, Anna, Milenković, Milica R., Nikolić, Aleksandar S., Anđelković, Ljubica, "The influence of the starch coating on the magnetic properties of nanosized cobalt ferrites obtained by different synthetic methods" in Materials Research Bulletin, 134 (2021):111117,
https://doi.org/10.1016/j.materresbull.2020.111117 . .
19
5
18