Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI
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2022
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The heavy metal and organic pollution caused by mining activities keep attracting attention, thus an economic and efficient treatment for combined pollution is pressing. In this study, the simultaneous removal performance of typical organic flotation reagent 8-hydroxyquinoline (8-HQ) and Cr(VI) was investigated via heterogeneous Fenton process induced by a novel polydopamine (PDA) functionalized attapulgite supported nano sized zero-valent iron (nZVI) composite (PDA/ATP-nZVI). Batch experiments showed that PDA/ATP-nZVI had better catalytic reactivity and reduction ability than both ATP-nZVI and nZVI. Under acidic condition, 96.0% of 8-HQ was degraded accompanied with the 42.5% of total organic carbon (TOC) decrease, while 95.8% of Cr(VI) removal efficiency was accomplished by PDA/ATP-nZVI. PDA not only served as redox mediator in expediting electron transfer, but also acted as electron donor that accelerated transformation from Fe(III) to both dissolved Fe(II) and surface Fe(II), which... resulted in the increased degradation of 8-HQ. The synergic removal behavior between 8-HQ and Cr(VI) was discussed and the reaction mechanism in the persulfate (PS)-PDA/ATP-nZVI system was also explored. This study developed a highly efficient heterogeneous catalyst, and demonstrated that the PS-PDA/ATP-nZVI system had a potential for remediation of mine environment polluted by both heavy metals and organic flotation reagents.
Ključne reči:
Cr(VI) / Fenton / Organic flotation reagents / Polydopamine / Simultaneous removalIzvor:
Journal of Hazardous Materials, 2022, 424, 126698Izdavač:
- Elsevier
Finansiranje / projekti:
- Ministarstvo nauke, tehnološkog razvoja i inovacija Republike Srbije, institucionalno finansiranje - 200026 (Univerzitet u Beogradu, Institut za hemiju, tehnologiju i metalurgiju - IHTM) (RS-MESTD-inst-2020-200026)
- The National Natural Science Foundation of China (41720104007)
- The National Natural Science Foundation of China (41430106)
- The Major National R & D Projects for Chinese Ministry of Science and Technology (2019YFC1803500)
- The International Joint Scientific and Technical Collaboration between People’s Republic of China and the Republic of Serbia as part of the Project number 4-18
DOI: 10.1016/j.jhazmat.2021.126698
ISSN: 0304-3894; 1873-3336
PubMed: 34315632
WoS: 000734391000001
Scopus: 2-s2.0-85111599948
Institucija/grupa
IHTMTY - JOUR AU - Ma, Bo AU - Yao, Jun AU - Šolević Knudsen, Tatjana AU - Chen, Zhihui AU - Liu, Bang AU - Zhao, Chenchen AU - Zhu, Xiaozhe PY - 2022 UR - https://cer.ihtm.bg.ac.rs/handle/123456789/5405 AB - The heavy metal and organic pollution caused by mining activities keep attracting attention, thus an economic and efficient treatment for combined pollution is pressing. In this study, the simultaneous removal performance of typical organic flotation reagent 8-hydroxyquinoline (8-HQ) and Cr(VI) was investigated via heterogeneous Fenton process induced by a novel polydopamine (PDA) functionalized attapulgite supported nano sized zero-valent iron (nZVI) composite (PDA/ATP-nZVI). Batch experiments showed that PDA/ATP-nZVI had better catalytic reactivity and reduction ability than both ATP-nZVI and nZVI. Under acidic condition, 96.0% of 8-HQ was degraded accompanied with the 42.5% of total organic carbon (TOC) decrease, while 95.8% of Cr(VI) removal efficiency was accomplished by PDA/ATP-nZVI. PDA not only served as redox mediator in expediting electron transfer, but also acted as electron donor that accelerated transformation from Fe(III) to both dissolved Fe(II) and surface Fe(II), which resulted in the increased degradation of 8-HQ. The synergic removal behavior between 8-HQ and Cr(VI) was discussed and the reaction mechanism in the persulfate (PS)-PDA/ATP-nZVI system was also explored. This study developed a highly efficient heterogeneous catalyst, and demonstrated that the PS-PDA/ATP-nZVI system had a potential for remediation of mine environment polluted by both heavy metals and organic flotation reagents. PB - Elsevier T2 - Journal of Hazardous Materials T1 - Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI VL - 424 IS - 126698 DO - 10.1016/j.jhazmat.2021.126698 ER -
@article{ author = "Ma, Bo and Yao, Jun and Šolević Knudsen, Tatjana and Chen, Zhihui and Liu, Bang and Zhao, Chenchen and Zhu, Xiaozhe", year = "2022", abstract = "The heavy metal and organic pollution caused by mining activities keep attracting attention, thus an economic and efficient treatment for combined pollution is pressing. In this study, the simultaneous removal performance of typical organic flotation reagent 8-hydroxyquinoline (8-HQ) and Cr(VI) was investigated via heterogeneous Fenton process induced by a novel polydopamine (PDA) functionalized attapulgite supported nano sized zero-valent iron (nZVI) composite (PDA/ATP-nZVI). Batch experiments showed that PDA/ATP-nZVI had better catalytic reactivity and reduction ability than both ATP-nZVI and nZVI. Under acidic condition, 96.0% of 8-HQ was degraded accompanied with the 42.5% of total organic carbon (TOC) decrease, while 95.8% of Cr(VI) removal efficiency was accomplished by PDA/ATP-nZVI. PDA not only served as redox mediator in expediting electron transfer, but also acted as electron donor that accelerated transformation from Fe(III) to both dissolved Fe(II) and surface Fe(II), which resulted in the increased degradation of 8-HQ. The synergic removal behavior between 8-HQ and Cr(VI) was discussed and the reaction mechanism in the persulfate (PS)-PDA/ATP-nZVI system was also explored. This study developed a highly efficient heterogeneous catalyst, and demonstrated that the PS-PDA/ATP-nZVI system had a potential for remediation of mine environment polluted by both heavy metals and organic flotation reagents.", publisher = "Elsevier", journal = "Journal of Hazardous Materials", title = "Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI", volume = "424", number = "126698", doi = "10.1016/j.jhazmat.2021.126698" }
Ma, B., Yao, J., Šolević Knudsen, T., Chen, Z., Liu, B., Zhao, C.,& Zhu, X.. (2022). Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI. in Journal of Hazardous Materials Elsevier., 424(126698). https://doi.org/10.1016/j.jhazmat.2021.126698
Ma B, Yao J, Šolević Knudsen T, Chen Z, Liu B, Zhao C, Zhu X. Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI. in Journal of Hazardous Materials. 2022;424(126698). doi:10.1016/j.jhazmat.2021.126698 .
Ma, Bo, Yao, Jun, Šolević Knudsen, Tatjana, Chen, Zhihui, Liu, Bang, Zhao, Chenchen, Zhu, Xiaozhe, "Simultaneous removal of typical flotation reagent 8-hydroxyquinoline and Cr(VI) through heterogeneous Fenton-like processes mediated by polydopamine functionalized ATP supported nZVI" in Journal of Hazardous Materials, 424, no. 126698 (2022), https://doi.org/10.1016/j.jhazmat.2021.126698 . .