Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor
Apstrakt
The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred tank reactor (CSTR) when inlet concentration and/or flow rate is periodically modulated. The product yield corresponding to periodic operation is defined, expressions for its estimation, based on the NFR method, are derived, and it is used to evaluate the performance improvements due to periodic operation. Part I considers the general nonisothermal case. In Part II, these results are applied to an adiabatic CSTR and used to evaluate possible improvements for the case of the hydrolysis reaction of acetic anhydride.
Ključne reči:
Nonisothermal CSTR / Nonlinear frequency response / Periodic operation / Reactor modeling / Two-input modulationIzvor:
Chemical Engineering & Technology, 2016, 39, 11, 2020-2028Izdavač:
- Wiley
Finansiranje / projekti:
- Razvoj efikasnijih hemijsko-inženjerskih procesa zasnovan na istraživanjima fenomena prenosa i principima intenzifikacije procesa (RS-MESTD-Basic Research (BR or ON)-172022)
- Nanostrukturni funkcionalni i kompozitni materijali u katalitičkim i sorpcionim procesima (RS-MESTD-Integrated and Interdisciplinary Research (IIR or III)-45001)
Napomena:
- This is the peer-reviewed version of the article: Daliborka Nikolić, Andreas Seidel‐Morgenstern, Menka Petkovska, Periodic Operation with Modulation of Inlet Concentration and Flow Rate. Part I: Nonisothermal Continuous Stirred‐Tank Reactor, Chemical Engineering & Technology, 2016, 39, 11, 2020-2028, https://doi.org/10.1002/ceat.201600185
- The published version: https://cer.ihtm.bg.ac.rs/handle/123456789/1889
Povezane informacije:
- Druga verzija
https://cer.ihtm.bg.ac.rs/handle/123456789/1889 - Druga verzija
https://doi.org/10.1002/ceat.201600185
DOI: 10.1002/ceat.201600185
ISSN: 0930-7516
WoS: 000387766900005
Scopus: 2-s2.0-84992128586
Institucija/grupa
IHTMTY - JOUR AU - Nikolić-Paunić, Daliborka AU - Seidel-Morgenstern, Andreas AU - Petkovska, Menka PY - 2016 UR - https://cer.ihtm.bg.ac.rs/handle/123456789/4381 AB - The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred tank reactor (CSTR) when inlet concentration and/or flow rate is periodically modulated. The product yield corresponding to periodic operation is defined, expressions for its estimation, based on the NFR method, are derived, and it is used to evaluate the performance improvements due to periodic operation. Part I considers the general nonisothermal case. In Part II, these results are applied to an adiabatic CSTR and used to evaluate possible improvements for the case of the hydrolysis reaction of acetic anhydride. PB - Wiley T2 - Chemical Engineering & Technology T1 - Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor VL - 39 IS - 11 SP - 2020 EP - 2028 DO - 10.1002/ceat.201600185 ER -
@article{ author = "Nikolić-Paunić, Daliborka and Seidel-Morgenstern, Andreas and Petkovska, Menka", year = "2016", abstract = "The nonlinear frequency response (NFR) method, which is an analytical, fast, and easy method for evaluating the performance of forced periodically operated chemical reactors, was used to investigate possible improvements to a nonisothermal continuous stirred tank reactor (CSTR) when inlet concentration and/or flow rate is periodically modulated. The product yield corresponding to periodic operation is defined, expressions for its estimation, based on the NFR method, are derived, and it is used to evaluate the performance improvements due to periodic operation. Part I considers the general nonisothermal case. In Part II, these results are applied to an adiabatic CSTR and used to evaluate possible improvements for the case of the hydrolysis reaction of acetic anhydride.", publisher = "Wiley", journal = "Chemical Engineering & Technology", title = "Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor", volume = "39", number = "11", pages = "2020-2028", doi = "10.1002/ceat.201600185" }
Nikolić-Paunić, D., Seidel-Morgenstern, A.,& Petkovska, M.. (2016). Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor. in Chemical Engineering & Technology Wiley., 39(11), 2020-2028. https://doi.org/10.1002/ceat.201600185
Nikolić-Paunić D, Seidel-Morgenstern A, Petkovska M. Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor. in Chemical Engineering & Technology. 2016;39(11):2020-2028. doi:10.1002/ceat.201600185 .
Nikolić-Paunić, Daliborka, Seidel-Morgenstern, Andreas, Petkovska, Menka, "Periodic Operation with Modulation of Inlet Concentration and Flow Rate Part I: Nonisothermal Continuous Stirred-Tank Reactor" in Chemical Engineering & Technology, 39, no. 11 (2016):2020-2028, https://doi.org/10.1002/ceat.201600185 . .